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Tuning Coherent-Phonon Heat Transport in LaCoO(3)/SrTiO(3) Superlattices

[Image: see text] Accessing the regime of coherent phonon propagation in nanostructures opens enormous possibilities to control the thermal conductivity in energy harvesting devices, phononic circuits, etc. In this paper we show that coherent phonons contribute substantially to the thermal conductiv...

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Autores principales: Bugallo, D., Langenberg, E., Carbó-Argibay, E., Varela Dominguez, Noa, Fumega, A. O., Pardo, V., Lucas, Irene, Morellón, Luis, Rivadulla, F.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2021
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8686111/
https://www.ncbi.nlm.nih.gov/pubmed/34875171
http://dx.doi.org/10.1021/acs.jpclett.1c03418
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author Bugallo, D.
Langenberg, E.
Carbó-Argibay, E.
Varela Dominguez, Noa
Fumega, A. O.
Pardo, V.
Lucas, Irene
Morellón, Luis
Rivadulla, F.
author_facet Bugallo, D.
Langenberg, E.
Carbó-Argibay, E.
Varela Dominguez, Noa
Fumega, A. O.
Pardo, V.
Lucas, Irene
Morellón, Luis
Rivadulla, F.
author_sort Bugallo, D.
collection PubMed
description [Image: see text] Accessing the regime of coherent phonon propagation in nanostructures opens enormous possibilities to control the thermal conductivity in energy harvesting devices, phononic circuits, etc. In this paper we show that coherent phonons contribute substantially to the thermal conductivity of LaCoO(3)/SrTiO(3) oxide superlattices, up to room temperature. We show that their contribution can be tuned through small variations of the superlattice periodicity, without changing the total superlattice thickness. Using this strategy, we tuned the thermal conductivity by 20% at room temperature. We also discuss the role of interface mixing and epitaxial relaxation as an extrinsic, material dependent key parameter for understanding the thermal conductivity of oxide superlattices.
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spelling pubmed-86861112021-12-21 Tuning Coherent-Phonon Heat Transport in LaCoO(3)/SrTiO(3) Superlattices Bugallo, D. Langenberg, E. Carbó-Argibay, E. Varela Dominguez, Noa Fumega, A. O. Pardo, V. Lucas, Irene Morellón, Luis Rivadulla, F. J Phys Chem Lett [Image: see text] Accessing the regime of coherent phonon propagation in nanostructures opens enormous possibilities to control the thermal conductivity in energy harvesting devices, phononic circuits, etc. In this paper we show that coherent phonons contribute substantially to the thermal conductivity of LaCoO(3)/SrTiO(3) oxide superlattices, up to room temperature. We show that their contribution can be tuned through small variations of the superlattice periodicity, without changing the total superlattice thickness. Using this strategy, we tuned the thermal conductivity by 20% at room temperature. We also discuss the role of interface mixing and epitaxial relaxation as an extrinsic, material dependent key parameter for understanding the thermal conductivity of oxide superlattices. American Chemical Society 2021-12-07 2021-12-16 /pmc/articles/PMC8686111/ /pubmed/34875171 http://dx.doi.org/10.1021/acs.jpclett.1c03418 Text en © 2021 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by/4.0/Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Bugallo, D.
Langenberg, E.
Carbó-Argibay, E.
Varela Dominguez, Noa
Fumega, A. O.
Pardo, V.
Lucas, Irene
Morellón, Luis
Rivadulla, F.
Tuning Coherent-Phonon Heat Transport in LaCoO(3)/SrTiO(3) Superlattices
title Tuning Coherent-Phonon Heat Transport in LaCoO(3)/SrTiO(3) Superlattices
title_full Tuning Coherent-Phonon Heat Transport in LaCoO(3)/SrTiO(3) Superlattices
title_fullStr Tuning Coherent-Phonon Heat Transport in LaCoO(3)/SrTiO(3) Superlattices
title_full_unstemmed Tuning Coherent-Phonon Heat Transport in LaCoO(3)/SrTiO(3) Superlattices
title_short Tuning Coherent-Phonon Heat Transport in LaCoO(3)/SrTiO(3) Superlattices
title_sort tuning coherent-phonon heat transport in lacoo(3)/srtio(3) superlattices
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8686111/
https://www.ncbi.nlm.nih.gov/pubmed/34875171
http://dx.doi.org/10.1021/acs.jpclett.1c03418
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