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Low-symmetry nonlocal transport in microstructured squares of delafossite metals

Intense work studying the ballistic regime of electron transport in two-dimensional systems based on semiconductors and graphene had been thought to have established most of the key experimental facts of the field. In recent years, however, additional forms of ballistic transport have become accessi...

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Autores principales: McGuinness, Philippa H., Zhakina, Elina, König, Markus, Bachmann, Maja D., Putzke, Carsten, Moll, Philip J. W., Khim, Seunghyun, Mackenzie, Andrew P.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: National Academy of Sciences 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8672864/
https://www.ncbi.nlm.nih.gov/pubmed/34782472
http://dx.doi.org/10.1073/pnas.2113185118
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author McGuinness, Philippa H.
Zhakina, Elina
König, Markus
Bachmann, Maja D.
Putzke, Carsten
Moll, Philip J. W.
Khim, Seunghyun
Mackenzie, Andrew P.
author_facet McGuinness, Philippa H.
Zhakina, Elina
König, Markus
Bachmann, Maja D.
Putzke, Carsten
Moll, Philip J. W.
Khim, Seunghyun
Mackenzie, Andrew P.
author_sort McGuinness, Philippa H.
collection PubMed
description Intense work studying the ballistic regime of electron transport in two-dimensional systems based on semiconductors and graphene had been thought to have established most of the key experimental facts of the field. In recent years, however, additional forms of ballistic transport have become accessible in the quasi–two-dimensional delafossite metals, whose Fermi wavelength is a factor of 100 shorter than those typically studied in the previous work and whose Fermi surfaces are nearly hexagonal in shape and therefore strongly faceted. This has some profound consequences for results obtained from the classic ballistic transport experiment of studying bend and Hall resistances in mesoscopic squares fabricated from delafossite single crystals. We observe pronounced anisotropies in bend resistances and even a Hall voltage that is strongly asymmetric in magnetic field. Although some of our observations are nonintuitive at first sight, we show that they can be understood within a nonlocal Landauer-Büttiker analysis tailored to the symmetries of the square/hexagonal geometries of our combined device/Fermi surface system. Signatures of nonlocal transport can be resolved for squares of linear dimension of nearly 100 µm, approximately a factor of 15 larger than the bulk mean free path of the crystal from which the device was fabricated.
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spelling pubmed-86728642021-12-30 Low-symmetry nonlocal transport in microstructured squares of delafossite metals McGuinness, Philippa H. Zhakina, Elina König, Markus Bachmann, Maja D. Putzke, Carsten Moll, Philip J. W. Khim, Seunghyun Mackenzie, Andrew P. Proc Natl Acad Sci U S A Physical Sciences Intense work studying the ballistic regime of electron transport in two-dimensional systems based on semiconductors and graphene had been thought to have established most of the key experimental facts of the field. In recent years, however, additional forms of ballistic transport have become accessible in the quasi–two-dimensional delafossite metals, whose Fermi wavelength is a factor of 100 shorter than those typically studied in the previous work and whose Fermi surfaces are nearly hexagonal in shape and therefore strongly faceted. This has some profound consequences for results obtained from the classic ballistic transport experiment of studying bend and Hall resistances in mesoscopic squares fabricated from delafossite single crystals. We observe pronounced anisotropies in bend resistances and even a Hall voltage that is strongly asymmetric in magnetic field. Although some of our observations are nonintuitive at first sight, we show that they can be understood within a nonlocal Landauer-Büttiker analysis tailored to the symmetries of the square/hexagonal geometries of our combined device/Fermi surface system. Signatures of nonlocal transport can be resolved for squares of linear dimension of nearly 100 µm, approximately a factor of 15 larger than the bulk mean free path of the crystal from which the device was fabricated. National Academy of Sciences 2021-11-15 2021-11-23 /pmc/articles/PMC8672864/ /pubmed/34782472 http://dx.doi.org/10.1073/pnas.2113185118 Text en Copyright © 2021 the Author(s). Published by PNAS. https://creativecommons.org/licenses/by-nc-nd/4.0/This open access article is distributed under Creative Commons Attribution-NonCommercial-NoDerivatives License 4.0 (CC BY-NC-ND) (https://creativecommons.org/licenses/by-nc-nd/4.0/) .
spellingShingle Physical Sciences
McGuinness, Philippa H.
Zhakina, Elina
König, Markus
Bachmann, Maja D.
Putzke, Carsten
Moll, Philip J. W.
Khim, Seunghyun
Mackenzie, Andrew P.
Low-symmetry nonlocal transport in microstructured squares of delafossite metals
title Low-symmetry nonlocal transport in microstructured squares of delafossite metals
title_full Low-symmetry nonlocal transport in microstructured squares of delafossite metals
title_fullStr Low-symmetry nonlocal transport in microstructured squares of delafossite metals
title_full_unstemmed Low-symmetry nonlocal transport in microstructured squares of delafossite metals
title_short Low-symmetry nonlocal transport in microstructured squares of delafossite metals
title_sort low-symmetry nonlocal transport in microstructured squares of delafossite metals
topic Physical Sciences
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8672864/
https://www.ncbi.nlm.nih.gov/pubmed/34782472
http://dx.doi.org/10.1073/pnas.2113185118
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