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Tomographic mapping of the hidden dimension in quasi-particle interference

Quasiparticle interference (QPI) imaging is well established to study the low-energy electronic structure in strongly correlated electron materials with unrivalled energy resolution. Yet, being a surface-sensitive technique, the interpretation of QPI only works well for anisotropic materials, where...

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Autores principales: Marques, C. A., Bahramy, M. S., Trainer, C., Marković, I., Watson, M. D., Mazzola, F., Rajan, A., Raub, T. D., King, P. D. C., Wahl, P.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8602440/
https://www.ncbi.nlm.nih.gov/pubmed/34795276
http://dx.doi.org/10.1038/s41467-021-27082-1
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author Marques, C. A.
Bahramy, M. S.
Trainer, C.
Marković, I.
Watson, M. D.
Mazzola, F.
Rajan, A.
Raub, T. D.
King, P. D. C.
Wahl, P.
author_facet Marques, C. A.
Bahramy, M. S.
Trainer, C.
Marković, I.
Watson, M. D.
Mazzola, F.
Rajan, A.
Raub, T. D.
King, P. D. C.
Wahl, P.
author_sort Marques, C. A.
collection PubMed
description Quasiparticle interference (QPI) imaging is well established to study the low-energy electronic structure in strongly correlated electron materials with unrivalled energy resolution. Yet, being a surface-sensitive technique, the interpretation of QPI only works well for anisotropic materials, where the dispersion in the direction perpendicular to the surface can be neglected and the quasiparticle interference is dominated by a quasi-2D electronic structure. Here, we explore QPI imaging of galena, a material with an electronic structure that does not exhibit pronounced anisotropy. We find that the quasiparticle interference signal is dominated by scattering vectors which are parallel to the surface plane however originate from bias-dependent cuts of the 3D electronic structure. We develop a formalism for the theoretical description of the QPI signal and demonstrate how this quasiparticle tomography can be used to obtain information about the 3D electronic structure and orbital character of the bands.
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spelling pubmed-86024402021-12-03 Tomographic mapping of the hidden dimension in quasi-particle interference Marques, C. A. Bahramy, M. S. Trainer, C. Marković, I. Watson, M. D. Mazzola, F. Rajan, A. Raub, T. D. King, P. D. C. Wahl, P. Nat Commun Article Quasiparticle interference (QPI) imaging is well established to study the low-energy electronic structure in strongly correlated electron materials with unrivalled energy resolution. Yet, being a surface-sensitive technique, the interpretation of QPI only works well for anisotropic materials, where the dispersion in the direction perpendicular to the surface can be neglected and the quasiparticle interference is dominated by a quasi-2D electronic structure. Here, we explore QPI imaging of galena, a material with an electronic structure that does not exhibit pronounced anisotropy. We find that the quasiparticle interference signal is dominated by scattering vectors which are parallel to the surface plane however originate from bias-dependent cuts of the 3D electronic structure. We develop a formalism for the theoretical description of the QPI signal and demonstrate how this quasiparticle tomography can be used to obtain information about the 3D electronic structure and orbital character of the bands. Nature Publishing Group UK 2021-11-18 /pmc/articles/PMC8602440/ /pubmed/34795276 http://dx.doi.org/10.1038/s41467-021-27082-1 Text en © The Author(s) 2021 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Marques, C. A.
Bahramy, M. S.
Trainer, C.
Marković, I.
Watson, M. D.
Mazzola, F.
Rajan, A.
Raub, T. D.
King, P. D. C.
Wahl, P.
Tomographic mapping of the hidden dimension in quasi-particle interference
title Tomographic mapping of the hidden dimension in quasi-particle interference
title_full Tomographic mapping of the hidden dimension in quasi-particle interference
title_fullStr Tomographic mapping of the hidden dimension in quasi-particle interference
title_full_unstemmed Tomographic mapping of the hidden dimension in quasi-particle interference
title_short Tomographic mapping of the hidden dimension in quasi-particle interference
title_sort tomographic mapping of the hidden dimension in quasi-particle interference
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8602440/
https://www.ncbi.nlm.nih.gov/pubmed/34795276
http://dx.doi.org/10.1038/s41467-021-27082-1
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