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Giant anomalous Nernst signal in the antiferromagnet YbMnBi(2)

A large anomalous Nernst effect (ANE) is crucial for thermoelectric energy conversion applications because the associated unique transverse geometry facilitates module fabrication. Topological ferromagnets with large Berry curvatures show large ANEs; however, they face drawbacks such as strong magne...

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Detalles Bibliográficos
Autores principales: Pan, Yu, Le, Congcong, He, Bin, Watzman, Sarah J., Yao, Mengyu, Gooth, Johannes, Heremans, Joseph P., Sun, Yan, Felser, Claudia
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8810386/
https://www.ncbi.nlm.nih.gov/pubmed/34811495
http://dx.doi.org/10.1038/s41563-021-01149-2
Descripción
Sumario:A large anomalous Nernst effect (ANE) is crucial for thermoelectric energy conversion applications because the associated unique transverse geometry facilitates module fabrication. Topological ferromagnets with large Berry curvatures show large ANEs; however, they face drawbacks such as strong magnetic disturbances and low mobility due to high magnetization. Herein, we demonstrate that YbMnBi(2), a canted antiferromagnet, has a large ANE conductivity of ~10 A m(−1) K(−1) that surpasses large values observed in other ferromagnets (3–5 A m(−1) K(−1)). The canted spin structure of Mn guarantees a non-zero Berry curvature, but generates only a weak magnetization three orders of magnitude lower than that of general ferromagnets. The heavy Bi with a large spin–orbit coupling enables a large ANE and low thermal conductivity, whereas its highly dispersive p(x/y) orbitals ensure low resistivity. The high anomalous transverse thermoelectric performance and extremely small magnetization make YbMnBi(2) an excellent candidate for transverse thermoelectrics.