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One-Pot Method to Synthesize Silver Nanoparticle-Modified Bamboo-Based Carbon Aerogels for Formaldehyde Removal
The present study demonstrated a freeze-drying-carbonization method to synthesize silver nanoparticle-modified bamboo-based carbon aerogels to remove formaldehyde. The bamboo-based carbon aerogel (BCA) has the advantages of controllable pore size and rich oxygen-containing groups, which can provide...
Autores principales: | , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
MDPI
2022
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8912511/ https://www.ncbi.nlm.nih.gov/pubmed/35267682 http://dx.doi.org/10.3390/polym14050860 |
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author | Jing, Wenxiang Yang, Chai Luo, Shuang Lin, Xiaoyan Tang, Min Zheng, Renhong Lian, Dongming Luo, Xuegang |
author_facet | Jing, Wenxiang Yang, Chai Luo, Shuang Lin, Xiaoyan Tang, Min Zheng, Renhong Lian, Dongming Luo, Xuegang |
author_sort | Jing, Wenxiang |
collection | PubMed |
description | The present study demonstrated a freeze-drying-carbonization method to synthesize silver nanoparticle-modified bamboo-based carbon aerogels to remove formaldehyde. The bamboo-based carbon aerogel (BCA) has the advantages of controllable pore size and rich oxygen-containing groups, which can provide a good foundation for surface modification. BCA can greatly enhance the purification of formaldehyde by loading silver nanoparticles. The maximum adsorption capacity of 5% Ag/BCA for formaldehyde reached 42 mg/g under 25 ppm formaldehyde concentration, which is 5.25 times more than that of BCA. The relevant data were fitted by the Langmuir model and the pseudo 2nd-order model and good results were obtained, indicating that chemical absorption occurred between the carbonyl of formaldehyde and the hydroxyl of BCA. Therefore, silver nanoparticle-modified bamboo-based carbon aerogels play a positive role in the selective removal of formaldehyde. Silver nanoparticles promoted the activation of oxygen and strengthened the effect of BCA on HCHO adsorption. |
format | Online Article Text |
id | pubmed-8912511 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2022 |
publisher | MDPI |
record_format | MEDLINE/PubMed |
spelling | pubmed-89125112022-03-11 One-Pot Method to Synthesize Silver Nanoparticle-Modified Bamboo-Based Carbon Aerogels for Formaldehyde Removal Jing, Wenxiang Yang, Chai Luo, Shuang Lin, Xiaoyan Tang, Min Zheng, Renhong Lian, Dongming Luo, Xuegang Polymers (Basel) Article The present study demonstrated a freeze-drying-carbonization method to synthesize silver nanoparticle-modified bamboo-based carbon aerogels to remove formaldehyde. The bamboo-based carbon aerogel (BCA) has the advantages of controllable pore size and rich oxygen-containing groups, which can provide a good foundation for surface modification. BCA can greatly enhance the purification of formaldehyde by loading silver nanoparticles. The maximum adsorption capacity of 5% Ag/BCA for formaldehyde reached 42 mg/g under 25 ppm formaldehyde concentration, which is 5.25 times more than that of BCA. The relevant data were fitted by the Langmuir model and the pseudo 2nd-order model and good results were obtained, indicating that chemical absorption occurred between the carbonyl of formaldehyde and the hydroxyl of BCA. Therefore, silver nanoparticle-modified bamboo-based carbon aerogels play a positive role in the selective removal of formaldehyde. Silver nanoparticles promoted the activation of oxygen and strengthened the effect of BCA on HCHO adsorption. MDPI 2022-02-22 /pmc/articles/PMC8912511/ /pubmed/35267682 http://dx.doi.org/10.3390/polym14050860 Text en © 2022 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/). |
spellingShingle | Article Jing, Wenxiang Yang, Chai Luo, Shuang Lin, Xiaoyan Tang, Min Zheng, Renhong Lian, Dongming Luo, Xuegang One-Pot Method to Synthesize Silver Nanoparticle-Modified Bamboo-Based Carbon Aerogels for Formaldehyde Removal |
title | One-Pot Method to Synthesize Silver Nanoparticle-Modified Bamboo-Based Carbon Aerogels for Formaldehyde Removal |
title_full | One-Pot Method to Synthesize Silver Nanoparticle-Modified Bamboo-Based Carbon Aerogels for Formaldehyde Removal |
title_fullStr | One-Pot Method to Synthesize Silver Nanoparticle-Modified Bamboo-Based Carbon Aerogels for Formaldehyde Removal |
title_full_unstemmed | One-Pot Method to Synthesize Silver Nanoparticle-Modified Bamboo-Based Carbon Aerogels for Formaldehyde Removal |
title_short | One-Pot Method to Synthesize Silver Nanoparticle-Modified Bamboo-Based Carbon Aerogels for Formaldehyde Removal |
title_sort | one-pot method to synthesize silver nanoparticle-modified bamboo-based carbon aerogels for formaldehyde removal |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8912511/ https://www.ncbi.nlm.nih.gov/pubmed/35267682 http://dx.doi.org/10.3390/polym14050860 |
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