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One-Pot Method to Synthesize Silver Nanoparticle-Modified Bamboo-Based Carbon Aerogels for Formaldehyde Removal

The present study demonstrated a freeze-drying-carbonization method to synthesize silver nanoparticle-modified bamboo-based carbon aerogels to remove formaldehyde. The bamboo-based carbon aerogel (BCA) has the advantages of controllable pore size and rich oxygen-containing groups, which can provide...

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Detalles Bibliográficos
Autores principales: Jing, Wenxiang, Yang, Chai, Luo, Shuang, Lin, Xiaoyan, Tang, Min, Zheng, Renhong, Lian, Dongming, Luo, Xuegang
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8912511/
https://www.ncbi.nlm.nih.gov/pubmed/35267682
http://dx.doi.org/10.3390/polym14050860
Descripción
Sumario:The present study demonstrated a freeze-drying-carbonization method to synthesize silver nanoparticle-modified bamboo-based carbon aerogels to remove formaldehyde. The bamboo-based carbon aerogel (BCA) has the advantages of controllable pore size and rich oxygen-containing groups, which can provide a good foundation for surface modification. BCA can greatly enhance the purification of formaldehyde by loading silver nanoparticles. The maximum adsorption capacity of 5% Ag/BCA for formaldehyde reached 42 mg/g under 25 ppm formaldehyde concentration, which is 5.25 times more than that of BCA. The relevant data were fitted by the Langmuir model and the pseudo 2nd-order model and good results were obtained, indicating that chemical absorption occurred between the carbonyl of formaldehyde and the hydroxyl of BCA. Therefore, silver nanoparticle-modified bamboo-based carbon aerogels play a positive role in the selective removal of formaldehyde. Silver nanoparticles promoted the activation of oxygen and strengthened the effect of BCA on HCHO adsorption.