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SrSnO(3)-Assembled MWCNT Heterojunctions for Superior Hydrogen Production under Visible Light

[Image: see text] A one-step sol–gel method for SrSnO(3) nanoparticle synthesis and the incorporation of multi-walled carbon nanotubes (MWCNTs) to produce a SrSnO(3)@MWCNT photocatalyst is presented. The incorporation of MWCNTs results in enhancement of structural, optical, and optoelectrical proper...

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Detalles Bibliográficos
Autores principales: Kadi, Mohammad W., Mohamed, Reda M.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2021
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8600627/
https://www.ncbi.nlm.nih.gov/pubmed/34805682
http://dx.doi.org/10.1021/acsomega.1c04143
Descripción
Sumario:[Image: see text] A one-step sol–gel method for SrSnO(3) nanoparticle synthesis and the incorporation of multi-walled carbon nanotubes (MWCNTs) to produce a SrSnO(3)@MWCNT photocatalyst is presented. The incorporation of MWCNTs results in enhancement of structural, optical, and optoelectrical properties of SrSnO(3). The optimized 3.0% addition of MWCNTs results in light absorption enhancement and a reduction of the band gap from 3.68 to 2.85 eV. Upon application of the photocatalyst in the photocatalytic hydrogen production reaction, SrSnO(3)@MWCNT-3.0% yields 4200 μmol g(–1) of H(2) in just 9 h with the use of 1.6 g L(–1) of the photocatalyst. SrSnO(3)@MWCNT exhibits remarkable chemical and photocatalytic stability upon regeneration. Enhanced photocatalytic ability is attributed to improved surface properties and charge-carrier recombination suppression induced by the MWCNT addition. This study highlights the remarkable improvements in chemical and physical properties of semiconductors with MWCNT incorporation.