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Electrocatalytic Degradation of Levofloxacin, a Typical Antibiotic in Hospital Wastewater

Presently, in the context of the novel coronavirus pneumonia epidemic, several antibiotics are overused in hospitals, causing heavy pressure on the hospital’s wastewater treatment process. Therefore, developing stable, safe, and efficient hospital wastewater treatment equipment is crucial. Herein, a...

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Autores principales: Lv, Hongxia, Han, Peiwei, Li, Xiaogang, Mu, Zhao, Zuo, Yuan, Wang, Xu, Tan, Yannan, He, Guangxiang, Jin, Haibo, Sun, Chenglin, Wei, Huangzhao, Ma, Lei
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8621070/
https://www.ncbi.nlm.nih.gov/pubmed/34832216
http://dx.doi.org/10.3390/ma14226814
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author Lv, Hongxia
Han, Peiwei
Li, Xiaogang
Mu, Zhao
Zuo, Yuan
Wang, Xu
Tan, Yannan
He, Guangxiang
Jin, Haibo
Sun, Chenglin
Wei, Huangzhao
Ma, Lei
author_facet Lv, Hongxia
Han, Peiwei
Li, Xiaogang
Mu, Zhao
Zuo, Yuan
Wang, Xu
Tan, Yannan
He, Guangxiang
Jin, Haibo
Sun, Chenglin
Wei, Huangzhao
Ma, Lei
author_sort Lv, Hongxia
collection PubMed
description Presently, in the context of the novel coronavirus pneumonia epidemic, several antibiotics are overused in hospitals, causing heavy pressure on the hospital’s wastewater treatment process. Therefore, developing stable, safe, and efficient hospital wastewater treatment equipment is crucial. Herein, a bench-scale electrooxidation equipment for hospital wastewater was used to evaluate the removal effect of the main antibiotic levofloxacin (LVX) in hospital wastewater using response surface methodology (RSM). During the degradation process, the influence of the following five factors on total organic carbon (TOC) removal was discussed and the best reaction condition was obtained: current density, initial pH, flow rate, chloride ion concentration, and reaction time of 39.6 A/m(2), 6.5, 50 mL/min, 4‰, and 120 min, respectively. The TOC removal could reach 41% after a reaction time of 120 min, which was consistent with the result predicted by the response surface (40.48%). Moreover, the morphology and properties of the electrode were analyzed. The degradation pathway of LVX was analyzed using high-performance liquid chromatography–mass spectrometry (LC–MS). Subsequently, the bench-scale electrooxidation equipment was changed into onboard-scale electrooxidation equipment, and the onboard-scale equipment was promoted to several hospitals in Dalian.
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spelling pubmed-86210702021-11-27 Electrocatalytic Degradation of Levofloxacin, a Typical Antibiotic in Hospital Wastewater Lv, Hongxia Han, Peiwei Li, Xiaogang Mu, Zhao Zuo, Yuan Wang, Xu Tan, Yannan He, Guangxiang Jin, Haibo Sun, Chenglin Wei, Huangzhao Ma, Lei Materials (Basel) Article Presently, in the context of the novel coronavirus pneumonia epidemic, several antibiotics are overused in hospitals, causing heavy pressure on the hospital’s wastewater treatment process. Therefore, developing stable, safe, and efficient hospital wastewater treatment equipment is crucial. Herein, a bench-scale electrooxidation equipment for hospital wastewater was used to evaluate the removal effect of the main antibiotic levofloxacin (LVX) in hospital wastewater using response surface methodology (RSM). During the degradation process, the influence of the following five factors on total organic carbon (TOC) removal was discussed and the best reaction condition was obtained: current density, initial pH, flow rate, chloride ion concentration, and reaction time of 39.6 A/m(2), 6.5, 50 mL/min, 4‰, and 120 min, respectively. The TOC removal could reach 41% after a reaction time of 120 min, which was consistent with the result predicted by the response surface (40.48%). Moreover, the morphology and properties of the electrode were analyzed. The degradation pathway of LVX was analyzed using high-performance liquid chromatography–mass spectrometry (LC–MS). Subsequently, the bench-scale electrooxidation equipment was changed into onboard-scale electrooxidation equipment, and the onboard-scale equipment was promoted to several hospitals in Dalian. MDPI 2021-11-11 /pmc/articles/PMC8621070/ /pubmed/34832216 http://dx.doi.org/10.3390/ma14226814 Text en © 2021 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Lv, Hongxia
Han, Peiwei
Li, Xiaogang
Mu, Zhao
Zuo, Yuan
Wang, Xu
Tan, Yannan
He, Guangxiang
Jin, Haibo
Sun, Chenglin
Wei, Huangzhao
Ma, Lei
Electrocatalytic Degradation of Levofloxacin, a Typical Antibiotic in Hospital Wastewater
title Electrocatalytic Degradation of Levofloxacin, a Typical Antibiotic in Hospital Wastewater
title_full Electrocatalytic Degradation of Levofloxacin, a Typical Antibiotic in Hospital Wastewater
title_fullStr Electrocatalytic Degradation of Levofloxacin, a Typical Antibiotic in Hospital Wastewater
title_full_unstemmed Electrocatalytic Degradation of Levofloxacin, a Typical Antibiotic in Hospital Wastewater
title_short Electrocatalytic Degradation of Levofloxacin, a Typical Antibiotic in Hospital Wastewater
title_sort electrocatalytic degradation of levofloxacin, a typical antibiotic in hospital wastewater
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8621070/
https://www.ncbi.nlm.nih.gov/pubmed/34832216
http://dx.doi.org/10.3390/ma14226814
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