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Quantum Confinement Suppressing Electronic Heat Flow below the Wiedemann–Franz Law

[Image: see text] The Wiedemann–Franz law states that the charge conductance and the electronic contribution to the heat conductance are proportional. This sets stringent constraints on efficiency bounds for thermoelectric applications, which seek a large charge conduction in response to a small hea...

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Autores principales: Majidi, Danial, Josefsson, Martin, Kumar, Mukesh, Leijnse, Martin, Samuelson, Lars, Courtois, Hervé, Winkelmann, Clemens B., Maisi, Ville F.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2022
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8802316/
https://www.ncbi.nlm.nih.gov/pubmed/35030004
http://dx.doi.org/10.1021/acs.nanolett.1c03437
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author Majidi, Danial
Josefsson, Martin
Kumar, Mukesh
Leijnse, Martin
Samuelson, Lars
Courtois, Hervé
Winkelmann, Clemens B.
Maisi, Ville F.
author_facet Majidi, Danial
Josefsson, Martin
Kumar, Mukesh
Leijnse, Martin
Samuelson, Lars
Courtois, Hervé
Winkelmann, Clemens B.
Maisi, Ville F.
author_sort Majidi, Danial
collection PubMed
description [Image: see text] The Wiedemann–Franz law states that the charge conductance and the electronic contribution to the heat conductance are proportional. This sets stringent constraints on efficiency bounds for thermoelectric applications, which seek a large charge conduction in response to a small heat flow. We present experiments based on a quantum dot formed inside a semiconducting InAs nanowire transistor, in which the heat conduction can be tuned significantly below the Wiedemann–Franz prediction. Comparison with scattering theory shows that this is caused by quantum confinement and the resulting energy-selective transport properties of the quantum dot. Our results open up perspectives for tailoring independently the heat and electrical conduction properties in semiconductor nanostructures.
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spelling pubmed-88023162022-02-01 Quantum Confinement Suppressing Electronic Heat Flow below the Wiedemann–Franz Law Majidi, Danial Josefsson, Martin Kumar, Mukesh Leijnse, Martin Samuelson, Lars Courtois, Hervé Winkelmann, Clemens B. Maisi, Ville F. Nano Lett [Image: see text] The Wiedemann–Franz law states that the charge conductance and the electronic contribution to the heat conductance are proportional. This sets stringent constraints on efficiency bounds for thermoelectric applications, which seek a large charge conduction in response to a small heat flow. We present experiments based on a quantum dot formed inside a semiconducting InAs nanowire transistor, in which the heat conduction can be tuned significantly below the Wiedemann–Franz prediction. Comparison with scattering theory shows that this is caused by quantum confinement and the resulting energy-selective transport properties of the quantum dot. Our results open up perspectives for tailoring independently the heat and electrical conduction properties in semiconductor nanostructures. American Chemical Society 2022-01-14 2022-01-26 /pmc/articles/PMC8802316/ /pubmed/35030004 http://dx.doi.org/10.1021/acs.nanolett.1c03437 Text en © 2022 American Chemical Society https://creativecommons.org/licenses/by/4.0/Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Majidi, Danial
Josefsson, Martin
Kumar, Mukesh
Leijnse, Martin
Samuelson, Lars
Courtois, Hervé
Winkelmann, Clemens B.
Maisi, Ville F.
Quantum Confinement Suppressing Electronic Heat Flow below the Wiedemann–Franz Law
title Quantum Confinement Suppressing Electronic Heat Flow below the Wiedemann–Franz Law
title_full Quantum Confinement Suppressing Electronic Heat Flow below the Wiedemann–Franz Law
title_fullStr Quantum Confinement Suppressing Electronic Heat Flow below the Wiedemann–Franz Law
title_full_unstemmed Quantum Confinement Suppressing Electronic Heat Flow below the Wiedemann–Franz Law
title_short Quantum Confinement Suppressing Electronic Heat Flow below the Wiedemann–Franz Law
title_sort quantum confinement suppressing electronic heat flow below the wiedemann–franz law
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8802316/
https://www.ncbi.nlm.nih.gov/pubmed/35030004
http://dx.doi.org/10.1021/acs.nanolett.1c03437
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