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Universality of ultrasonic attenuation coefficient of amorphous systems at low temperatures

The competition between unretarded dispersion interactions between molecules prevailing at medium range order length scales and their phonon induced coupling at larger scales leads to appearance of nano-scale sub structures in amorphous systems. The complexity of intermolecular interactions gives ri...

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Autor principal: Shukla, Pragya
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8854728/
https://www.ncbi.nlm.nih.gov/pubmed/35177709
http://dx.doi.org/10.1038/s41598-022-06589-7
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author Shukla, Pragya
author_facet Shukla, Pragya
author_sort Shukla, Pragya
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description The competition between unretarded dispersion interactions between molecules prevailing at medium range order length scales and their phonon induced coupling at larger scales leads to appearance of nano-scale sub structures in amorphous systems. The complexity of intermolecular interactions gives rise to randomization of their operators. Based on a random matrix modelling of the Hamiltonian and its linear response to an external strain field, we show that the ultrasonic attenuation coefficient can be expressed as a ratio of two crucial length-scales related to molecular dynamics. A nearly constant value of the ratio for a wide range of materials then provides a theoretical explanation of the experimentally observed qualitative universality of the ultrasonic attenuation coefficient at low temperatures.
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spelling pubmed-88547282022-02-22 Universality of ultrasonic attenuation coefficient of amorphous systems at low temperatures Shukla, Pragya Sci Rep Article The competition between unretarded dispersion interactions between molecules prevailing at medium range order length scales and their phonon induced coupling at larger scales leads to appearance of nano-scale sub structures in amorphous systems. The complexity of intermolecular interactions gives rise to randomization of their operators. Based on a random matrix modelling of the Hamiltonian and its linear response to an external strain field, we show that the ultrasonic attenuation coefficient can be expressed as a ratio of two crucial length-scales related to molecular dynamics. A nearly constant value of the ratio for a wide range of materials then provides a theoretical explanation of the experimentally observed qualitative universality of the ultrasonic attenuation coefficient at low temperatures. Nature Publishing Group UK 2022-02-17 /pmc/articles/PMC8854728/ /pubmed/35177709 http://dx.doi.org/10.1038/s41598-022-06589-7 Text en © The Author(s) 2022 https://creativecommons.org/licenses/by/4.0/Open AccessThis article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article's Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article's Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Shukla, Pragya
Universality of ultrasonic attenuation coefficient of amorphous systems at low temperatures
title Universality of ultrasonic attenuation coefficient of amorphous systems at low temperatures
title_full Universality of ultrasonic attenuation coefficient of amorphous systems at low temperatures
title_fullStr Universality of ultrasonic attenuation coefficient of amorphous systems at low temperatures
title_full_unstemmed Universality of ultrasonic attenuation coefficient of amorphous systems at low temperatures
title_short Universality of ultrasonic attenuation coefficient of amorphous systems at low temperatures
title_sort universality of ultrasonic attenuation coefficient of amorphous systems at low temperatures
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8854728/
https://www.ncbi.nlm.nih.gov/pubmed/35177709
http://dx.doi.org/10.1038/s41598-022-06589-7
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