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Study on Localized Surface Plasmon Coupling with Many Radiators

Localized surface plasmon (LSP) coupling with many radiators are investigated. The LSP is generated by excitation of laser or electron beam on the random Ag nano particles (NPs) and arrayed ones embedded in the p-GaN of green LEDs. They couple with the excitons or radiative recombination in the quan...

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Autores principales: Chen, Zhizhong, Deng, Chuhan, Xi, Xin, Chen, Yifan, Feng, Yulong, Jiang, Shuang, Chen, Weihua, Kang, Xiangning, Wang, Qi, Zhang, Guoyi, Shen, Bo
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8620948/
https://www.ncbi.nlm.nih.gov/pubmed/34835869
http://dx.doi.org/10.3390/nano11113105
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author Chen, Zhizhong
Deng, Chuhan
Xi, Xin
Chen, Yifan
Feng, Yulong
Jiang, Shuang
Chen, Weihua
Kang, Xiangning
Wang, Qi
Zhang, Guoyi
Shen, Bo
author_facet Chen, Zhizhong
Deng, Chuhan
Xi, Xin
Chen, Yifan
Feng, Yulong
Jiang, Shuang
Chen, Weihua
Kang, Xiangning
Wang, Qi
Zhang, Guoyi
Shen, Bo
author_sort Chen, Zhizhong
collection PubMed
description Localized surface plasmon (LSP) coupling with many radiators are investigated. The LSP is generated by excitation of laser or electron beam on the random Ag nano particles (NPs) and arrayed ones embedded in the p-GaN of green LEDs. They couple with the excitons or radiative recombination in the quantum well (QW) and electron beam, which enhance or suppress the luminescence of the radiators. The photoluminescence (PL) intensity of periodic Ag NPs can get as much as 4.5 times higher than that of bare LED. In addition to the periodic structure, the morphology of Ag NPs also affects the localized SP (LSP) resonance intensity and light scattering efficiency. In the finite difference time domain (FDTD) simulation, five x-polarized dipoles are approximated to five quantum wells. Considering the interaction between the five dipoles and their feedback effect on LSP, the enhancement effect of SP dipole coupling with Ag NPs is amplified and the energy dissipation is reduced. The enhancement of cathodoluminescence (CL) was also found in green LEDs with Ag NPs. The three-body model composed of two orthogonal dipoles and an Ag NP is used for 3D FDTD simulation. The LSP-QWs coupling effect is separated from the electron beam (e-beam)-LSP-QW system by linear approximation. Under the excitation of electron beam, the introduction of z-dipole greatly reduces the energy dissipation. In the cross-sectional sample, z-polarized dipoles in QWs show more coupling strength to the dipole and quadrupole modes of LSP. The perturbation theory is used to separate the LSP coupling effects to x-dipole and z-dipole. At last, the resonator and the antenna effects are discussed for LSP coupling at different positions to the Ag NP.
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spelling pubmed-86209482021-11-27 Study on Localized Surface Plasmon Coupling with Many Radiators Chen, Zhizhong Deng, Chuhan Xi, Xin Chen, Yifan Feng, Yulong Jiang, Shuang Chen, Weihua Kang, Xiangning Wang, Qi Zhang, Guoyi Shen, Bo Nanomaterials (Basel) Review Localized surface plasmon (LSP) coupling with many radiators are investigated. The LSP is generated by excitation of laser or electron beam on the random Ag nano particles (NPs) and arrayed ones embedded in the p-GaN of green LEDs. They couple with the excitons or radiative recombination in the quantum well (QW) and electron beam, which enhance or suppress the luminescence of the radiators. The photoluminescence (PL) intensity of periodic Ag NPs can get as much as 4.5 times higher than that of bare LED. In addition to the periodic structure, the morphology of Ag NPs also affects the localized SP (LSP) resonance intensity and light scattering efficiency. In the finite difference time domain (FDTD) simulation, five x-polarized dipoles are approximated to five quantum wells. Considering the interaction between the five dipoles and their feedback effect on LSP, the enhancement effect of SP dipole coupling with Ag NPs is amplified and the energy dissipation is reduced. The enhancement of cathodoluminescence (CL) was also found in green LEDs with Ag NPs. The three-body model composed of two orthogonal dipoles and an Ag NP is used for 3D FDTD simulation. The LSP-QWs coupling effect is separated from the electron beam (e-beam)-LSP-QW system by linear approximation. Under the excitation of electron beam, the introduction of z-dipole greatly reduces the energy dissipation. In the cross-sectional sample, z-polarized dipoles in QWs show more coupling strength to the dipole and quadrupole modes of LSP. The perturbation theory is used to separate the LSP coupling effects to x-dipole and z-dipole. At last, the resonator and the antenna effects are discussed for LSP coupling at different positions to the Ag NP. MDPI 2021-11-18 /pmc/articles/PMC8620948/ /pubmed/34835869 http://dx.doi.org/10.3390/nano11113105 Text en © 2021 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Review
Chen, Zhizhong
Deng, Chuhan
Xi, Xin
Chen, Yifan
Feng, Yulong
Jiang, Shuang
Chen, Weihua
Kang, Xiangning
Wang, Qi
Zhang, Guoyi
Shen, Bo
Study on Localized Surface Plasmon Coupling with Many Radiators
title Study on Localized Surface Plasmon Coupling with Many Radiators
title_full Study on Localized Surface Plasmon Coupling with Many Radiators
title_fullStr Study on Localized Surface Plasmon Coupling with Many Radiators
title_full_unstemmed Study on Localized Surface Plasmon Coupling with Many Radiators
title_short Study on Localized Surface Plasmon Coupling with Many Radiators
title_sort study on localized surface plasmon coupling with many radiators
topic Review
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8620948/
https://www.ncbi.nlm.nih.gov/pubmed/34835869
http://dx.doi.org/10.3390/nano11113105
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