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Tuning Coherent-Phonon Heat Transport in LaCoO(3)/SrTiO(3) Superlattices

[Image: see text] Accessing the regime of coherent phonon propagation in nanostructures opens enormous possibilities to control the thermal conductivity in energy harvesting devices, phononic circuits, etc. In this paper we show that coherent phonons contribute substantially to the thermal conductiv...

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Detalles Bibliográficos
Autores principales: Bugallo, D., Langenberg, E., Carbó-Argibay, E., Varela Dominguez, Noa, Fumega, A. O., Pardo, V., Lucas, Irene, Morellón, Luis, Rivadulla, F.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2021
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8686111/
https://www.ncbi.nlm.nih.gov/pubmed/34875171
http://dx.doi.org/10.1021/acs.jpclett.1c03418
Descripción
Sumario:[Image: see text] Accessing the regime of coherent phonon propagation in nanostructures opens enormous possibilities to control the thermal conductivity in energy harvesting devices, phononic circuits, etc. In this paper we show that coherent phonons contribute substantially to the thermal conductivity of LaCoO(3)/SrTiO(3) oxide superlattices, up to room temperature. We show that their contribution can be tuned through small variations of the superlattice periodicity, without changing the total superlattice thickness. Using this strategy, we tuned the thermal conductivity by 20% at room temperature. We also discuss the role of interface mixing and epitaxial relaxation as an extrinsic, material dependent key parameter for understanding the thermal conductivity of oxide superlattices.