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Terahertz Fingerprint of Monolayer Wigner Crystals

[Image: see text] The strong Coulomb interaction in monolayer semiconductors represents a unique opportunity for the realization of Wigner crystals without external magnetic fields. In this work, we predict that the formation of monolayer Wigner crystals can be detected by their terahertz response s...

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Detalles Bibliográficos
Autores principales: Brem, Samuel, Malic, Ermin
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2022
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8832488/
https://www.ncbi.nlm.nih.gov/pubmed/35048702
http://dx.doi.org/10.1021/acs.nanolett.1c04620
Descripción
Sumario:[Image: see text] The strong Coulomb interaction in monolayer semiconductors represents a unique opportunity for the realization of Wigner crystals without external magnetic fields. In this work, we predict that the formation of monolayer Wigner crystals can be detected by their terahertz response spectrum, which exhibits a characteristic sequence of internal optical transitions. We apply the density matrix formalism to derive the internal quantum structure and the optical conductivity of the Wigner crystal and to microscopically analyze the multipeak shape of the obtained terahertz spectrum. Moreover, we predict a characteristic shift of the peak position as a function of charge density for different atomically thin materials and show how our results can be generalized to an arbitrary two-dimensional system.