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Giant anomalous Nernst signal in the antiferromagnet YbMnBi(2)

A large anomalous Nernst effect (ANE) is crucial for thermoelectric energy conversion applications because the associated unique transverse geometry facilitates module fabrication. Topological ferromagnets with large Berry curvatures show large ANEs; however, they face drawbacks such as strong magne...

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Autores principales: Pan, Yu, Le, Congcong, He, Bin, Watzman, Sarah J., Yao, Mengyu, Gooth, Johannes, Heremans, Joseph P., Sun, Yan, Felser, Claudia
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8810386/
https://www.ncbi.nlm.nih.gov/pubmed/34811495
http://dx.doi.org/10.1038/s41563-021-01149-2
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author Pan, Yu
Le, Congcong
He, Bin
Watzman, Sarah J.
Yao, Mengyu
Gooth, Johannes
Heremans, Joseph P.
Sun, Yan
Felser, Claudia
author_facet Pan, Yu
Le, Congcong
He, Bin
Watzman, Sarah J.
Yao, Mengyu
Gooth, Johannes
Heremans, Joseph P.
Sun, Yan
Felser, Claudia
author_sort Pan, Yu
collection PubMed
description A large anomalous Nernst effect (ANE) is crucial for thermoelectric energy conversion applications because the associated unique transverse geometry facilitates module fabrication. Topological ferromagnets with large Berry curvatures show large ANEs; however, they face drawbacks such as strong magnetic disturbances and low mobility due to high magnetization. Herein, we demonstrate that YbMnBi(2), a canted antiferromagnet, has a large ANE conductivity of ~10 A m(−1) K(−1) that surpasses large values observed in other ferromagnets (3–5 A m(−1) K(−1)). The canted spin structure of Mn guarantees a non-zero Berry curvature, but generates only a weak magnetization three orders of magnitude lower than that of general ferromagnets. The heavy Bi with a large spin–orbit coupling enables a large ANE and low thermal conductivity, whereas its highly dispersive p(x/y) orbitals ensure low resistivity. The high anomalous transverse thermoelectric performance and extremely small magnetization make YbMnBi(2) an excellent candidate for transverse thermoelectrics.
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spelling pubmed-88103862022-02-09 Giant anomalous Nernst signal in the antiferromagnet YbMnBi(2) Pan, Yu Le, Congcong He, Bin Watzman, Sarah J. Yao, Mengyu Gooth, Johannes Heremans, Joseph P. Sun, Yan Felser, Claudia Nat Mater Article A large anomalous Nernst effect (ANE) is crucial for thermoelectric energy conversion applications because the associated unique transverse geometry facilitates module fabrication. Topological ferromagnets with large Berry curvatures show large ANEs; however, they face drawbacks such as strong magnetic disturbances and low mobility due to high magnetization. Herein, we demonstrate that YbMnBi(2), a canted antiferromagnet, has a large ANE conductivity of ~10 A m(−1) K(−1) that surpasses large values observed in other ferromagnets (3–5 A m(−1) K(−1)). The canted spin structure of Mn guarantees a non-zero Berry curvature, but generates only a weak magnetization three orders of magnitude lower than that of general ferromagnets. The heavy Bi with a large spin–orbit coupling enables a large ANE and low thermal conductivity, whereas its highly dispersive p(x/y) orbitals ensure low resistivity. The high anomalous transverse thermoelectric performance and extremely small magnetization make YbMnBi(2) an excellent candidate for transverse thermoelectrics. Nature Publishing Group UK 2021-11-22 2022 /pmc/articles/PMC8810386/ /pubmed/34811495 http://dx.doi.org/10.1038/s41563-021-01149-2 Text en © The Author(s) 2021 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Pan, Yu
Le, Congcong
He, Bin
Watzman, Sarah J.
Yao, Mengyu
Gooth, Johannes
Heremans, Joseph P.
Sun, Yan
Felser, Claudia
Giant anomalous Nernst signal in the antiferromagnet YbMnBi(2)
title Giant anomalous Nernst signal in the antiferromagnet YbMnBi(2)
title_full Giant anomalous Nernst signal in the antiferromagnet YbMnBi(2)
title_fullStr Giant anomalous Nernst signal in the antiferromagnet YbMnBi(2)
title_full_unstemmed Giant anomalous Nernst signal in the antiferromagnet YbMnBi(2)
title_short Giant anomalous Nernst signal in the antiferromagnet YbMnBi(2)
title_sort giant anomalous nernst signal in the antiferromagnet ybmnbi(2)
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8810386/
https://www.ncbi.nlm.nih.gov/pubmed/34811495
http://dx.doi.org/10.1038/s41563-021-01149-2
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