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Resonant tunneling driven metal-insulator transition in double quantum-well structures of strongly correlated oxide

The metal-insulator transition (MIT), a fascinating phenomenon occurring in some strongly correlated materials, is of central interest in modern condensed-matter physics. Controlling the MIT by external stimuli is a key technological goal for applications in future electronic devices. However, the s...

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Autores principales: Yukawa, R., Kobayashi, M., Kanda, T., Shiga, D., Yoshimatsu, K., Ishibashi, S., Minohara, M., Kitamura, M., Horiba, K., Santander-Syro, A. F., Kumigashira, H.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8642393/
https://www.ncbi.nlm.nih.gov/pubmed/34862386
http://dx.doi.org/10.1038/s41467-021-27327-z
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author Yukawa, R.
Kobayashi, M.
Kanda, T.
Shiga, D.
Yoshimatsu, K.
Ishibashi, S.
Minohara, M.
Kitamura, M.
Horiba, K.
Santander-Syro, A. F.
Kumigashira, H.
author_facet Yukawa, R.
Kobayashi, M.
Kanda, T.
Shiga, D.
Yoshimatsu, K.
Ishibashi, S.
Minohara, M.
Kitamura, M.
Horiba, K.
Santander-Syro, A. F.
Kumigashira, H.
author_sort Yukawa, R.
collection PubMed
description The metal-insulator transition (MIT), a fascinating phenomenon occurring in some strongly correlated materials, is of central interest in modern condensed-matter physics. Controlling the MIT by external stimuli is a key technological goal for applications in future electronic devices. However, the standard control by means of the field effect, which works extremely well for semiconductor transistors, faces severe difficulties when applied to the MIT. Hence, a radically different approach is needed. Here, we report an MIT induced by resonant tunneling (RT) in double quantum well (QW) structures of strongly correlated oxides. In our structures, two layers of the strongly correlated conductive oxide SrVO(3) (SVO) sandwich a barrier layer of the band insulator SrTiO(3). The top QW is a marginal Mott-insulating SVO layer, while the bottom QW is a metallic SVO layer. Angle-resolved photoemission spectroscopy experiments reveal that the top QW layer becomes metallized when the thickness of the tunneling barrier layer is reduced. An analysis based on band structure calculations indicates that RT between the quantized states of the double QW induces the MIT. Our work opens avenues for realizing the Mott-transistor based on the wave-function engineering of strongly correlated electrons.
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spelling pubmed-86423932021-12-15 Resonant tunneling driven metal-insulator transition in double quantum-well structures of strongly correlated oxide Yukawa, R. Kobayashi, M. Kanda, T. Shiga, D. Yoshimatsu, K. Ishibashi, S. Minohara, M. Kitamura, M. Horiba, K. Santander-Syro, A. F. Kumigashira, H. Nat Commun Article The metal-insulator transition (MIT), a fascinating phenomenon occurring in some strongly correlated materials, is of central interest in modern condensed-matter physics. Controlling the MIT by external stimuli is a key technological goal for applications in future electronic devices. However, the standard control by means of the field effect, which works extremely well for semiconductor transistors, faces severe difficulties when applied to the MIT. Hence, a radically different approach is needed. Here, we report an MIT induced by resonant tunneling (RT) in double quantum well (QW) structures of strongly correlated oxides. In our structures, two layers of the strongly correlated conductive oxide SrVO(3) (SVO) sandwich a barrier layer of the band insulator SrTiO(3). The top QW is a marginal Mott-insulating SVO layer, while the bottom QW is a metallic SVO layer. Angle-resolved photoemission spectroscopy experiments reveal that the top QW layer becomes metallized when the thickness of the tunneling barrier layer is reduced. An analysis based on band structure calculations indicates that RT between the quantized states of the double QW induces the MIT. Our work opens avenues for realizing the Mott-transistor based on the wave-function engineering of strongly correlated electrons. Nature Publishing Group UK 2021-12-03 /pmc/articles/PMC8642393/ /pubmed/34862386 http://dx.doi.org/10.1038/s41467-021-27327-z Text en © The Author(s) 2021 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Yukawa, R.
Kobayashi, M.
Kanda, T.
Shiga, D.
Yoshimatsu, K.
Ishibashi, S.
Minohara, M.
Kitamura, M.
Horiba, K.
Santander-Syro, A. F.
Kumigashira, H.
Resonant tunneling driven metal-insulator transition in double quantum-well structures of strongly correlated oxide
title Resonant tunneling driven metal-insulator transition in double quantum-well structures of strongly correlated oxide
title_full Resonant tunneling driven metal-insulator transition in double quantum-well structures of strongly correlated oxide
title_fullStr Resonant tunneling driven metal-insulator transition in double quantum-well structures of strongly correlated oxide
title_full_unstemmed Resonant tunneling driven metal-insulator transition in double quantum-well structures of strongly correlated oxide
title_short Resonant tunneling driven metal-insulator transition in double quantum-well structures of strongly correlated oxide
title_sort resonant tunneling driven metal-insulator transition in double quantum-well structures of strongly correlated oxide
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8642393/
https://www.ncbi.nlm.nih.gov/pubmed/34862386
http://dx.doi.org/10.1038/s41467-021-27327-z
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