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SrSnO(3)-Assembled MWCNT Heterojunctions for Superior Hydrogen Production under Visible Light
[Image: see text] A one-step sol–gel method for SrSnO(3) nanoparticle synthesis and the incorporation of multi-walled carbon nanotubes (MWCNTs) to produce a SrSnO(3)@MWCNT photocatalyst is presented. The incorporation of MWCNTs results in enhancement of structural, optical, and optoelectrical proper...
Autores principales: | , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Chemical Society
2021
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Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8600627/ https://www.ncbi.nlm.nih.gov/pubmed/34805682 http://dx.doi.org/10.1021/acsomega.1c04143 |
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author | Kadi, Mohammad W. Mohamed, Reda M. |
author_facet | Kadi, Mohammad W. Mohamed, Reda M. |
author_sort | Kadi, Mohammad W. |
collection | PubMed |
description | [Image: see text] A one-step sol–gel method for SrSnO(3) nanoparticle synthesis and the incorporation of multi-walled carbon nanotubes (MWCNTs) to produce a SrSnO(3)@MWCNT photocatalyst is presented. The incorporation of MWCNTs results in enhancement of structural, optical, and optoelectrical properties of SrSnO(3). The optimized 3.0% addition of MWCNTs results in light absorption enhancement and a reduction of the band gap from 3.68 to 2.85 eV. Upon application of the photocatalyst in the photocatalytic hydrogen production reaction, SrSnO(3)@MWCNT-3.0% yields 4200 μmol g(–1) of H(2) in just 9 h with the use of 1.6 g L(–1) of the photocatalyst. SrSnO(3)@MWCNT exhibits remarkable chemical and photocatalytic stability upon regeneration. Enhanced photocatalytic ability is attributed to improved surface properties and charge-carrier recombination suppression induced by the MWCNT addition. This study highlights the remarkable improvements in chemical and physical properties of semiconductors with MWCNT incorporation. |
format | Online Article Text |
id | pubmed-8600627 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2021 |
publisher | American Chemical Society |
record_format | MEDLINE/PubMed |
spelling | pubmed-86006272021-11-19 SrSnO(3)-Assembled MWCNT Heterojunctions for Superior Hydrogen Production under Visible Light Kadi, Mohammad W. Mohamed, Reda M. ACS Omega [Image: see text] A one-step sol–gel method for SrSnO(3) nanoparticle synthesis and the incorporation of multi-walled carbon nanotubes (MWCNTs) to produce a SrSnO(3)@MWCNT photocatalyst is presented. The incorporation of MWCNTs results in enhancement of structural, optical, and optoelectrical properties of SrSnO(3). The optimized 3.0% addition of MWCNTs results in light absorption enhancement and a reduction of the band gap from 3.68 to 2.85 eV. Upon application of the photocatalyst in the photocatalytic hydrogen production reaction, SrSnO(3)@MWCNT-3.0% yields 4200 μmol g(–1) of H(2) in just 9 h with the use of 1.6 g L(–1) of the photocatalyst. SrSnO(3)@MWCNT exhibits remarkable chemical and photocatalytic stability upon regeneration. Enhanced photocatalytic ability is attributed to improved surface properties and charge-carrier recombination suppression induced by the MWCNT addition. This study highlights the remarkable improvements in chemical and physical properties of semiconductors with MWCNT incorporation. American Chemical Society 2021-11-05 /pmc/articles/PMC8600627/ /pubmed/34805682 http://dx.doi.org/10.1021/acsomega.1c04143 Text en © 2021 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by-nc-nd/4.0/Permits non-commercial access and re-use, provided that author attribution and integrity are maintained; but does not permit creation of adaptations or other derivative works (https://creativecommons.org/licenses/by-nc-nd/4.0/). |
spellingShingle | Kadi, Mohammad W. Mohamed, Reda M. SrSnO(3)-Assembled MWCNT Heterojunctions for Superior Hydrogen Production under Visible Light |
title | SrSnO(3)-Assembled MWCNT Heterojunctions
for Superior Hydrogen Production under Visible Light |
title_full | SrSnO(3)-Assembled MWCNT Heterojunctions
for Superior Hydrogen Production under Visible Light |
title_fullStr | SrSnO(3)-Assembled MWCNT Heterojunctions
for Superior Hydrogen Production under Visible Light |
title_full_unstemmed | SrSnO(3)-Assembled MWCNT Heterojunctions
for Superior Hydrogen Production under Visible Light |
title_short | SrSnO(3)-Assembled MWCNT Heterojunctions
for Superior Hydrogen Production under Visible Light |
title_sort | srsno(3)-assembled mwcnt heterojunctions
for superior hydrogen production under visible light |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8600627/ https://www.ncbi.nlm.nih.gov/pubmed/34805682 http://dx.doi.org/10.1021/acsomega.1c04143 |
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