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SrSnO(3)-Assembled MWCNT Heterojunctions for Superior Hydrogen Production under Visible Light

[Image: see text] A one-step sol–gel method for SrSnO(3) nanoparticle synthesis and the incorporation of multi-walled carbon nanotubes (MWCNTs) to produce a SrSnO(3)@MWCNT photocatalyst is presented. The incorporation of MWCNTs results in enhancement of structural, optical, and optoelectrical proper...

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Autores principales: Kadi, Mohammad W., Mohamed, Reda M.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2021
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8600627/
https://www.ncbi.nlm.nih.gov/pubmed/34805682
http://dx.doi.org/10.1021/acsomega.1c04143
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author Kadi, Mohammad W.
Mohamed, Reda M.
author_facet Kadi, Mohammad W.
Mohamed, Reda M.
author_sort Kadi, Mohammad W.
collection PubMed
description [Image: see text] A one-step sol–gel method for SrSnO(3) nanoparticle synthesis and the incorporation of multi-walled carbon nanotubes (MWCNTs) to produce a SrSnO(3)@MWCNT photocatalyst is presented. The incorporation of MWCNTs results in enhancement of structural, optical, and optoelectrical properties of SrSnO(3). The optimized 3.0% addition of MWCNTs results in light absorption enhancement and a reduction of the band gap from 3.68 to 2.85 eV. Upon application of the photocatalyst in the photocatalytic hydrogen production reaction, SrSnO(3)@MWCNT-3.0% yields 4200 μmol g(–1) of H(2) in just 9 h with the use of 1.6 g L(–1) of the photocatalyst. SrSnO(3)@MWCNT exhibits remarkable chemical and photocatalytic stability upon regeneration. Enhanced photocatalytic ability is attributed to improved surface properties and charge-carrier recombination suppression induced by the MWCNT addition. This study highlights the remarkable improvements in chemical and physical properties of semiconductors with MWCNT incorporation.
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spelling pubmed-86006272021-11-19 SrSnO(3)-Assembled MWCNT Heterojunctions for Superior Hydrogen Production under Visible Light Kadi, Mohammad W. Mohamed, Reda M. ACS Omega [Image: see text] A one-step sol–gel method for SrSnO(3) nanoparticle synthesis and the incorporation of multi-walled carbon nanotubes (MWCNTs) to produce a SrSnO(3)@MWCNT photocatalyst is presented. The incorporation of MWCNTs results in enhancement of structural, optical, and optoelectrical properties of SrSnO(3). The optimized 3.0% addition of MWCNTs results in light absorption enhancement and a reduction of the band gap from 3.68 to 2.85 eV. Upon application of the photocatalyst in the photocatalytic hydrogen production reaction, SrSnO(3)@MWCNT-3.0% yields 4200 μmol g(–1) of H(2) in just 9 h with the use of 1.6 g L(–1) of the photocatalyst. SrSnO(3)@MWCNT exhibits remarkable chemical and photocatalytic stability upon regeneration. Enhanced photocatalytic ability is attributed to improved surface properties and charge-carrier recombination suppression induced by the MWCNT addition. This study highlights the remarkable improvements in chemical and physical properties of semiconductors with MWCNT incorporation. American Chemical Society 2021-11-05 /pmc/articles/PMC8600627/ /pubmed/34805682 http://dx.doi.org/10.1021/acsomega.1c04143 Text en © 2021 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by-nc-nd/4.0/Permits non-commercial access and re-use, provided that author attribution and integrity are maintained; but does not permit creation of adaptations or other derivative works (https://creativecommons.org/licenses/by-nc-nd/4.0/).
spellingShingle Kadi, Mohammad W.
Mohamed, Reda M.
SrSnO(3)-Assembled MWCNT Heterojunctions for Superior Hydrogen Production under Visible Light
title SrSnO(3)-Assembled MWCNT Heterojunctions for Superior Hydrogen Production under Visible Light
title_full SrSnO(3)-Assembled MWCNT Heterojunctions for Superior Hydrogen Production under Visible Light
title_fullStr SrSnO(3)-Assembled MWCNT Heterojunctions for Superior Hydrogen Production under Visible Light
title_full_unstemmed SrSnO(3)-Assembled MWCNT Heterojunctions for Superior Hydrogen Production under Visible Light
title_short SrSnO(3)-Assembled MWCNT Heterojunctions for Superior Hydrogen Production under Visible Light
title_sort srsno(3)-assembled mwcnt heterojunctions for superior hydrogen production under visible light
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8600627/
https://www.ncbi.nlm.nih.gov/pubmed/34805682
http://dx.doi.org/10.1021/acsomega.1c04143
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