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Terahertz Fingerprint of Monolayer Wigner Crystals
[Image: see text] The strong Coulomb interaction in monolayer semiconductors represents a unique opportunity for the realization of Wigner crystals without external magnetic fields. In this work, we predict that the formation of monolayer Wigner crystals can be detected by their terahertz response s...
Autores principales: | , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Chemical Society
2022
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Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8832488/ https://www.ncbi.nlm.nih.gov/pubmed/35048702 http://dx.doi.org/10.1021/acs.nanolett.1c04620 |
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author | Brem, Samuel Malic, Ermin |
author_facet | Brem, Samuel Malic, Ermin |
author_sort | Brem, Samuel |
collection | PubMed |
description | [Image: see text] The strong Coulomb interaction in monolayer semiconductors represents a unique opportunity for the realization of Wigner crystals without external magnetic fields. In this work, we predict that the formation of monolayer Wigner crystals can be detected by their terahertz response spectrum, which exhibits a characteristic sequence of internal optical transitions. We apply the density matrix formalism to derive the internal quantum structure and the optical conductivity of the Wigner crystal and to microscopically analyze the multipeak shape of the obtained terahertz spectrum. Moreover, we predict a characteristic shift of the peak position as a function of charge density for different atomically thin materials and show how our results can be generalized to an arbitrary two-dimensional system. |
format | Online Article Text |
id | pubmed-8832488 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2022 |
publisher | American Chemical Society |
record_format | MEDLINE/PubMed |
spelling | pubmed-88324882022-02-11 Terahertz Fingerprint of Monolayer Wigner Crystals Brem, Samuel Malic, Ermin Nano Lett [Image: see text] The strong Coulomb interaction in monolayer semiconductors represents a unique opportunity for the realization of Wigner crystals without external magnetic fields. In this work, we predict that the formation of monolayer Wigner crystals can be detected by their terahertz response spectrum, which exhibits a characteristic sequence of internal optical transitions. We apply the density matrix formalism to derive the internal quantum structure and the optical conductivity of the Wigner crystal and to microscopically analyze the multipeak shape of the obtained terahertz spectrum. Moreover, we predict a characteristic shift of the peak position as a function of charge density for different atomically thin materials and show how our results can be generalized to an arbitrary two-dimensional system. American Chemical Society 2022-01-20 2022-02-09 /pmc/articles/PMC8832488/ /pubmed/35048702 http://dx.doi.org/10.1021/acs.nanolett.1c04620 Text en © 2022 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by/4.0/Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/). |
spellingShingle | Brem, Samuel Malic, Ermin Terahertz Fingerprint of Monolayer Wigner Crystals |
title | Terahertz Fingerprint of Monolayer Wigner Crystals |
title_full | Terahertz Fingerprint of Monolayer Wigner Crystals |
title_fullStr | Terahertz Fingerprint of Monolayer Wigner Crystals |
title_full_unstemmed | Terahertz Fingerprint of Monolayer Wigner Crystals |
title_short | Terahertz Fingerprint of Monolayer Wigner Crystals |
title_sort | terahertz fingerprint of monolayer wigner crystals |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8832488/ https://www.ncbi.nlm.nih.gov/pubmed/35048702 http://dx.doi.org/10.1021/acs.nanolett.1c04620 |
work_keys_str_mv | AT bremsamuel terahertzfingerprintofmonolayerwignercrystals AT malicermin terahertzfingerprintofmonolayerwignercrystals |