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Intermixed Time-Dependent Self-Focusing and Defocusing Nonlinearities in Polymer Solutions
[Image: see text] Low-power visible light can lead to spectacular nonlinear effects in soft-matter systems. The propagation of visible light through transparent solutions of certain polymers can experience either self-focusing or defocusing nonlinearity, depending on the solvent. We show how the sel...
Autores principales: | , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Chemical Society
2022
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Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8855434/ https://www.ncbi.nlm.nih.gov/pubmed/35211646 http://dx.doi.org/10.1021/acsphotonics.1c01917 |
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author | Bogris, Athanasios Burger, Nikolaos A. Makris, Konstantinos G. Loppinet, Benoit Fytas, George |
author_facet | Bogris, Athanasios Burger, Nikolaos A. Makris, Konstantinos G. Loppinet, Benoit Fytas, George |
author_sort | Bogris, Athanasios |
collection | PubMed |
description | [Image: see text] Low-power visible light can lead to spectacular nonlinear effects in soft-matter systems. The propagation of visible light through transparent solutions of certain polymers can experience either self-focusing or defocusing nonlinearity, depending on the solvent. We show how the self-focusing and defocusing responses can be captured by a nonlinear propagation model using local spatial and time-integrating responses. We realize a remarkable pattern formation in ternary solutions and model it assuming a linear combination of the self-focusing and defocusing nonlinearities in the constituent solvents. This versatile response of solutions to light irradiation may introduce a new approach for self-written waveguides and patterns. |
format | Online Article Text |
id | pubmed-8855434 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2022 |
publisher | American Chemical Society |
record_format | MEDLINE/PubMed |
spelling | pubmed-88554342022-02-22 Intermixed Time-Dependent Self-Focusing and Defocusing Nonlinearities in Polymer Solutions Bogris, Athanasios Burger, Nikolaos A. Makris, Konstantinos G. Loppinet, Benoit Fytas, George ACS Photonics [Image: see text] Low-power visible light can lead to spectacular nonlinear effects in soft-matter systems. The propagation of visible light through transparent solutions of certain polymers can experience either self-focusing or defocusing nonlinearity, depending on the solvent. We show how the self-focusing and defocusing responses can be captured by a nonlinear propagation model using local spatial and time-integrating responses. We realize a remarkable pattern formation in ternary solutions and model it assuming a linear combination of the self-focusing and defocusing nonlinearities in the constituent solvents. This versatile response of solutions to light irradiation may introduce a new approach for self-written waveguides and patterns. American Chemical Society 2022-02-01 2022-02-16 /pmc/articles/PMC8855434/ /pubmed/35211646 http://dx.doi.org/10.1021/acsphotonics.1c01917 Text en © 2022 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by/4.0/Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/). |
spellingShingle | Bogris, Athanasios Burger, Nikolaos A. Makris, Konstantinos G. Loppinet, Benoit Fytas, George Intermixed Time-Dependent Self-Focusing and Defocusing Nonlinearities in Polymer Solutions |
title | Intermixed Time-Dependent Self-Focusing and Defocusing
Nonlinearities in Polymer Solutions |
title_full | Intermixed Time-Dependent Self-Focusing and Defocusing
Nonlinearities in Polymer Solutions |
title_fullStr | Intermixed Time-Dependent Self-Focusing and Defocusing
Nonlinearities in Polymer Solutions |
title_full_unstemmed | Intermixed Time-Dependent Self-Focusing and Defocusing
Nonlinearities in Polymer Solutions |
title_short | Intermixed Time-Dependent Self-Focusing and Defocusing
Nonlinearities in Polymer Solutions |
title_sort | intermixed time-dependent self-focusing and defocusing
nonlinearities in polymer solutions |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8855434/ https://www.ncbi.nlm.nih.gov/pubmed/35211646 http://dx.doi.org/10.1021/acsphotonics.1c01917 |
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