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Explorations on Growth of Blue-Green-Yellow-Red InGaN Quantum Dots by Plasma-Assisted Molecular Beam Epitaxy

Self-assembled growth of blue-green-yellow-red InGaN quantum dots (QDs) on GaN templates using plasma-assisted molecular beam epitaxy were investigated. We concluded that growth conditions, including small N(2) flow and high growth temperature are beneficial to the formation of InGaN QDs and improve...

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Autores principales: Zhang, Xue, Xing, Zhiwei, Yang, Wenxian, Qiu, Haibing, Gu, Ying, Suzuki, Yuta, Kaneko, Sakuya, Matsuda, Yuki, Izumi, Shinji, Nakamura, Yuichi, Cai, Yong, Bian, Lifeng, Lu, Shulong, Tackeuchi, Atsushi
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8912505/
https://www.ncbi.nlm.nih.gov/pubmed/35269287
http://dx.doi.org/10.3390/nano12050800
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author Zhang, Xue
Xing, Zhiwei
Yang, Wenxian
Qiu, Haibing
Gu, Ying
Suzuki, Yuta
Kaneko, Sakuya
Matsuda, Yuki
Izumi, Shinji
Nakamura, Yuichi
Cai, Yong
Bian, Lifeng
Lu, Shulong
Tackeuchi, Atsushi
author_facet Zhang, Xue
Xing, Zhiwei
Yang, Wenxian
Qiu, Haibing
Gu, Ying
Suzuki, Yuta
Kaneko, Sakuya
Matsuda, Yuki
Izumi, Shinji
Nakamura, Yuichi
Cai, Yong
Bian, Lifeng
Lu, Shulong
Tackeuchi, Atsushi
author_sort Zhang, Xue
collection PubMed
description Self-assembled growth of blue-green-yellow-red InGaN quantum dots (QDs) on GaN templates using plasma-assisted molecular beam epitaxy were investigated. We concluded that growth conditions, including small N(2) flow and high growth temperature are beneficial to the formation of InGaN QDs and improve the crystal quality. The lower In/Ga flux ratio and lower growth temperature are favorable for the formation of QDs of long emission wavelength. Moreover, the nitrogen modulation epitaxy method can extend the wavelength of QDs from green to red. As a result, visible light emissions from 460 nm to 622 nm have been achieved. Furthermore, a 505 nm green light-emitting diode (LED) based on InGaN/GaN MQDs was prepared. The LED has a low external quantum efficiency of 0.14% and shows an efficiency droop with increasing injection current. However, electroluminescence spectra exhibited a strong wavelength stability, with a negligible shift of less than 1.0 nm as injection current density increased from 8 A/cm(2) to 160 A/cm(2), owing to the screening of polarization-related electric field in QDs.
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spelling pubmed-89125052022-03-11 Explorations on Growth of Blue-Green-Yellow-Red InGaN Quantum Dots by Plasma-Assisted Molecular Beam Epitaxy Zhang, Xue Xing, Zhiwei Yang, Wenxian Qiu, Haibing Gu, Ying Suzuki, Yuta Kaneko, Sakuya Matsuda, Yuki Izumi, Shinji Nakamura, Yuichi Cai, Yong Bian, Lifeng Lu, Shulong Tackeuchi, Atsushi Nanomaterials (Basel) Article Self-assembled growth of blue-green-yellow-red InGaN quantum dots (QDs) on GaN templates using plasma-assisted molecular beam epitaxy were investigated. We concluded that growth conditions, including small N(2) flow and high growth temperature are beneficial to the formation of InGaN QDs and improve the crystal quality. The lower In/Ga flux ratio and lower growth temperature are favorable for the formation of QDs of long emission wavelength. Moreover, the nitrogen modulation epitaxy method can extend the wavelength of QDs from green to red. As a result, visible light emissions from 460 nm to 622 nm have been achieved. Furthermore, a 505 nm green light-emitting diode (LED) based on InGaN/GaN MQDs was prepared. The LED has a low external quantum efficiency of 0.14% and shows an efficiency droop with increasing injection current. However, electroluminescence spectra exhibited a strong wavelength stability, with a negligible shift of less than 1.0 nm as injection current density increased from 8 A/cm(2) to 160 A/cm(2), owing to the screening of polarization-related electric field in QDs. MDPI 2022-02-26 /pmc/articles/PMC8912505/ /pubmed/35269287 http://dx.doi.org/10.3390/nano12050800 Text en © 2022 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Zhang, Xue
Xing, Zhiwei
Yang, Wenxian
Qiu, Haibing
Gu, Ying
Suzuki, Yuta
Kaneko, Sakuya
Matsuda, Yuki
Izumi, Shinji
Nakamura, Yuichi
Cai, Yong
Bian, Lifeng
Lu, Shulong
Tackeuchi, Atsushi
Explorations on Growth of Blue-Green-Yellow-Red InGaN Quantum Dots by Plasma-Assisted Molecular Beam Epitaxy
title Explorations on Growth of Blue-Green-Yellow-Red InGaN Quantum Dots by Plasma-Assisted Molecular Beam Epitaxy
title_full Explorations on Growth of Blue-Green-Yellow-Red InGaN Quantum Dots by Plasma-Assisted Molecular Beam Epitaxy
title_fullStr Explorations on Growth of Blue-Green-Yellow-Red InGaN Quantum Dots by Plasma-Assisted Molecular Beam Epitaxy
title_full_unstemmed Explorations on Growth of Blue-Green-Yellow-Red InGaN Quantum Dots by Plasma-Assisted Molecular Beam Epitaxy
title_short Explorations on Growth of Blue-Green-Yellow-Red InGaN Quantum Dots by Plasma-Assisted Molecular Beam Epitaxy
title_sort explorations on growth of blue-green-yellow-red ingan quantum dots by plasma-assisted molecular beam epitaxy
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8912505/
https://www.ncbi.nlm.nih.gov/pubmed/35269287
http://dx.doi.org/10.3390/nano12050800
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