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Concept of a fast breeder reactor to transmute MAs and LLFPs

The long-term issues of nuclear power systems are the effective use of uranium resources and the reduction of radioactive waste. Important radioactive wastes are minor actinides (MAs: (237)Np, (241)Am, (243)Am, etc.) and long-lived fission products (LLFPs: (129)I, (99)Tc, (79)Se, etc.). The purpose...

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Detalles Bibliográficos
Autor principal: Wakabayashi, Toshio
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8599852/
https://www.ncbi.nlm.nih.gov/pubmed/34789833
http://dx.doi.org/10.1038/s41598-021-01986-w
Descripción
Sumario:The long-term issues of nuclear power systems are the effective use of uranium resources and the reduction of radioactive waste. Important radioactive wastes are minor actinides (MAs: (237)Np, (241)Am, (243)Am, etc.) and long-lived fission products (LLFPs: (129)I, (99)Tc, (79)Se, etc.). The purpose of this study was to show a concept that can simultaneously achieve the breeding of fissile materials and the transmutation of MAs and LLFPs in one fast reactor. Transmutation was carried out by loading innovative Duplex-type MA fuel in the core region and LLFP-containing moderator in the first layer of the radial blanket. Breeding was achieved in the core and axial blanket. As a result, it was clarified that in this fast breeder reactor, a breeding ratio of approximately 1.1 was obtained, and MAs and LLFPs achieved a support ratio of 1 or more. The transmutation rate was 10.3%/y for (237)Np, 14.1%/y for (241)Am, 9.9%/y for (243)Am, 1.6%/y for (129)I, 0.75%/y for (99)Tc, and 4%/y for (79)Se. By simultaneously breeding fissile materials and transmuting MAs and LLFPs in one fast reactor, it will be possible to solve the long-term issues of the nuclear power reactor system, such as securing nuclear fuel resources and reducing radioactive waste.