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Thermal Conductivity of Large-Area Polycrystalline MoSe(2) Films Grown by Chemical Vapor Deposition

[Image: see text] It is of great importance to understand the thermal properties of MoSe(2) films for electronic and optoelectronic applications. In this work, large-area polycrystalline MoSe(2) films are prepared using a low-cost, controllable, large-scale, and repeatable chemical vapor deposition...

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Autores principales: Sun, Jie, Dai, Kai, Xia, Wei, Chen, Junhui, Jiang, Kai, Li, Yawei, Zhang, Jinzhong, Zhu, Liangqing, Shang, Liyan, Hu, Zhigao, Chu, Junhao
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2021
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8600615/
https://www.ncbi.nlm.nih.gov/pubmed/34805681
http://dx.doi.org/10.1021/acsomega.1c03921
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author Sun, Jie
Dai, Kai
Xia, Wei
Chen, Junhui
Jiang, Kai
Li, Yawei
Zhang, Jinzhong
Zhu, Liangqing
Shang, Liyan
Hu, Zhigao
Chu, Junhao
author_facet Sun, Jie
Dai, Kai
Xia, Wei
Chen, Junhui
Jiang, Kai
Li, Yawei
Zhang, Jinzhong
Zhu, Liangqing
Shang, Liyan
Hu, Zhigao
Chu, Junhao
author_sort Sun, Jie
collection PubMed
description [Image: see text] It is of great importance to understand the thermal properties of MoSe(2) films for electronic and optoelectronic applications. In this work, large-area polycrystalline MoSe(2) films are prepared using a low-cost, controllable, large-scale, and repeatable chemical vapor deposition method, which facilitates direct device fabrication. Raman spectra and X-ray diffraction patterns indicate a hexagonal (2H) crystal structure of the MoSe(2) film. Ellipsometric spectra analysis indicates that the optical band gap of the MoSe(2) film is estimated to be ∼1.23 eV. From the analysis of the temperature-dependent and laser-power-dependent Raman spectra, the thermal conductivity of the suspended MoSe(2) films is found to be ∼28.48 W/(m·K) at room temperature. The results can provide useful guidance for an effective thermal management of large-area polycrystalline MoSe(2)-based electronic and optoelectronic devices.
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spelling pubmed-86006152021-11-19 Thermal Conductivity of Large-Area Polycrystalline MoSe(2) Films Grown by Chemical Vapor Deposition Sun, Jie Dai, Kai Xia, Wei Chen, Junhui Jiang, Kai Li, Yawei Zhang, Jinzhong Zhu, Liangqing Shang, Liyan Hu, Zhigao Chu, Junhao ACS Omega [Image: see text] It is of great importance to understand the thermal properties of MoSe(2) films for electronic and optoelectronic applications. In this work, large-area polycrystalline MoSe(2) films are prepared using a low-cost, controllable, large-scale, and repeatable chemical vapor deposition method, which facilitates direct device fabrication. Raman spectra and X-ray diffraction patterns indicate a hexagonal (2H) crystal structure of the MoSe(2) film. Ellipsometric spectra analysis indicates that the optical band gap of the MoSe(2) film is estimated to be ∼1.23 eV. From the analysis of the temperature-dependent and laser-power-dependent Raman spectra, the thermal conductivity of the suspended MoSe(2) films is found to be ∼28.48 W/(m·K) at room temperature. The results can provide useful guidance for an effective thermal management of large-area polycrystalline MoSe(2)-based electronic and optoelectronic devices. American Chemical Society 2021-11-04 /pmc/articles/PMC8600615/ /pubmed/34805681 http://dx.doi.org/10.1021/acsomega.1c03921 Text en © 2021 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by-nc-nd/4.0/Permits non-commercial access and re-use, provided that author attribution and integrity are maintained; but does not permit creation of adaptations or other derivative works (https://creativecommons.org/licenses/by-nc-nd/4.0/).
spellingShingle Sun, Jie
Dai, Kai
Xia, Wei
Chen, Junhui
Jiang, Kai
Li, Yawei
Zhang, Jinzhong
Zhu, Liangqing
Shang, Liyan
Hu, Zhigao
Chu, Junhao
Thermal Conductivity of Large-Area Polycrystalline MoSe(2) Films Grown by Chemical Vapor Deposition
title Thermal Conductivity of Large-Area Polycrystalline MoSe(2) Films Grown by Chemical Vapor Deposition
title_full Thermal Conductivity of Large-Area Polycrystalline MoSe(2) Films Grown by Chemical Vapor Deposition
title_fullStr Thermal Conductivity of Large-Area Polycrystalline MoSe(2) Films Grown by Chemical Vapor Deposition
title_full_unstemmed Thermal Conductivity of Large-Area Polycrystalline MoSe(2) Films Grown by Chemical Vapor Deposition
title_short Thermal Conductivity of Large-Area Polycrystalline MoSe(2) Films Grown by Chemical Vapor Deposition
title_sort thermal conductivity of large-area polycrystalline mose(2) films grown by chemical vapor deposition
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8600615/
https://www.ncbi.nlm.nih.gov/pubmed/34805681
http://dx.doi.org/10.1021/acsomega.1c03921
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