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Electron Dynamics and Correlations During High-Order Harmonic Generation in Be

We investigate theoretically the high-order harmonic generation in beryllium atom irradiated by a short 1850 nm linearly polarized laser pulse in the intermediate strong-field ionization regime with the Keldysh parameter of 0.85. To this end, the respective time-dependent Schrödinger equation is sol...

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Autores principales: Kutscher, Eric, Artemyev, Anton N., Demekhin, Philipp V.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Frontiers Media S.A. 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8841356/
https://www.ncbi.nlm.nih.gov/pubmed/35174138
http://dx.doi.org/10.3389/fchem.2022.809137
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author Kutscher, Eric
Artemyev, Anton N.
Demekhin, Philipp V.
author_facet Kutscher, Eric
Artemyev, Anton N.
Demekhin, Philipp V.
author_sort Kutscher, Eric
collection PubMed
description We investigate theoretically the high-order harmonic generation in beryllium atom irradiated by a short 1850 nm linearly polarized laser pulse in the intermediate strong-field ionization regime with the Keldysh parameter of 0.85. To this end, the respective time-dependent Schrödinger equation is solved by the time-dependent restricted-active-space configuration-interaction (TD-RASCI) method. By systematically increasing the active space of included configurations, we demonstrate an individual effect of different physical processes evoked by the pulse, which, all together, significantly enrich and extend the computed high-order harmonic generation spectrum.
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spelling pubmed-88413562022-02-15 Electron Dynamics and Correlations During High-Order Harmonic Generation in Be Kutscher, Eric Artemyev, Anton N. Demekhin, Philipp V. Front Chem Chemistry We investigate theoretically the high-order harmonic generation in beryllium atom irradiated by a short 1850 nm linearly polarized laser pulse in the intermediate strong-field ionization regime with the Keldysh parameter of 0.85. To this end, the respective time-dependent Schrödinger equation is solved by the time-dependent restricted-active-space configuration-interaction (TD-RASCI) method. By systematically increasing the active space of included configurations, we demonstrate an individual effect of different physical processes evoked by the pulse, which, all together, significantly enrich and extend the computed high-order harmonic generation spectrum. Frontiers Media S.A. 2022-01-31 /pmc/articles/PMC8841356/ /pubmed/35174138 http://dx.doi.org/10.3389/fchem.2022.809137 Text en Copyright © 2022 Kutscher, Artemyev and Demekhin. https://creativecommons.org/licenses/by/4.0/This is an open-access article distributed under the terms of the Creative Commons Attribution License (CC BY). The use, distribution or reproduction in other forums is permitted, provided the original author(s) and the copyright owner(s) are credited and that the original publication in this journal is cited, in accordance with accepted academic practice. No use, distribution or reproduction is permitted which does not comply with these terms.
spellingShingle Chemistry
Kutscher, Eric
Artemyev, Anton N.
Demekhin, Philipp V.
Electron Dynamics and Correlations During High-Order Harmonic Generation in Be
title Electron Dynamics and Correlations During High-Order Harmonic Generation in Be
title_full Electron Dynamics and Correlations During High-Order Harmonic Generation in Be
title_fullStr Electron Dynamics and Correlations During High-Order Harmonic Generation in Be
title_full_unstemmed Electron Dynamics and Correlations During High-Order Harmonic Generation in Be
title_short Electron Dynamics and Correlations During High-Order Harmonic Generation in Be
title_sort electron dynamics and correlations during high-order harmonic generation in be
topic Chemistry
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8841356/
https://www.ncbi.nlm.nih.gov/pubmed/35174138
http://dx.doi.org/10.3389/fchem.2022.809137
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