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Temperature-Based Selective Detection of Hydrogen Sulfide and Ethanol with MoS(2)/WO(3) Composite
[Image: see text] A sensitive and temperature-based selective sensor toward hydrogen sulfide and ethanol using MoS(2)/WO(3) composite as a sensing surface was developed in this work. The MoS(2)/WO(3) nanocomposite was successfully obtained using a facile two-step method. Structural analysis revealed...
Autores principales: | , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Chemical Society
2022
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Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8867485/ https://www.ncbi.nlm.nih.gov/pubmed/35224369 http://dx.doi.org/10.1021/acsomega.1c06471 |
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author | Singh, Sukhwinder Sharma, Sandeep |
author_facet | Singh, Sukhwinder Sharma, Sandeep |
author_sort | Singh, Sukhwinder |
collection | PubMed |
description | [Image: see text] A sensitive and temperature-based selective sensor toward hydrogen sulfide and ethanol using MoS(2)/WO(3) composite as a sensing surface was developed in this work. The MoS(2)/WO(3) nanocomposite was successfully obtained using a facile two-step method. Structural analysis revealed the successful formation of the composite. Further, the n-type semiconducting nature as revealed in the initial gas-sensing measurements was also confirmed via Mott–Schottky plots. The composite-based sensor showed preferential detection of ethanol (260 °C) and hydrogen sulfide (320 °C) by simply modulating the temperature of the sensor device. The device also displayed repeatability and long-term stability at respective operating temperatures. Improved sensitivity and selectivity are ascribed to synergistic effects arising from the formation of n–n type heterostructures. The present work indicates the potential use of composite-based heterojunctions to tune the sensing parameters and provide new possibilities to enhance the applications of MoS(2) and metal-oxide semiconductor-based composites. |
format | Online Article Text |
id | pubmed-8867485 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2022 |
publisher | American Chemical Society |
record_format | MEDLINE/PubMed |
spelling | pubmed-88674852022-02-25 Temperature-Based Selective Detection of Hydrogen Sulfide and Ethanol with MoS(2)/WO(3) Composite Singh, Sukhwinder Sharma, Sandeep ACS Omega [Image: see text] A sensitive and temperature-based selective sensor toward hydrogen sulfide and ethanol using MoS(2)/WO(3) composite as a sensing surface was developed in this work. The MoS(2)/WO(3) nanocomposite was successfully obtained using a facile two-step method. Structural analysis revealed the successful formation of the composite. Further, the n-type semiconducting nature as revealed in the initial gas-sensing measurements was also confirmed via Mott–Schottky plots. The composite-based sensor showed preferential detection of ethanol (260 °C) and hydrogen sulfide (320 °C) by simply modulating the temperature of the sensor device. The device also displayed repeatability and long-term stability at respective operating temperatures. Improved sensitivity and selectivity are ascribed to synergistic effects arising from the formation of n–n type heterostructures. The present work indicates the potential use of composite-based heterojunctions to tune the sensing parameters and provide new possibilities to enhance the applications of MoS(2) and metal-oxide semiconductor-based composites. American Chemical Society 2022-02-07 /pmc/articles/PMC8867485/ /pubmed/35224369 http://dx.doi.org/10.1021/acsomega.1c06471 Text en © 2022 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by-nc-nd/4.0/Permits non-commercial access and re-use, provided that author attribution and integrity are maintained; but does not permit creation of adaptations or other derivative works (https://creativecommons.org/licenses/by-nc-nd/4.0/). |
spellingShingle | Singh, Sukhwinder Sharma, Sandeep Temperature-Based Selective Detection of Hydrogen Sulfide and Ethanol with MoS(2)/WO(3) Composite |
title | Temperature-Based Selective Detection of Hydrogen
Sulfide and Ethanol with MoS(2)/WO(3) Composite |
title_full | Temperature-Based Selective Detection of Hydrogen
Sulfide and Ethanol with MoS(2)/WO(3) Composite |
title_fullStr | Temperature-Based Selective Detection of Hydrogen
Sulfide and Ethanol with MoS(2)/WO(3) Composite |
title_full_unstemmed | Temperature-Based Selective Detection of Hydrogen
Sulfide and Ethanol with MoS(2)/WO(3) Composite |
title_short | Temperature-Based Selective Detection of Hydrogen
Sulfide and Ethanol with MoS(2)/WO(3) Composite |
title_sort | temperature-based selective detection of hydrogen
sulfide and ethanol with mos(2)/wo(3) composite |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8867485/ https://www.ncbi.nlm.nih.gov/pubmed/35224369 http://dx.doi.org/10.1021/acsomega.1c06471 |
work_keys_str_mv | AT singhsukhwinder temperaturebasedselectivedetectionofhydrogensulfideandethanolwithmos2wo3composite AT sharmasandeep temperaturebasedselectivedetectionofhydrogensulfideandethanolwithmos2wo3composite |