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Observation of giant and tunable thermal diffusivity of a Dirac fluid at room temperature

Conducting materials typically exhibit either diffusive or ballistic charge transport. When electron–electron interactions dominate, a hydrodynamic regime with viscous charge flow emerges(1–13). More stringent conditions eventually yield a quantum-critical Dirac-fluid regime, where electronic heat c...

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Autores principales: Block, Alexander, Principi, Alessandro, Hesp, Niels C. H., Cummings, Aron W., Liebel, Matz, Watanabe, Kenji, Taniguchi, Takashi, Roche, Stephan, Koppens, Frank H. L., van Hulst, Niek F., Tielrooij, Klaas-Jan
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8592840/
https://www.ncbi.nlm.nih.gov/pubmed/34426681
http://dx.doi.org/10.1038/s41565-021-00957-6
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author Block, Alexander
Principi, Alessandro
Hesp, Niels C. H.
Cummings, Aron W.
Liebel, Matz
Watanabe, Kenji
Taniguchi, Takashi
Roche, Stephan
Koppens, Frank H. L.
van Hulst, Niek F.
Tielrooij, Klaas-Jan
author_facet Block, Alexander
Principi, Alessandro
Hesp, Niels C. H.
Cummings, Aron W.
Liebel, Matz
Watanabe, Kenji
Taniguchi, Takashi
Roche, Stephan
Koppens, Frank H. L.
van Hulst, Niek F.
Tielrooij, Klaas-Jan
author_sort Block, Alexander
collection PubMed
description Conducting materials typically exhibit either diffusive or ballistic charge transport. When electron–electron interactions dominate, a hydrodynamic regime with viscous charge flow emerges(1–13). More stringent conditions eventually yield a quantum-critical Dirac-fluid regime, where electronic heat can flow more efficiently than charge(14–22). However, observing and controlling the flow of electronic heat in the hydrodynamic regime at room temperature has so far remained elusive. Here we observe heat transport in graphene in the diffusive and hydrodynamic regimes, and report a controllable transition to the Dirac-fluid regime at room temperature, using carrier temperature and carrier density as control knobs. We introduce the technique of spatiotemporal thermoelectric microscopy with femtosecond temporal and nanometre spatial resolution, which allows for tracking electronic heat spreading. In the diffusive regime, we find a thermal diffusivity of roughly 2,000 cm(2) s(−1), consistent with charge transport. Moreover, within the hydrodynamic time window before momentum relaxation, we observe heat spreading corresponding to a giant diffusivity up to 70,000 cm(2) s(−1), indicative of a Dirac fluid. Our results offer the possibility of further exploration of these interesting physical phenomena and their potential applications in nanoscale thermal management.
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spelling pubmed-85928402021-11-23 Observation of giant and tunable thermal diffusivity of a Dirac fluid at room temperature Block, Alexander Principi, Alessandro Hesp, Niels C. H. Cummings, Aron W. Liebel, Matz Watanabe, Kenji Taniguchi, Takashi Roche, Stephan Koppens, Frank H. L. van Hulst, Niek F. Tielrooij, Klaas-Jan Nat Nanotechnol Letter Conducting materials typically exhibit either diffusive or ballistic charge transport. When electron–electron interactions dominate, a hydrodynamic regime with viscous charge flow emerges(1–13). More stringent conditions eventually yield a quantum-critical Dirac-fluid regime, where electronic heat can flow more efficiently than charge(14–22). However, observing and controlling the flow of electronic heat in the hydrodynamic regime at room temperature has so far remained elusive. Here we observe heat transport in graphene in the diffusive and hydrodynamic regimes, and report a controllable transition to the Dirac-fluid regime at room temperature, using carrier temperature and carrier density as control knobs. We introduce the technique of spatiotemporal thermoelectric microscopy with femtosecond temporal and nanometre spatial resolution, which allows for tracking electronic heat spreading. In the diffusive regime, we find a thermal diffusivity of roughly 2,000 cm(2) s(−1), consistent with charge transport. Moreover, within the hydrodynamic time window before momentum relaxation, we observe heat spreading corresponding to a giant diffusivity up to 70,000 cm(2) s(−1), indicative of a Dirac fluid. Our results offer the possibility of further exploration of these interesting physical phenomena and their potential applications in nanoscale thermal management. Nature Publishing Group UK 2021-08-23 2021 /pmc/articles/PMC8592840/ /pubmed/34426681 http://dx.doi.org/10.1038/s41565-021-00957-6 Text en © The Author(s) 2021 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Letter
Block, Alexander
Principi, Alessandro
Hesp, Niels C. H.
Cummings, Aron W.
Liebel, Matz
Watanabe, Kenji
Taniguchi, Takashi
Roche, Stephan
Koppens, Frank H. L.
van Hulst, Niek F.
Tielrooij, Klaas-Jan
Observation of giant and tunable thermal diffusivity of a Dirac fluid at room temperature
title Observation of giant and tunable thermal diffusivity of a Dirac fluid at room temperature
title_full Observation of giant and tunable thermal diffusivity of a Dirac fluid at room temperature
title_fullStr Observation of giant and tunable thermal diffusivity of a Dirac fluid at room temperature
title_full_unstemmed Observation of giant and tunable thermal diffusivity of a Dirac fluid at room temperature
title_short Observation of giant and tunable thermal diffusivity of a Dirac fluid at room temperature
title_sort observation of giant and tunable thermal diffusivity of a dirac fluid at room temperature
topic Letter
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8592840/
https://www.ncbi.nlm.nih.gov/pubmed/34426681
http://dx.doi.org/10.1038/s41565-021-00957-6
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