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Concept of a fast breeder reactor to transmute MAs and LLFPs

The long-term issues of nuclear power systems are the effective use of uranium resources and the reduction of radioactive waste. Important radioactive wastes are minor actinides (MAs: (237)Np, (241)Am, (243)Am, etc.) and long-lived fission products (LLFPs: (129)I, (99)Tc, (79)Se, etc.). The purpose...

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Autor principal: Wakabayashi, Toshio
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8599852/
https://www.ncbi.nlm.nih.gov/pubmed/34789833
http://dx.doi.org/10.1038/s41598-021-01986-w
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author Wakabayashi, Toshio
author_facet Wakabayashi, Toshio
author_sort Wakabayashi, Toshio
collection PubMed
description The long-term issues of nuclear power systems are the effective use of uranium resources and the reduction of radioactive waste. Important radioactive wastes are minor actinides (MAs: (237)Np, (241)Am, (243)Am, etc.) and long-lived fission products (LLFPs: (129)I, (99)Tc, (79)Se, etc.). The purpose of this study was to show a concept that can simultaneously achieve the breeding of fissile materials and the transmutation of MAs and LLFPs in one fast reactor. Transmutation was carried out by loading innovative Duplex-type MA fuel in the core region and LLFP-containing moderator in the first layer of the radial blanket. Breeding was achieved in the core and axial blanket. As a result, it was clarified that in this fast breeder reactor, a breeding ratio of approximately 1.1 was obtained, and MAs and LLFPs achieved a support ratio of 1 or more. The transmutation rate was 10.3%/y for (237)Np, 14.1%/y for (241)Am, 9.9%/y for (243)Am, 1.6%/y for (129)I, 0.75%/y for (99)Tc, and 4%/y for (79)Se. By simultaneously breeding fissile materials and transmuting MAs and LLFPs in one fast reactor, it will be possible to solve the long-term issues of the nuclear power reactor system, such as securing nuclear fuel resources and reducing radioactive waste.
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spelling pubmed-85998522021-11-19 Concept of a fast breeder reactor to transmute MAs and LLFPs Wakabayashi, Toshio Sci Rep Article The long-term issues of nuclear power systems are the effective use of uranium resources and the reduction of radioactive waste. Important radioactive wastes are minor actinides (MAs: (237)Np, (241)Am, (243)Am, etc.) and long-lived fission products (LLFPs: (129)I, (99)Tc, (79)Se, etc.). The purpose of this study was to show a concept that can simultaneously achieve the breeding of fissile materials and the transmutation of MAs and LLFPs in one fast reactor. Transmutation was carried out by loading innovative Duplex-type MA fuel in the core region and LLFP-containing moderator in the first layer of the radial blanket. Breeding was achieved in the core and axial blanket. As a result, it was clarified that in this fast breeder reactor, a breeding ratio of approximately 1.1 was obtained, and MAs and LLFPs achieved a support ratio of 1 or more. The transmutation rate was 10.3%/y for (237)Np, 14.1%/y for (241)Am, 9.9%/y for (243)Am, 1.6%/y for (129)I, 0.75%/y for (99)Tc, and 4%/y for (79)Se. By simultaneously breeding fissile materials and transmuting MAs and LLFPs in one fast reactor, it will be possible to solve the long-term issues of the nuclear power reactor system, such as securing nuclear fuel resources and reducing radioactive waste. Nature Publishing Group UK 2021-11-17 /pmc/articles/PMC8599852/ /pubmed/34789833 http://dx.doi.org/10.1038/s41598-021-01986-w Text en © The Author(s) 2021 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article's Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article's Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Wakabayashi, Toshio
Concept of a fast breeder reactor to transmute MAs and LLFPs
title Concept of a fast breeder reactor to transmute MAs and LLFPs
title_full Concept of a fast breeder reactor to transmute MAs and LLFPs
title_fullStr Concept of a fast breeder reactor to transmute MAs and LLFPs
title_full_unstemmed Concept of a fast breeder reactor to transmute MAs and LLFPs
title_short Concept of a fast breeder reactor to transmute MAs and LLFPs
title_sort concept of a fast breeder reactor to transmute mas and llfps
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8599852/
https://www.ncbi.nlm.nih.gov/pubmed/34789833
http://dx.doi.org/10.1038/s41598-021-01986-w
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