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Enhancing the efficiency of the hydrogen evolution reaction utilising Fe(3)P bulk modified screen-printed electrodes via the application of a magnetic field

We report the fabrication and optimisation of Fe(3)P bulk modified screen-printed electrochemical platforms (SPEs) for the hydrogen evolution reaction (HER) within acidic media. We optimise the achievable current density towards the HER of the Fe(3)P SPEs by utilising ball-milled Fe(3)P variants and...

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Detalles Bibliográficos
Autores principales: Hughes, Jack. P., Rowley-Neale, Samuel, Banks, Craig
Formato: Online Artículo Texto
Lenguaje:English
Publicado: The Royal Society of Chemistry 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8695104/
https://www.ncbi.nlm.nih.gov/pubmed/35423332
http://dx.doi.org/10.1039/d0ra10150h
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author Hughes, Jack. P.
Rowley-Neale, Samuel
Banks, Craig
author_facet Hughes, Jack. P.
Rowley-Neale, Samuel
Banks, Craig
author_sort Hughes, Jack. P.
collection PubMed
description We report the fabrication and optimisation of Fe(3)P bulk modified screen-printed electrochemical platforms (SPEs) for the hydrogen evolution reaction (HER) within acidic media. We optimise the achievable current density towards the HER of the Fe(3)P SPEs by utilising ball-milled Fe(3)P variants and increasing the mass percentage of Fe(3)P incorporated into the SPEs. Additionally, the synergy of the application of a variable weak (constant) external magnetic field (330 mT to 40 mT) beneficially augments the current density output by 56%. This paper not only highlights the benefits of physical catalyst optimisation but also demonstrates a methodology to further enhance the cathodic efficiency of the HER with the facile application of a weak (constant) magnetic field.
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spelling pubmed-86951042022-04-13 Enhancing the efficiency of the hydrogen evolution reaction utilising Fe(3)P bulk modified screen-printed electrodes via the application of a magnetic field Hughes, Jack. P. Rowley-Neale, Samuel Banks, Craig RSC Adv Chemistry We report the fabrication and optimisation of Fe(3)P bulk modified screen-printed electrochemical platforms (SPEs) for the hydrogen evolution reaction (HER) within acidic media. We optimise the achievable current density towards the HER of the Fe(3)P SPEs by utilising ball-milled Fe(3)P variants and increasing the mass percentage of Fe(3)P incorporated into the SPEs. Additionally, the synergy of the application of a variable weak (constant) external magnetic field (330 mT to 40 mT) beneficially augments the current density output by 56%. This paper not only highlights the benefits of physical catalyst optimisation but also demonstrates a methodology to further enhance the cathodic efficiency of the HER with the facile application of a weak (constant) magnetic field. The Royal Society of Chemistry 2021-02-18 /pmc/articles/PMC8695104/ /pubmed/35423332 http://dx.doi.org/10.1039/d0ra10150h Text en This journal is © The Royal Society of Chemistry https://creativecommons.org/licenses/by-nc/3.0/
spellingShingle Chemistry
Hughes, Jack. P.
Rowley-Neale, Samuel
Banks, Craig
Enhancing the efficiency of the hydrogen evolution reaction utilising Fe(3)P bulk modified screen-printed electrodes via the application of a magnetic field
title Enhancing the efficiency of the hydrogen evolution reaction utilising Fe(3)P bulk modified screen-printed electrodes via the application of a magnetic field
title_full Enhancing the efficiency of the hydrogen evolution reaction utilising Fe(3)P bulk modified screen-printed electrodes via the application of a magnetic field
title_fullStr Enhancing the efficiency of the hydrogen evolution reaction utilising Fe(3)P bulk modified screen-printed electrodes via the application of a magnetic field
title_full_unstemmed Enhancing the efficiency of the hydrogen evolution reaction utilising Fe(3)P bulk modified screen-printed electrodes via the application of a magnetic field
title_short Enhancing the efficiency of the hydrogen evolution reaction utilising Fe(3)P bulk modified screen-printed electrodes via the application of a magnetic field
title_sort enhancing the efficiency of the hydrogen evolution reaction utilising fe(3)p bulk modified screen-printed electrodes via the application of a magnetic field
topic Chemistry
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8695104/
https://www.ncbi.nlm.nih.gov/pubmed/35423332
http://dx.doi.org/10.1039/d0ra10150h
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