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Applied Artificial Neural Network for Hydrogen Sulfide Solubility in Natural Gas Purification
[Image: see text] Solubility of hydrogen sulfide (H(2)S) in 46 single and blended physical absorbents, amines, ionic liquids, and hybrid absorbents of amines + ionic liquids and amines + physical absorbents was successfully predicted based on artificial neural networks (ANNs). Three neural network a...
Autores principales: | , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Chemical Society
2021
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Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8613862/ https://www.ncbi.nlm.nih.gov/pubmed/34841175 http://dx.doi.org/10.1021/acsomega.1c05169 |
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author | Nimmanterdwong, Prathana Changpun, Rachaneeporn Janthboon, Patipon Nakrak, Sukanya Gao, Hongxia Liang, Zhiwu Tontiwachwuthikul, Paitoon Sema, Teerawat |
author_facet | Nimmanterdwong, Prathana Changpun, Rachaneeporn Janthboon, Patipon Nakrak, Sukanya Gao, Hongxia Liang, Zhiwu Tontiwachwuthikul, Paitoon Sema, Teerawat |
author_sort | Nimmanterdwong, Prathana |
collection | PubMed |
description | [Image: see text] Solubility of hydrogen sulfide (H(2)S) in 46 single and blended physical absorbents, amines, ionic liquids, and hybrid absorbents of amines + ionic liquids and amines + physical absorbents was successfully predicted based on artificial neural networks (ANNs). Three neural network algorithms of Levenberg–Marquardt (LM), Bayesian regularization (BR), and scaled conjugate gradient (SCG) were applied for architecting the ANN models. The results showed that both the number of hidden neurons and the prediction algorithm affected the prediction of H(2)S solubility. Based on the mean square error (MSE) and determination coefficient (R(2)), the most attractive model was the LM-ANN model with 17 hidden neurons. As a result, very satisfactory prediction performance (for the testing data set) with an MSE of 0.0014 and an R(2) of 0.9817 was obtained from the developed LM-ANN model. Additionally, a parity chart confirmed that the predicted solubility of H(2)S well aligned with the experimental data. To effectively absorb H(2)S and maintain high solubility of H(2)S, the absorbent should be well complied with the operating pressure. For a low-pressure range of less than 100 kPa, amines are very attractive. As the pressure elevated to 100–1000 kPa, amines and hybrid amine + physical absorbents are suggested. Lastly, at a high pressure over 1000 kPa, physical absorbents and ionic liquids are recommended. |
format | Online Article Text |
id | pubmed-8613862 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2021 |
publisher | American Chemical Society |
record_format | MEDLINE/PubMed |
spelling | pubmed-86138622021-11-26 Applied Artificial Neural Network for Hydrogen Sulfide Solubility in Natural Gas Purification Nimmanterdwong, Prathana Changpun, Rachaneeporn Janthboon, Patipon Nakrak, Sukanya Gao, Hongxia Liang, Zhiwu Tontiwachwuthikul, Paitoon Sema, Teerawat ACS Omega [Image: see text] Solubility of hydrogen sulfide (H(2)S) in 46 single and blended physical absorbents, amines, ionic liquids, and hybrid absorbents of amines + ionic liquids and amines + physical absorbents was successfully predicted based on artificial neural networks (ANNs). Three neural network algorithms of Levenberg–Marquardt (LM), Bayesian regularization (BR), and scaled conjugate gradient (SCG) were applied for architecting the ANN models. The results showed that both the number of hidden neurons and the prediction algorithm affected the prediction of H(2)S solubility. Based on the mean square error (MSE) and determination coefficient (R(2)), the most attractive model was the LM-ANN model with 17 hidden neurons. As a result, very satisfactory prediction performance (for the testing data set) with an MSE of 0.0014 and an R(2) of 0.9817 was obtained from the developed LM-ANN model. Additionally, a parity chart confirmed that the predicted solubility of H(2)S well aligned with the experimental data. To effectively absorb H(2)S and maintain high solubility of H(2)S, the absorbent should be well complied with the operating pressure. For a low-pressure range of less than 100 kPa, amines are very attractive. As the pressure elevated to 100–1000 kPa, amines and hybrid amine + physical absorbents are suggested. Lastly, at a high pressure over 1000 kPa, physical absorbents and ionic liquids are recommended. American Chemical Society 2021-11-10 /pmc/articles/PMC8613862/ /pubmed/34841175 http://dx.doi.org/10.1021/acsomega.1c05169 Text en © 2021 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by-nc-nd/4.0/Permits non-commercial access and re-use, provided that author attribution and integrity are maintained; but does not permit creation of adaptations or other derivative works (https://creativecommons.org/licenses/by-nc-nd/4.0/). |
spellingShingle | Nimmanterdwong, Prathana Changpun, Rachaneeporn Janthboon, Patipon Nakrak, Sukanya Gao, Hongxia Liang, Zhiwu Tontiwachwuthikul, Paitoon Sema, Teerawat Applied Artificial Neural Network for Hydrogen Sulfide Solubility in Natural Gas Purification |
title | Applied Artificial Neural Network for Hydrogen Sulfide
Solubility in Natural Gas Purification |
title_full | Applied Artificial Neural Network for Hydrogen Sulfide
Solubility in Natural Gas Purification |
title_fullStr | Applied Artificial Neural Network for Hydrogen Sulfide
Solubility in Natural Gas Purification |
title_full_unstemmed | Applied Artificial Neural Network for Hydrogen Sulfide
Solubility in Natural Gas Purification |
title_short | Applied Artificial Neural Network for Hydrogen Sulfide
Solubility in Natural Gas Purification |
title_sort | applied artificial neural network for hydrogen sulfide
solubility in natural gas purification |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8613862/ https://www.ncbi.nlm.nih.gov/pubmed/34841175 http://dx.doi.org/10.1021/acsomega.1c05169 |
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