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Intermixed Time-Dependent Self-Focusing and Defocusing Nonlinearities in Polymer Solutions

[Image: see text] Low-power visible light can lead to spectacular nonlinear effects in soft-matter systems. The propagation of visible light through transparent solutions of certain polymers can experience either self-focusing or defocusing nonlinearity, depending on the solvent. We show how the sel...

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Autores principales: Bogris, Athanasios, Burger, Nikolaos A., Makris, Konstantinos G., Loppinet, Benoit, Fytas, George
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2022
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8855434/
https://www.ncbi.nlm.nih.gov/pubmed/35211646
http://dx.doi.org/10.1021/acsphotonics.1c01917
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author Bogris, Athanasios
Burger, Nikolaos A.
Makris, Konstantinos G.
Loppinet, Benoit
Fytas, George
author_facet Bogris, Athanasios
Burger, Nikolaos A.
Makris, Konstantinos G.
Loppinet, Benoit
Fytas, George
author_sort Bogris, Athanasios
collection PubMed
description [Image: see text] Low-power visible light can lead to spectacular nonlinear effects in soft-matter systems. The propagation of visible light through transparent solutions of certain polymers can experience either self-focusing or defocusing nonlinearity, depending on the solvent. We show how the self-focusing and defocusing responses can be captured by a nonlinear propagation model using local spatial and time-integrating responses. We realize a remarkable pattern formation in ternary solutions and model it assuming a linear combination of the self-focusing and defocusing nonlinearities in the constituent solvents. This versatile response of solutions to light irradiation may introduce a new approach for self-written waveguides and patterns.
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spelling pubmed-88554342022-02-22 Intermixed Time-Dependent Self-Focusing and Defocusing Nonlinearities in Polymer Solutions Bogris, Athanasios Burger, Nikolaos A. Makris, Konstantinos G. Loppinet, Benoit Fytas, George ACS Photonics [Image: see text] Low-power visible light can lead to spectacular nonlinear effects in soft-matter systems. The propagation of visible light through transparent solutions of certain polymers can experience either self-focusing or defocusing nonlinearity, depending on the solvent. We show how the self-focusing and defocusing responses can be captured by a nonlinear propagation model using local spatial and time-integrating responses. We realize a remarkable pattern formation in ternary solutions and model it assuming a linear combination of the self-focusing and defocusing nonlinearities in the constituent solvents. This versatile response of solutions to light irradiation may introduce a new approach for self-written waveguides and patterns. American Chemical Society 2022-02-01 2022-02-16 /pmc/articles/PMC8855434/ /pubmed/35211646 http://dx.doi.org/10.1021/acsphotonics.1c01917 Text en © 2022 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by/4.0/Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Bogris, Athanasios
Burger, Nikolaos A.
Makris, Konstantinos G.
Loppinet, Benoit
Fytas, George
Intermixed Time-Dependent Self-Focusing and Defocusing Nonlinearities in Polymer Solutions
title Intermixed Time-Dependent Self-Focusing and Defocusing Nonlinearities in Polymer Solutions
title_full Intermixed Time-Dependent Self-Focusing and Defocusing Nonlinearities in Polymer Solutions
title_fullStr Intermixed Time-Dependent Self-Focusing and Defocusing Nonlinearities in Polymer Solutions
title_full_unstemmed Intermixed Time-Dependent Self-Focusing and Defocusing Nonlinearities in Polymer Solutions
title_short Intermixed Time-Dependent Self-Focusing and Defocusing Nonlinearities in Polymer Solutions
title_sort intermixed time-dependent self-focusing and defocusing nonlinearities in polymer solutions
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8855434/
https://www.ncbi.nlm.nih.gov/pubmed/35211646
http://dx.doi.org/10.1021/acsphotonics.1c01917
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