Highly Dispersed CoO Embedded on Graphitized Ordered Mesoporous Carbon as an Effective Catalyst for Selective Fischer–Tropsch Synthesis of C(5+) Hydrocarbons

Herein, we report the high Fischer–Tropsch synthesis performance of the Co-based catalysts supported on graphitized ordered mesoporous carbon (GMC-900) by using a facile strategy. Compared with CMK-3 and active carbon (AC), the obtained GMC-900 by using pollution-free soybean oil as a carbon source...

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Autores principales: Bai, Jirong, Song, Mingyao, Pang, Jiazheng, Wang, Lingling, Zhang, Jianping, Jiang, Xiankai, Ni, Zhijiang, Wang, Zhilei, Zhou, Quanfa
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Frontiers Media S.A. 2022
Materias:
Chemistry
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8866306/
https://www.ncbi.nlm.nih.gov/pubmed/35223776
http://dx.doi.org/10.3389/fchem.2022.849505
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author Bai, Jirong
Song, Mingyao
Pang, Jiazheng
Wang, Lingling
Zhang, Jianping
Jiang, Xiankai
Ni, Zhijiang
Wang, Zhilei
Zhou, Quanfa
author_facet Bai, Jirong
Song, Mingyao
Pang, Jiazheng
Wang, Lingling
Zhang, Jianping
Jiang, Xiankai
Ni, Zhijiang
Wang, Zhilei
Zhou, Quanfa
author_sort Bai, Jirong
collection PubMed
description Herein, we report the high Fischer–Tropsch synthesis performance of the Co-based catalysts supported on graphitized ordered mesoporous carbon (GMC-900) by using a facile strategy. Compared with CMK-3 and active carbon (AC), the obtained GMC-900 by using pollution-free soybean oil as a carbon source exhibited enhanced catalytic performance after loading Co species due to its highly crystallized graphitic structure and uniform dispersion of CoO. As a result, Co/GMC-900 was an effective catalyst with the maximum C(5+) selectivity of 52.6%, which much outperformed Co/CMK-3 and Co/AC. This research provides an approach to produce advanced Co-based catalysts with satisfactory performance for efficient Fischer–Tropsch synthesis.
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spelling pubmed-88663062022-02-25 Highly Dispersed CoO Embedded on Graphitized Ordered Mesoporous Carbon as an Effective Catalyst for Selective Fischer–Tropsch Synthesis of C(5+) Hydrocarbons Bai, Jirong Song, Mingyao Pang, Jiazheng Wang, Lingling Zhang, Jianping Jiang, Xiankai Ni, Zhijiang Wang, Zhilei Zhou, Quanfa Front Chem Chemistry Herein, we report the high Fischer–Tropsch synthesis performance of the Co-based catalysts supported on graphitized ordered mesoporous carbon (GMC-900) by using a facile strategy. Compared with CMK-3 and active carbon (AC), the obtained GMC-900 by using pollution-free soybean oil as a carbon source exhibited enhanced catalytic performance after loading Co species due to its highly crystallized graphitic structure and uniform dispersion of CoO. As a result, Co/GMC-900 was an effective catalyst with the maximum C(5+) selectivity of 52.6%, which much outperformed Co/CMK-3 and Co/AC. This research provides an approach to produce advanced Co-based catalysts with satisfactory performance for efficient Fischer–Tropsch synthesis. Frontiers Media S.A. 2022-02-10 /pmc/articles/PMC8866306/ /pubmed/35223776 http://dx.doi.org/10.3389/fchem.2022.849505 Text en Copyright © 2022 Bai, Song, Pang, Wang, Zhang, Jiang, Ni, Wang and Zhou. https://creativecommons.org/licenses/by/4.0/This is an open-access article distributed under the terms of the Creative Commons Attribution License (CC BY). The use, distribution or reproduction in other forums is permitted, provided the original author(s) and the copyright owner(s) are credited and that the original publication in this journal is cited, in accordance with accepted academic practice. No use, distribution or reproduction is permitted which does not comply with these terms.
spellingShingle Chemistry
Bai, Jirong
Song, Mingyao
Pang, Jiazheng
Wang, Lingling
Zhang, Jianping
Jiang, Xiankai
Ni, Zhijiang
Wang, Zhilei
Zhou, Quanfa
Highly Dispersed CoO Embedded on Graphitized Ordered Mesoporous Carbon as an Effective Catalyst for Selective Fischer–Tropsch Synthesis of C(5+) Hydrocarbons
title Highly Dispersed CoO Embedded on Graphitized Ordered Mesoporous Carbon as an Effective Catalyst for Selective Fischer–Tropsch Synthesis of C(5+) Hydrocarbons
title_full Highly Dispersed CoO Embedded on Graphitized Ordered Mesoporous Carbon as an Effective Catalyst for Selective Fischer–Tropsch Synthesis of C(5+) Hydrocarbons
title_fullStr Highly Dispersed CoO Embedded on Graphitized Ordered Mesoporous Carbon as an Effective Catalyst for Selective Fischer–Tropsch Synthesis of C(5+) Hydrocarbons
title_full_unstemmed Highly Dispersed CoO Embedded on Graphitized Ordered Mesoporous Carbon as an Effective Catalyst for Selective Fischer–Tropsch Synthesis of C(5+) Hydrocarbons
title_short Highly Dispersed CoO Embedded on Graphitized Ordered Mesoporous Carbon as an Effective Catalyst for Selective Fischer–Tropsch Synthesis of C(5+) Hydrocarbons
title_sort highly dispersed coo embedded on graphitized ordered mesoporous carbon as an effective catalyst for selective fischer–tropsch synthesis of c(5+) hydrocarbons
topic Chemistry
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8866306/
https://www.ncbi.nlm.nih.gov/pubmed/35223776
http://dx.doi.org/10.3389/fchem.2022.849505
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