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Enhancing the efficiency of the hydrogen evolution reaction utilising Fe(3)P bulk modified screen-printed electrodes via the application of a magnetic field
We report the fabrication and optimisation of Fe(3)P bulk modified screen-printed electrochemical platforms (SPEs) for the hydrogen evolution reaction (HER) within acidic media. We optimise the achievable current density towards the HER of the Fe(3)P SPEs by utilising ball-milled Fe(3)P variants and...
Autores principales: | , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
The Royal Society of Chemistry
2021
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8695104/ https://www.ncbi.nlm.nih.gov/pubmed/35423332 http://dx.doi.org/10.1039/d0ra10150h |
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author | Hughes, Jack. P. Rowley-Neale, Samuel Banks, Craig |
author_facet | Hughes, Jack. P. Rowley-Neale, Samuel Banks, Craig |
author_sort | Hughes, Jack. P. |
collection | PubMed |
description | We report the fabrication and optimisation of Fe(3)P bulk modified screen-printed electrochemical platforms (SPEs) for the hydrogen evolution reaction (HER) within acidic media. We optimise the achievable current density towards the HER of the Fe(3)P SPEs by utilising ball-milled Fe(3)P variants and increasing the mass percentage of Fe(3)P incorporated into the SPEs. Additionally, the synergy of the application of a variable weak (constant) external magnetic field (330 mT to 40 mT) beneficially augments the current density output by 56%. This paper not only highlights the benefits of physical catalyst optimisation but also demonstrates a methodology to further enhance the cathodic efficiency of the HER with the facile application of a weak (constant) magnetic field. |
format | Online Article Text |
id | pubmed-8695104 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2021 |
publisher | The Royal Society of Chemistry |
record_format | MEDLINE/PubMed |
spelling | pubmed-86951042022-04-13 Enhancing the efficiency of the hydrogen evolution reaction utilising Fe(3)P bulk modified screen-printed electrodes via the application of a magnetic field Hughes, Jack. P. Rowley-Neale, Samuel Banks, Craig RSC Adv Chemistry We report the fabrication and optimisation of Fe(3)P bulk modified screen-printed electrochemical platforms (SPEs) for the hydrogen evolution reaction (HER) within acidic media. We optimise the achievable current density towards the HER of the Fe(3)P SPEs by utilising ball-milled Fe(3)P variants and increasing the mass percentage of Fe(3)P incorporated into the SPEs. Additionally, the synergy of the application of a variable weak (constant) external magnetic field (330 mT to 40 mT) beneficially augments the current density output by 56%. This paper not only highlights the benefits of physical catalyst optimisation but also demonstrates a methodology to further enhance the cathodic efficiency of the HER with the facile application of a weak (constant) magnetic field. The Royal Society of Chemistry 2021-02-18 /pmc/articles/PMC8695104/ /pubmed/35423332 http://dx.doi.org/10.1039/d0ra10150h Text en This journal is © The Royal Society of Chemistry https://creativecommons.org/licenses/by-nc/3.0/ |
spellingShingle | Chemistry Hughes, Jack. P. Rowley-Neale, Samuel Banks, Craig Enhancing the efficiency of the hydrogen evolution reaction utilising Fe(3)P bulk modified screen-printed electrodes via the application of a magnetic field |
title | Enhancing the efficiency of the hydrogen evolution reaction utilising Fe(3)P bulk modified screen-printed electrodes via the application of a magnetic field |
title_full | Enhancing the efficiency of the hydrogen evolution reaction utilising Fe(3)P bulk modified screen-printed electrodes via the application of a magnetic field |
title_fullStr | Enhancing the efficiency of the hydrogen evolution reaction utilising Fe(3)P bulk modified screen-printed electrodes via the application of a magnetic field |
title_full_unstemmed | Enhancing the efficiency of the hydrogen evolution reaction utilising Fe(3)P bulk modified screen-printed electrodes via the application of a magnetic field |
title_short | Enhancing the efficiency of the hydrogen evolution reaction utilising Fe(3)P bulk modified screen-printed electrodes via the application of a magnetic field |
title_sort | enhancing the efficiency of the hydrogen evolution reaction utilising fe(3)p bulk modified screen-printed electrodes via the application of a magnetic field |
topic | Chemistry |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8695104/ https://www.ncbi.nlm.nih.gov/pubmed/35423332 http://dx.doi.org/10.1039/d0ra10150h |
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