Cargando…

Preparation of Ag(3)PO(4)/TiO(2)(B) Heterojunction Nanobelt with Extended Light Response and Enhanced Photocatalytic Performance

Photocatalytic degradation, as an emerging method to control environmental pollution, is considered one of the most promising environmental purification technologies. As Tibet is a region with some of the strongest solar radiation in China and even in the world, it is extremely rich in solar energy...

Descripción completa

Detalles Bibliográficos
Autores principales: Li, Yong, Liu, Yanfang, Zhang, Mingqing, Zhou, Qianyu, Li, Xin, Chen, Tianlu, Wang, Shifeng
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8620934/
https://www.ncbi.nlm.nih.gov/pubmed/34834078
http://dx.doi.org/10.3390/molecules26226987
_version_ 1784605336638849024
author Li, Yong
Liu, Yanfang
Zhang, Mingqing
Zhou, Qianyu
Li, Xin
Chen, Tianlu
Wang, Shifeng
author_facet Li, Yong
Liu, Yanfang
Zhang, Mingqing
Zhou, Qianyu
Li, Xin
Chen, Tianlu
Wang, Shifeng
author_sort Li, Yong
collection PubMed
description Photocatalytic degradation, as an emerging method to control environmental pollution, is considered one of the most promising environmental purification technologies. As Tibet is a region with some of the strongest solar radiation in China and even in the world, it is extremely rich in solar energy resources, which is ideal for applying photocatalytic technology to its ecological environment protection and governance. In this study, Na(2)Ti(3)O(7) nanobelts were prepared via a hydrothermal method and converted to TiO(2)∙xH(2)O ion exchange, which was followed by high-temperature calcination to prepare TiO(2)(B) nanobelts (“B” in TiO(2)(B) means “Bronze phase”). A simple in situ method was used to generate Ag(3)PO(4) particles on the surface of the TiO(2) nanobelts to construct a Ag(3)PO(4)/TiO(2)(B) heterojunction composite photocatalyst. By generating Ag(3)PO(4) nanoparticles on the surface of the TiO(2)(B) nanobelts to construct heterojunctions, the light absorption range of the photocatalyst was successfully extended from UV (ultraviolet) to the visible region. Furthermore, the recombination of photogenerated electron–hole pairs in the catalyst was inhibited by the construction of the heterojunctions, thus greatly enhancing its light quantum efficiency. Therefore, the prepared Ag(3)PO(4)/TiO(2)(B) heterojunction composite photocatalyst greatly outperformed the TiO(2)(B) nanobelt in terms of photocatalytic degradation.
format Online
Article
Text
id pubmed-8620934
institution National Center for Biotechnology Information
language English
publishDate 2021
publisher MDPI
record_format MEDLINE/PubMed
spelling pubmed-86209342021-11-27 Preparation of Ag(3)PO(4)/TiO(2)(B) Heterojunction Nanobelt with Extended Light Response and Enhanced Photocatalytic Performance Li, Yong Liu, Yanfang Zhang, Mingqing Zhou, Qianyu Li, Xin Chen, Tianlu Wang, Shifeng Molecules Article Photocatalytic degradation, as an emerging method to control environmental pollution, is considered one of the most promising environmental purification technologies. As Tibet is a region with some of the strongest solar radiation in China and even in the world, it is extremely rich in solar energy resources, which is ideal for applying photocatalytic technology to its ecological environment protection and governance. In this study, Na(2)Ti(3)O(7) nanobelts were prepared via a hydrothermal method and converted to TiO(2)∙xH(2)O ion exchange, which was followed by high-temperature calcination to prepare TiO(2)(B) nanobelts (“B” in TiO(2)(B) means “Bronze phase”). A simple in situ method was used to generate Ag(3)PO(4) particles on the surface of the TiO(2) nanobelts to construct a Ag(3)PO(4)/TiO(2)(B) heterojunction composite photocatalyst. By generating Ag(3)PO(4) nanoparticles on the surface of the TiO(2)(B) nanobelts to construct heterojunctions, the light absorption range of the photocatalyst was successfully extended from UV (ultraviolet) to the visible region. Furthermore, the recombination of photogenerated electron–hole pairs in the catalyst was inhibited by the construction of the heterojunctions, thus greatly enhancing its light quantum efficiency. Therefore, the prepared Ag(3)PO(4)/TiO(2)(B) heterojunction composite photocatalyst greatly outperformed the TiO(2)(B) nanobelt in terms of photocatalytic degradation. MDPI 2021-11-19 /pmc/articles/PMC8620934/ /pubmed/34834078 http://dx.doi.org/10.3390/molecules26226987 Text en © 2021 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Li, Yong
Liu, Yanfang
Zhang, Mingqing
Zhou, Qianyu
Li, Xin
Chen, Tianlu
Wang, Shifeng
Preparation of Ag(3)PO(4)/TiO(2)(B) Heterojunction Nanobelt with Extended Light Response and Enhanced Photocatalytic Performance
title Preparation of Ag(3)PO(4)/TiO(2)(B) Heterojunction Nanobelt with Extended Light Response and Enhanced Photocatalytic Performance
title_full Preparation of Ag(3)PO(4)/TiO(2)(B) Heterojunction Nanobelt with Extended Light Response and Enhanced Photocatalytic Performance
title_fullStr Preparation of Ag(3)PO(4)/TiO(2)(B) Heterojunction Nanobelt with Extended Light Response and Enhanced Photocatalytic Performance
title_full_unstemmed Preparation of Ag(3)PO(4)/TiO(2)(B) Heterojunction Nanobelt with Extended Light Response and Enhanced Photocatalytic Performance
title_short Preparation of Ag(3)PO(4)/TiO(2)(B) Heterojunction Nanobelt with Extended Light Response and Enhanced Photocatalytic Performance
title_sort preparation of ag(3)po(4)/tio(2)(b) heterojunction nanobelt with extended light response and enhanced photocatalytic performance
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8620934/
https://www.ncbi.nlm.nih.gov/pubmed/34834078
http://dx.doi.org/10.3390/molecules26226987
work_keys_str_mv AT liyong preparationofag3po4tio2bheterojunctionnanobeltwithextendedlightresponseandenhancedphotocatalyticperformance
AT liuyanfang preparationofag3po4tio2bheterojunctionnanobeltwithextendedlightresponseandenhancedphotocatalyticperformance
AT zhangmingqing preparationofag3po4tio2bheterojunctionnanobeltwithextendedlightresponseandenhancedphotocatalyticperformance
AT zhouqianyu preparationofag3po4tio2bheterojunctionnanobeltwithextendedlightresponseandenhancedphotocatalyticperformance
AT lixin preparationofag3po4tio2bheterojunctionnanobeltwithextendedlightresponseandenhancedphotocatalyticperformance
AT chentianlu preparationofag3po4tio2bheterojunctionnanobeltwithextendedlightresponseandenhancedphotocatalyticperformance
AT wangshifeng preparationofag3po4tio2bheterojunctionnanobeltwithextendedlightresponseandenhancedphotocatalyticperformance