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Selective Deposition of Candle Soot on a Cellulose Membrane for Efficient Solar Evaporation

[Image: see text] Owing to their natural abundance, seawater together with sunlight has a potential to meet the global challenges in terms of water scarcity and energy crisis. Herein, we demonstrate a solar vapor generator composed of an inner flame candle soot (IFCS) deposited on a cellulose filter...

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Autores principales: Rashid, Mamoon Ur, Tahir, Zeeshan, Kim, Sungdo, Jang, Joon I., Kim, Yong Soo
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2021
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8613860/
https://www.ncbi.nlm.nih.gov/pubmed/34841180
http://dx.doi.org/10.1021/acsomega.1c05348
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author Rashid, Mamoon Ur
Tahir, Zeeshan
Kim, Sungdo
Jang, Joon I.
Kim, Yong Soo
author_facet Rashid, Mamoon Ur
Tahir, Zeeshan
Kim, Sungdo
Jang, Joon I.
Kim, Yong Soo
author_sort Rashid, Mamoon Ur
collection PubMed
description [Image: see text] Owing to their natural abundance, seawater together with sunlight has a potential to meet the global challenges in terms of water scarcity and energy crisis. Herein, we demonstrate a solar vapor generator composed of an inner flame candle soot (IFCS) deposited on a cellulose filter paper (FP) prepared by a simple two-step process. The resultant IFCS/FP device exhibits a high photothermal conversion ability owing to the broadband solar absorption of the IFCS layer along with the multiple scattering of the incoming sunlight in the porous microstructure of the cellulose FP. Additionally, the low thermal conductivity of the IFCS effectively localizes the photothermally generated heat at the IFCS/FP surface, thereby significantly suppressing the conduction heat losses to the underlying bulk water. Meanwhile, the capillary action of the FP supplies an adequate amount of water to the heated surface for accelerating the evaporation process. Benefitting from the synergistic effect of these characteristics, the IFCS/FP achieves high evaporation rates of ∼1.16 and ∼4.09 kg m(–2) h(–1) and their corresponding efficiencies of ∼75.1 and 90.9% under one and three sun illumination, respectively. Moreover, the IFCS/FP device presents an excellent longevity owing to the persistent performance over 15 repeated cycles under one and three sun illumination. Hence, the facile fabrication, fine mechanical strength, desalination, and the salt-resistance ability of our IFCS/FP make it a suitable candidate for practical applications.
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spelling pubmed-86138602021-11-26 Selective Deposition of Candle Soot on a Cellulose Membrane for Efficient Solar Evaporation Rashid, Mamoon Ur Tahir, Zeeshan Kim, Sungdo Jang, Joon I. Kim, Yong Soo ACS Omega [Image: see text] Owing to their natural abundance, seawater together with sunlight has a potential to meet the global challenges in terms of water scarcity and energy crisis. Herein, we demonstrate a solar vapor generator composed of an inner flame candle soot (IFCS) deposited on a cellulose filter paper (FP) prepared by a simple two-step process. The resultant IFCS/FP device exhibits a high photothermal conversion ability owing to the broadband solar absorption of the IFCS layer along with the multiple scattering of the incoming sunlight in the porous microstructure of the cellulose FP. Additionally, the low thermal conductivity of the IFCS effectively localizes the photothermally generated heat at the IFCS/FP surface, thereby significantly suppressing the conduction heat losses to the underlying bulk water. Meanwhile, the capillary action of the FP supplies an adequate amount of water to the heated surface for accelerating the evaporation process. Benefitting from the synergistic effect of these characteristics, the IFCS/FP achieves high evaporation rates of ∼1.16 and ∼4.09 kg m(–2) h(–1) and their corresponding efficiencies of ∼75.1 and 90.9% under one and three sun illumination, respectively. Moreover, the IFCS/FP device presents an excellent longevity owing to the persistent performance over 15 repeated cycles under one and three sun illumination. Hence, the facile fabrication, fine mechanical strength, desalination, and the salt-resistance ability of our IFCS/FP make it a suitable candidate for practical applications. American Chemical Society 2021-11-11 /pmc/articles/PMC8613860/ /pubmed/34841180 http://dx.doi.org/10.1021/acsomega.1c05348 Text en © 2021 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by-nc-nd/4.0/Permits non-commercial access and re-use, provided that author attribution and integrity are maintained; but does not permit creation of adaptations or other derivative works (https://creativecommons.org/licenses/by-nc-nd/4.0/).
spellingShingle Rashid, Mamoon Ur
Tahir, Zeeshan
Kim, Sungdo
Jang, Joon I.
Kim, Yong Soo
Selective Deposition of Candle Soot on a Cellulose Membrane for Efficient Solar Evaporation
title Selective Deposition of Candle Soot on a Cellulose Membrane for Efficient Solar Evaporation
title_full Selective Deposition of Candle Soot on a Cellulose Membrane for Efficient Solar Evaporation
title_fullStr Selective Deposition of Candle Soot on a Cellulose Membrane for Efficient Solar Evaporation
title_full_unstemmed Selective Deposition of Candle Soot on a Cellulose Membrane for Efficient Solar Evaporation
title_short Selective Deposition of Candle Soot on a Cellulose Membrane for Efficient Solar Evaporation
title_sort selective deposition of candle soot on a cellulose membrane for efficient solar evaporation
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8613860/
https://www.ncbi.nlm.nih.gov/pubmed/34841180
http://dx.doi.org/10.1021/acsomega.1c05348
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