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Giant anomalous Nernst signal in the antiferromagnet YbMnBi(2)
A large anomalous Nernst effect (ANE) is crucial for thermoelectric energy conversion applications because the associated unique transverse geometry facilitates module fabrication. Topological ferromagnets with large Berry curvatures show large ANEs; however, they face drawbacks such as strong magne...
Autores principales: | , , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group UK
2021
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8810386/ https://www.ncbi.nlm.nih.gov/pubmed/34811495 http://dx.doi.org/10.1038/s41563-021-01149-2 |
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author | Pan, Yu Le, Congcong He, Bin Watzman, Sarah J. Yao, Mengyu Gooth, Johannes Heremans, Joseph P. Sun, Yan Felser, Claudia |
author_facet | Pan, Yu Le, Congcong He, Bin Watzman, Sarah J. Yao, Mengyu Gooth, Johannes Heremans, Joseph P. Sun, Yan Felser, Claudia |
author_sort | Pan, Yu |
collection | PubMed |
description | A large anomalous Nernst effect (ANE) is crucial for thermoelectric energy conversion applications because the associated unique transverse geometry facilitates module fabrication. Topological ferromagnets with large Berry curvatures show large ANEs; however, they face drawbacks such as strong magnetic disturbances and low mobility due to high magnetization. Herein, we demonstrate that YbMnBi(2), a canted antiferromagnet, has a large ANE conductivity of ~10 A m(−1) K(−1) that surpasses large values observed in other ferromagnets (3–5 A m(−1) K(−1)). The canted spin structure of Mn guarantees a non-zero Berry curvature, but generates only a weak magnetization three orders of magnitude lower than that of general ferromagnets. The heavy Bi with a large spin–orbit coupling enables a large ANE and low thermal conductivity, whereas its highly dispersive p(x/y) orbitals ensure low resistivity. The high anomalous transverse thermoelectric performance and extremely small magnetization make YbMnBi(2) an excellent candidate for transverse thermoelectrics. |
format | Online Article Text |
id | pubmed-8810386 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2021 |
publisher | Nature Publishing Group UK |
record_format | MEDLINE/PubMed |
spelling | pubmed-88103862022-02-09 Giant anomalous Nernst signal in the antiferromagnet YbMnBi(2) Pan, Yu Le, Congcong He, Bin Watzman, Sarah J. Yao, Mengyu Gooth, Johannes Heremans, Joseph P. Sun, Yan Felser, Claudia Nat Mater Article A large anomalous Nernst effect (ANE) is crucial for thermoelectric energy conversion applications because the associated unique transverse geometry facilitates module fabrication. Topological ferromagnets with large Berry curvatures show large ANEs; however, they face drawbacks such as strong magnetic disturbances and low mobility due to high magnetization. Herein, we demonstrate that YbMnBi(2), a canted antiferromagnet, has a large ANE conductivity of ~10 A m(−1) K(−1) that surpasses large values observed in other ferromagnets (3–5 A m(−1) K(−1)). The canted spin structure of Mn guarantees a non-zero Berry curvature, but generates only a weak magnetization three orders of magnitude lower than that of general ferromagnets. The heavy Bi with a large spin–orbit coupling enables a large ANE and low thermal conductivity, whereas its highly dispersive p(x/y) orbitals ensure low resistivity. The high anomalous transverse thermoelectric performance and extremely small magnetization make YbMnBi(2) an excellent candidate for transverse thermoelectrics. Nature Publishing Group UK 2021-11-22 2022 /pmc/articles/PMC8810386/ /pubmed/34811495 http://dx.doi.org/10.1038/s41563-021-01149-2 Text en © The Author(s) 2021 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) . |
spellingShingle | Article Pan, Yu Le, Congcong He, Bin Watzman, Sarah J. Yao, Mengyu Gooth, Johannes Heremans, Joseph P. Sun, Yan Felser, Claudia Giant anomalous Nernst signal in the antiferromagnet YbMnBi(2) |
title | Giant anomalous Nernst signal in the antiferromagnet YbMnBi(2) |
title_full | Giant anomalous Nernst signal in the antiferromagnet YbMnBi(2) |
title_fullStr | Giant anomalous Nernst signal in the antiferromagnet YbMnBi(2) |
title_full_unstemmed | Giant anomalous Nernst signal in the antiferromagnet YbMnBi(2) |
title_short | Giant anomalous Nernst signal in the antiferromagnet YbMnBi(2) |
title_sort | giant anomalous nernst signal in the antiferromagnet ybmnbi(2) |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8810386/ https://www.ncbi.nlm.nih.gov/pubmed/34811495 http://dx.doi.org/10.1038/s41563-021-01149-2 |
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