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Unleashing nanofabrication through thermomechanical nanomolding

Advancements in nanotechnology require the development of nanofabrication methods for a wide range of materials, length scales, and elemental distributions. Today’s nanofabrication methods are typically missing at least one demanded characteristic. Hence, a general method enabling versatile nanofabr...

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Autores principales: Liu, Naijia, Liu, Guannan, Raj, Arindam, Sohn, Sungwoo, Morales-Acosta, Mayra Daniela, Liu, Jingbei, Schroers, Jan
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Association for the Advancement of Science 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8604398/
https://www.ncbi.nlm.nih.gov/pubmed/34797709
http://dx.doi.org/10.1126/sciadv.abi4567
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author Liu, Naijia
Liu, Guannan
Raj, Arindam
Sohn, Sungwoo
Morales-Acosta, Mayra Daniela
Liu, Jingbei
Schroers, Jan
author_facet Liu, Naijia
Liu, Guannan
Raj, Arindam
Sohn, Sungwoo
Morales-Acosta, Mayra Daniela
Liu, Jingbei
Schroers, Jan
author_sort Liu, Naijia
collection PubMed
description Advancements in nanotechnology require the development of nanofabrication methods for a wide range of materials, length scales, and elemental distributions. Today’s nanofabrication methods are typically missing at least one demanded characteristic. Hence, a general method enabling versatile nanofabrication remains elusive. Here, we show that, when revealing and using the underlying mechanisms of thermomechanical nanomolding, a highly versatile nanofabrication toolbox is the result. Specifically, we reveal interface diffusion and dislocation slip as the controlling mechanisms and use their transition to control, combine, and predict the ability to fabricate general materials, material combinations, and length scales. Designing specific elemental distributions is based on the relative diffusivities, the transition temperature, and the distribution of the materials in the feedstock. The mechanistic origins of thermomechanical nanomolding and their homologous temperature-dependent transition suggest a versatile toolbox capable of combining many materials in nanostructures and potentially producing any material in moldable shapes on the nanoscale.
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spelling pubmed-86043982021-12-01 Unleashing nanofabrication through thermomechanical nanomolding Liu, Naijia Liu, Guannan Raj, Arindam Sohn, Sungwoo Morales-Acosta, Mayra Daniela Liu, Jingbei Schroers, Jan Sci Adv Physical and Materials Sciences Advancements in nanotechnology require the development of nanofabrication methods for a wide range of materials, length scales, and elemental distributions. Today’s nanofabrication methods are typically missing at least one demanded characteristic. Hence, a general method enabling versatile nanofabrication remains elusive. Here, we show that, when revealing and using the underlying mechanisms of thermomechanical nanomolding, a highly versatile nanofabrication toolbox is the result. Specifically, we reveal interface diffusion and dislocation slip as the controlling mechanisms and use their transition to control, combine, and predict the ability to fabricate general materials, material combinations, and length scales. Designing specific elemental distributions is based on the relative diffusivities, the transition temperature, and the distribution of the materials in the feedstock. The mechanistic origins of thermomechanical nanomolding and their homologous temperature-dependent transition suggest a versatile toolbox capable of combining many materials in nanostructures and potentially producing any material in moldable shapes on the nanoscale. American Association for the Advancement of Science 2021-11-19 /pmc/articles/PMC8604398/ /pubmed/34797709 http://dx.doi.org/10.1126/sciadv.abi4567 Text en Copyright © 2021 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution License 4.0 (CC BY). https://creativecommons.org/licenses/by/4.0/This is an open-access article distributed under the terms of the Creative Commons Attribution license (https://creativecommons.org/licenses/by/4.0/) , which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited.
spellingShingle Physical and Materials Sciences
Liu, Naijia
Liu, Guannan
Raj, Arindam
Sohn, Sungwoo
Morales-Acosta, Mayra Daniela
Liu, Jingbei
Schroers, Jan
Unleashing nanofabrication through thermomechanical nanomolding
title Unleashing nanofabrication through thermomechanical nanomolding
title_full Unleashing nanofabrication through thermomechanical nanomolding
title_fullStr Unleashing nanofabrication through thermomechanical nanomolding
title_full_unstemmed Unleashing nanofabrication through thermomechanical nanomolding
title_short Unleashing nanofabrication through thermomechanical nanomolding
title_sort unleashing nanofabrication through thermomechanical nanomolding
topic Physical and Materials Sciences
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8604398/
https://www.ncbi.nlm.nih.gov/pubmed/34797709
http://dx.doi.org/10.1126/sciadv.abi4567
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