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2-Oxoglutarate derivatives can selectively enhance or inhibit the activity of human oxygenases

2-Oxoglutarate (2OG) oxygenases are validated agrochemical and human drug targets. The potential for modulating their activity with 2OG derivatives has not been explored, possibly due to concerns regarding selectivity. We report proof-of-principle studies demonstrating selective enhancement or inhib...

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Autores principales: Nakashima, Yu, Brewitz, Lennart, Tumber, Anthony, Salah, Eidarus, Schofield, Christopher J.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8580996/
https://www.ncbi.nlm.nih.gov/pubmed/34759269
http://dx.doi.org/10.1038/s41467-021-26673-2
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author Nakashima, Yu
Brewitz, Lennart
Tumber, Anthony
Salah, Eidarus
Schofield, Christopher J.
author_facet Nakashima, Yu
Brewitz, Lennart
Tumber, Anthony
Salah, Eidarus
Schofield, Christopher J.
author_sort Nakashima, Yu
collection PubMed
description 2-Oxoglutarate (2OG) oxygenases are validated agrochemical and human drug targets. The potential for modulating their activity with 2OG derivatives has not been explored, possibly due to concerns regarding selectivity. We report proof-of-principle studies demonstrating selective enhancement or inhibition of 2OG oxygenase activity by 2-oxo acids. The human 2OG oxygenases studied, factor inhibiting hypoxia-inducible transcription factor HIF-α (FIH) and aspartate/asparagine-β-hydroxylase (AspH), catalyze C3 hydroxylations of Asp/Asn-residues. Of 35 tested 2OG derivatives, 10 enhance and 17 inhibit FIH activity. Comparison with results for AspH reveals that 2OG derivatives selectively enhance or inhibit FIH or AspH. Comparison of FIH structures complexed with 2OG derivatives to those for AspH provides insight into the basis of the observed selectivity. 2-Oxo acid derivatives have potential as drugs, for use in biomimetic catalysis, and in functional studies. The results suggest that the in vivo activity of 2OG oxygenases may be regulated by natural 2-oxo acids other than 2OG.
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spelling pubmed-85809962021-11-15 2-Oxoglutarate derivatives can selectively enhance or inhibit the activity of human oxygenases Nakashima, Yu Brewitz, Lennart Tumber, Anthony Salah, Eidarus Schofield, Christopher J. Nat Commun Article 2-Oxoglutarate (2OG) oxygenases are validated agrochemical and human drug targets. The potential for modulating their activity with 2OG derivatives has not been explored, possibly due to concerns regarding selectivity. We report proof-of-principle studies demonstrating selective enhancement or inhibition of 2OG oxygenase activity by 2-oxo acids. The human 2OG oxygenases studied, factor inhibiting hypoxia-inducible transcription factor HIF-α (FIH) and aspartate/asparagine-β-hydroxylase (AspH), catalyze C3 hydroxylations of Asp/Asn-residues. Of 35 tested 2OG derivatives, 10 enhance and 17 inhibit FIH activity. Comparison with results for AspH reveals that 2OG derivatives selectively enhance or inhibit FIH or AspH. Comparison of FIH structures complexed with 2OG derivatives to those for AspH provides insight into the basis of the observed selectivity. 2-Oxo acid derivatives have potential as drugs, for use in biomimetic catalysis, and in functional studies. The results suggest that the in vivo activity of 2OG oxygenases may be regulated by natural 2-oxo acids other than 2OG. Nature Publishing Group UK 2021-11-10 /pmc/articles/PMC8580996/ /pubmed/34759269 http://dx.doi.org/10.1038/s41467-021-26673-2 Text en © The Author(s) 2021 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Nakashima, Yu
Brewitz, Lennart
Tumber, Anthony
Salah, Eidarus
Schofield, Christopher J.
2-Oxoglutarate derivatives can selectively enhance or inhibit the activity of human oxygenases
title 2-Oxoglutarate derivatives can selectively enhance or inhibit the activity of human oxygenases
title_full 2-Oxoglutarate derivatives can selectively enhance or inhibit the activity of human oxygenases
title_fullStr 2-Oxoglutarate derivatives can selectively enhance or inhibit the activity of human oxygenases
title_full_unstemmed 2-Oxoglutarate derivatives can selectively enhance or inhibit the activity of human oxygenases
title_short 2-Oxoglutarate derivatives can selectively enhance or inhibit the activity of human oxygenases
title_sort 2-oxoglutarate derivatives can selectively enhance or inhibit the activity of human oxygenases
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8580996/
https://www.ncbi.nlm.nih.gov/pubmed/34759269
http://dx.doi.org/10.1038/s41467-021-26673-2
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