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Purcell Effect and Beaming of Emission in Hybrid AlGaAs Nanowires with GaAs Quantum Dots

Control of directionality of emissions is an important task for the realization of novel nanophotonic devices based on nanowires. Most of the existing approaches providing high directionality of the light emitted from nanowires are based on the utilization of the tapered shape of nanowires, serving...

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Autores principales: Reznik, Rodion R., Cirlin, George E., Kotlyar, Konstantin P., Ilkiv, Igor V., Akopian, Nika, Leandro, Lorenzo, Nikolaev, Valentin V., Belonovski, Alexey V., Kaliteevski, Mikhail A.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8617613/
https://www.ncbi.nlm.nih.gov/pubmed/34835659
http://dx.doi.org/10.3390/nano11112894
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author Reznik, Rodion R.
Cirlin, George E.
Kotlyar, Konstantin P.
Ilkiv, Igor V.
Akopian, Nika
Leandro, Lorenzo
Nikolaev, Valentin V.
Belonovski, Alexey V.
Kaliteevski, Mikhail A.
author_facet Reznik, Rodion R.
Cirlin, George E.
Kotlyar, Konstantin P.
Ilkiv, Igor V.
Akopian, Nika
Leandro, Lorenzo
Nikolaev, Valentin V.
Belonovski, Alexey V.
Kaliteevski, Mikhail A.
author_sort Reznik, Rodion R.
collection PubMed
description Control of directionality of emissions is an important task for the realization of novel nanophotonic devices based on nanowires. Most of the existing approaches providing high directionality of the light emitted from nanowires are based on the utilization of the tapered shape of nanowires, serving as nanoantenna coupling with the light waveguided in nanowire and the directional output beam. Here we report the beaming of the emitted light with wavelength near 800 nm by naturally formed core-shell AlGaAs NW with multiply GaAs quantum dots (QDs) diameter 30 nm and height 10 nm, while the diameter of NW 130 nm, what does not support efficient emission into waveguided modes, including the mode HE(11). Experimental measurements show that intensity of emission for directions in the vicinity of the axis of NW is about two orders of magnitude higher than for perpendicular directions. The developed theoretical approach allowed us to calculate the probability of spontaneous emission for various directions and into waveguided modes and showed that highly directional radiation can be provided by the intrinsic emission properties of cylindrical NW. Our results suggest that for the small diameter of NW, directional emissions are associated with an TM(0) leaky mode (when electric field oriented in axial direction) and therefore manifests in an existence of axial electric dipole transitions in quantum dots.
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spelling pubmed-86176132021-11-27 Purcell Effect and Beaming of Emission in Hybrid AlGaAs Nanowires with GaAs Quantum Dots Reznik, Rodion R. Cirlin, George E. Kotlyar, Konstantin P. Ilkiv, Igor V. Akopian, Nika Leandro, Lorenzo Nikolaev, Valentin V. Belonovski, Alexey V. Kaliteevski, Mikhail A. Nanomaterials (Basel) Article Control of directionality of emissions is an important task for the realization of novel nanophotonic devices based on nanowires. Most of the existing approaches providing high directionality of the light emitted from nanowires are based on the utilization of the tapered shape of nanowires, serving as nanoantenna coupling with the light waveguided in nanowire and the directional output beam. Here we report the beaming of the emitted light with wavelength near 800 nm by naturally formed core-shell AlGaAs NW with multiply GaAs quantum dots (QDs) diameter 30 nm and height 10 nm, while the diameter of NW 130 nm, what does not support efficient emission into waveguided modes, including the mode HE(11). Experimental measurements show that intensity of emission for directions in the vicinity of the axis of NW is about two orders of magnitude higher than for perpendicular directions. The developed theoretical approach allowed us to calculate the probability of spontaneous emission for various directions and into waveguided modes and showed that highly directional radiation can be provided by the intrinsic emission properties of cylindrical NW. Our results suggest that for the small diameter of NW, directional emissions are associated with an TM(0) leaky mode (when electric field oriented in axial direction) and therefore manifests in an existence of axial electric dipole transitions in quantum dots. MDPI 2021-10-29 /pmc/articles/PMC8617613/ /pubmed/34835659 http://dx.doi.org/10.3390/nano11112894 Text en © 2021 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Reznik, Rodion R.
Cirlin, George E.
Kotlyar, Konstantin P.
Ilkiv, Igor V.
Akopian, Nika
Leandro, Lorenzo
Nikolaev, Valentin V.
Belonovski, Alexey V.
Kaliteevski, Mikhail A.
Purcell Effect and Beaming of Emission in Hybrid AlGaAs Nanowires with GaAs Quantum Dots
title Purcell Effect and Beaming of Emission in Hybrid AlGaAs Nanowires with GaAs Quantum Dots
title_full Purcell Effect and Beaming of Emission in Hybrid AlGaAs Nanowires with GaAs Quantum Dots
title_fullStr Purcell Effect and Beaming of Emission in Hybrid AlGaAs Nanowires with GaAs Quantum Dots
title_full_unstemmed Purcell Effect and Beaming of Emission in Hybrid AlGaAs Nanowires with GaAs Quantum Dots
title_short Purcell Effect and Beaming of Emission in Hybrid AlGaAs Nanowires with GaAs Quantum Dots
title_sort purcell effect and beaming of emission in hybrid algaas nanowires with gaas quantum dots
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8617613/
https://www.ncbi.nlm.nih.gov/pubmed/34835659
http://dx.doi.org/10.3390/nano11112894
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