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Universality of ultrasonic attenuation coefficient of amorphous systems at low temperatures
The competition between unretarded dispersion interactions between molecules prevailing at medium range order length scales and their phonon induced coupling at larger scales leads to appearance of nano-scale sub structures in amorphous systems. The complexity of intermolecular interactions gives ri...
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Formato: | Online Artículo Texto |
Lenguaje: | English |
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Nature Publishing Group UK
2022
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Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8854728/ https://www.ncbi.nlm.nih.gov/pubmed/35177709 http://dx.doi.org/10.1038/s41598-022-06589-7 |
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author | Shukla, Pragya |
author_facet | Shukla, Pragya |
author_sort | Shukla, Pragya |
collection | PubMed |
description | The competition between unretarded dispersion interactions between molecules prevailing at medium range order length scales and their phonon induced coupling at larger scales leads to appearance of nano-scale sub structures in amorphous systems. The complexity of intermolecular interactions gives rise to randomization of their operators. Based on a random matrix modelling of the Hamiltonian and its linear response to an external strain field, we show that the ultrasonic attenuation coefficient can be expressed as a ratio of two crucial length-scales related to molecular dynamics. A nearly constant value of the ratio for a wide range of materials then provides a theoretical explanation of the experimentally observed qualitative universality of the ultrasonic attenuation coefficient at low temperatures. |
format | Online Article Text |
id | pubmed-8854728 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2022 |
publisher | Nature Publishing Group UK |
record_format | MEDLINE/PubMed |
spelling | pubmed-88547282022-02-22 Universality of ultrasonic attenuation coefficient of amorphous systems at low temperatures Shukla, Pragya Sci Rep Article The competition between unretarded dispersion interactions between molecules prevailing at medium range order length scales and their phonon induced coupling at larger scales leads to appearance of nano-scale sub structures in amorphous systems. The complexity of intermolecular interactions gives rise to randomization of their operators. Based on a random matrix modelling of the Hamiltonian and its linear response to an external strain field, we show that the ultrasonic attenuation coefficient can be expressed as a ratio of two crucial length-scales related to molecular dynamics. A nearly constant value of the ratio for a wide range of materials then provides a theoretical explanation of the experimentally observed qualitative universality of the ultrasonic attenuation coefficient at low temperatures. Nature Publishing Group UK 2022-02-17 /pmc/articles/PMC8854728/ /pubmed/35177709 http://dx.doi.org/10.1038/s41598-022-06589-7 Text en © The Author(s) 2022 https://creativecommons.org/licenses/by/4.0/Open AccessThis article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article's Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article's Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) . |
spellingShingle | Article Shukla, Pragya Universality of ultrasonic attenuation coefficient of amorphous systems at low temperatures |
title | Universality of ultrasonic attenuation coefficient of amorphous systems at low temperatures |
title_full | Universality of ultrasonic attenuation coefficient of amorphous systems at low temperatures |
title_fullStr | Universality of ultrasonic attenuation coefficient of amorphous systems at low temperatures |
title_full_unstemmed | Universality of ultrasonic attenuation coefficient of amorphous systems at low temperatures |
title_short | Universality of ultrasonic attenuation coefficient of amorphous systems at low temperatures |
title_sort | universality of ultrasonic attenuation coefficient of amorphous systems at low temperatures |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8854728/ https://www.ncbi.nlm.nih.gov/pubmed/35177709 http://dx.doi.org/10.1038/s41598-022-06589-7 |
work_keys_str_mv | AT shuklapragya universalityofultrasonicattenuationcoefficientofamorphoussystemsatlowtemperatures |