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A Facile Preparation of Multicolor Carbon Dots

Carbon dots (CDs) have raised broad interest because of their great potential in the fluorescence related fields, such as photocatalysis and bioimaging. CDs exhibit different optical properties when dissolved in various solvents. However, the effects of solvents during the process of preparation on...

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Autores principales: Yu, Risheng, Liang, Sen, Ru, Yi, Li, Lu, Wang, Zhikun, Chen, Junlang, Chen, Liang
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Springer US 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8904681/
https://www.ncbi.nlm.nih.gov/pubmed/35258709
http://dx.doi.org/10.1186/s11671-022-03661-z
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author Yu, Risheng
Liang, Sen
Ru, Yi
Li, Lu
Wang, Zhikun
Chen, Junlang
Chen, Liang
author_facet Yu, Risheng
Liang, Sen
Ru, Yi
Li, Lu
Wang, Zhikun
Chen, Junlang
Chen, Liang
author_sort Yu, Risheng
collection PubMed
description Carbon dots (CDs) have raised broad interest because of their great potential in the fluorescence related fields, such as photocatalysis and bioimaging. CDs exhibit different optical properties when dissolved in various solvents. However, the effects of solvents during the process of preparation on the fluorescence emission of CDs are still unclear. In this work, CDs were prepared by a simple one-pot solvothermal route. Typical critic acid and thiourea were used as precursors. Through changing the volume ratio of water to N,N-dimethylformamide (DMF), we have obtained color tunable CDs, with the emission wavelength from 450 to 640 nm. TEM images, Raman and XPS spectra indicate that the particle size of CDs and the content of surface functional groups (C–N/C–S and C≡N bonds) increase with the increasing ratio of DMF to water, which results in the optimal emission wavelength red-shifted. The prepared multicolor CDs may have prospects in the lighting applications. GRAPHICAL ABSTRACT: [Image: see text] SUPPLEMENTARY INFORMATION: The online version contains supplementary material available at 10.1186/s11671-022-03661-z.
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spelling pubmed-89046812022-03-15 A Facile Preparation of Multicolor Carbon Dots Yu, Risheng Liang, Sen Ru, Yi Li, Lu Wang, Zhikun Chen, Junlang Chen, Liang Nanoscale Res Lett Nano Express Carbon dots (CDs) have raised broad interest because of their great potential in the fluorescence related fields, such as photocatalysis and bioimaging. CDs exhibit different optical properties when dissolved in various solvents. However, the effects of solvents during the process of preparation on the fluorescence emission of CDs are still unclear. In this work, CDs were prepared by a simple one-pot solvothermal route. Typical critic acid and thiourea were used as precursors. Through changing the volume ratio of water to N,N-dimethylformamide (DMF), we have obtained color tunable CDs, with the emission wavelength from 450 to 640 nm. TEM images, Raman and XPS spectra indicate that the particle size of CDs and the content of surface functional groups (C–N/C–S and C≡N bonds) increase with the increasing ratio of DMF to water, which results in the optimal emission wavelength red-shifted. The prepared multicolor CDs may have prospects in the lighting applications. GRAPHICAL ABSTRACT: [Image: see text] SUPPLEMENTARY INFORMATION: The online version contains supplementary material available at 10.1186/s11671-022-03661-z. Springer US 2022-03-08 /pmc/articles/PMC8904681/ /pubmed/35258709 http://dx.doi.org/10.1186/s11671-022-03661-z Text en © The Author(s) 2022 https://creativecommons.org/licenses/by/4.0/Open AccessThis article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article's Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article's Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Nano Express
Yu, Risheng
Liang, Sen
Ru, Yi
Li, Lu
Wang, Zhikun
Chen, Junlang
Chen, Liang
A Facile Preparation of Multicolor Carbon Dots
title A Facile Preparation of Multicolor Carbon Dots
title_full A Facile Preparation of Multicolor Carbon Dots
title_fullStr A Facile Preparation of Multicolor Carbon Dots
title_full_unstemmed A Facile Preparation of Multicolor Carbon Dots
title_short A Facile Preparation of Multicolor Carbon Dots
title_sort facile preparation of multicolor carbon dots
topic Nano Express
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8904681/
https://www.ncbi.nlm.nih.gov/pubmed/35258709
http://dx.doi.org/10.1186/s11671-022-03661-z
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