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Intermixed Time-Dependent Self-Focusing and Defocusing Nonlinearities in Polymer Solutions

[Image: see text] Low-power visible light can lead to spectacular nonlinear effects in soft-matter systems. The propagation of visible light through transparent solutions of certain polymers can experience either self-focusing or defocusing nonlinearity, depending on the solvent. We show how the sel...

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Detalles Bibliográficos
Autores principales: Bogris, Athanasios, Burger, Nikolaos A., Makris, Konstantinos G., Loppinet, Benoit, Fytas, George
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2022
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8855434/
https://www.ncbi.nlm.nih.gov/pubmed/35211646
http://dx.doi.org/10.1021/acsphotonics.1c01917
Descripción
Sumario:[Image: see text] Low-power visible light can lead to spectacular nonlinear effects in soft-matter systems. The propagation of visible light through transparent solutions of certain polymers can experience either self-focusing or defocusing nonlinearity, depending on the solvent. We show how the self-focusing and defocusing responses can be captured by a nonlinear propagation model using local spatial and time-integrating responses. We realize a remarkable pattern formation in ternary solutions and model it assuming a linear combination of the self-focusing and defocusing nonlinearities in the constituent solvents. This versatile response of solutions to light irradiation may introduce a new approach for self-written waveguides and patterns.