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Tuning Coherent-Phonon Heat Transport in LaCoO(3)/SrTiO(3) Superlattices
[Image: see text] Accessing the regime of coherent phonon propagation in nanostructures opens enormous possibilities to control the thermal conductivity in energy harvesting devices, phononic circuits, etc. In this paper we show that coherent phonons contribute substantially to the thermal conductiv...
Autores principales: | , , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Chemical Society
2021
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Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8686111/ https://www.ncbi.nlm.nih.gov/pubmed/34875171 http://dx.doi.org/10.1021/acs.jpclett.1c03418 |
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author | Bugallo, D. Langenberg, E. Carbó-Argibay, E. Varela Dominguez, Noa Fumega, A. O. Pardo, V. Lucas, Irene Morellón, Luis Rivadulla, F. |
author_facet | Bugallo, D. Langenberg, E. Carbó-Argibay, E. Varela Dominguez, Noa Fumega, A. O. Pardo, V. Lucas, Irene Morellón, Luis Rivadulla, F. |
author_sort | Bugallo, D. |
collection | PubMed |
description | [Image: see text] Accessing the regime of coherent phonon propagation in nanostructures opens enormous possibilities to control the thermal conductivity in energy harvesting devices, phononic circuits, etc. In this paper we show that coherent phonons contribute substantially to the thermal conductivity of LaCoO(3)/SrTiO(3) oxide superlattices, up to room temperature. We show that their contribution can be tuned through small variations of the superlattice periodicity, without changing the total superlattice thickness. Using this strategy, we tuned the thermal conductivity by 20% at room temperature. We also discuss the role of interface mixing and epitaxial relaxation as an extrinsic, material dependent key parameter for understanding the thermal conductivity of oxide superlattices. |
format | Online Article Text |
id | pubmed-8686111 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2021 |
publisher | American Chemical Society |
record_format | MEDLINE/PubMed |
spelling | pubmed-86861112021-12-21 Tuning Coherent-Phonon Heat Transport in LaCoO(3)/SrTiO(3) Superlattices Bugallo, D. Langenberg, E. Carbó-Argibay, E. Varela Dominguez, Noa Fumega, A. O. Pardo, V. Lucas, Irene Morellón, Luis Rivadulla, F. J Phys Chem Lett [Image: see text] Accessing the regime of coherent phonon propagation in nanostructures opens enormous possibilities to control the thermal conductivity in energy harvesting devices, phononic circuits, etc. In this paper we show that coherent phonons contribute substantially to the thermal conductivity of LaCoO(3)/SrTiO(3) oxide superlattices, up to room temperature. We show that their contribution can be tuned through small variations of the superlattice periodicity, without changing the total superlattice thickness. Using this strategy, we tuned the thermal conductivity by 20% at room temperature. We also discuss the role of interface mixing and epitaxial relaxation as an extrinsic, material dependent key parameter for understanding the thermal conductivity of oxide superlattices. American Chemical Society 2021-12-07 2021-12-16 /pmc/articles/PMC8686111/ /pubmed/34875171 http://dx.doi.org/10.1021/acs.jpclett.1c03418 Text en © 2021 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by/4.0/Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/). |
spellingShingle | Bugallo, D. Langenberg, E. Carbó-Argibay, E. Varela Dominguez, Noa Fumega, A. O. Pardo, V. Lucas, Irene Morellón, Luis Rivadulla, F. Tuning Coherent-Phonon Heat Transport in LaCoO(3)/SrTiO(3) Superlattices |
title | Tuning Coherent-Phonon Heat Transport in LaCoO(3)/SrTiO(3) Superlattices |
title_full | Tuning Coherent-Phonon Heat Transport in LaCoO(3)/SrTiO(3) Superlattices |
title_fullStr | Tuning Coherent-Phonon Heat Transport in LaCoO(3)/SrTiO(3) Superlattices |
title_full_unstemmed | Tuning Coherent-Phonon Heat Transport in LaCoO(3)/SrTiO(3) Superlattices |
title_short | Tuning Coherent-Phonon Heat Transport in LaCoO(3)/SrTiO(3) Superlattices |
title_sort | tuning coherent-phonon heat transport in lacoo(3)/srtio(3) superlattices |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8686111/ https://www.ncbi.nlm.nih.gov/pubmed/34875171 http://dx.doi.org/10.1021/acs.jpclett.1c03418 |
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