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One-Pot Method to Synthesize Silver Nanoparticle-Modified Bamboo-Based Carbon Aerogels for Formaldehyde Removal

The present study demonstrated a freeze-drying-carbonization method to synthesize silver nanoparticle-modified bamboo-based carbon aerogels to remove formaldehyde. The bamboo-based carbon aerogel (BCA) has the advantages of controllable pore size and rich oxygen-containing groups, which can provide...

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Autores principales: Jing, Wenxiang, Yang, Chai, Luo, Shuang, Lin, Xiaoyan, Tang, Min, Zheng, Renhong, Lian, Dongming, Luo, Xuegang
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8912511/
https://www.ncbi.nlm.nih.gov/pubmed/35267682
http://dx.doi.org/10.3390/polym14050860
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author Jing, Wenxiang
Yang, Chai
Luo, Shuang
Lin, Xiaoyan
Tang, Min
Zheng, Renhong
Lian, Dongming
Luo, Xuegang
author_facet Jing, Wenxiang
Yang, Chai
Luo, Shuang
Lin, Xiaoyan
Tang, Min
Zheng, Renhong
Lian, Dongming
Luo, Xuegang
author_sort Jing, Wenxiang
collection PubMed
description The present study demonstrated a freeze-drying-carbonization method to synthesize silver nanoparticle-modified bamboo-based carbon aerogels to remove formaldehyde. The bamboo-based carbon aerogel (BCA) has the advantages of controllable pore size and rich oxygen-containing groups, which can provide a good foundation for surface modification. BCA can greatly enhance the purification of formaldehyde by loading silver nanoparticles. The maximum adsorption capacity of 5% Ag/BCA for formaldehyde reached 42 mg/g under 25 ppm formaldehyde concentration, which is 5.25 times more than that of BCA. The relevant data were fitted by the Langmuir model and the pseudo 2nd-order model and good results were obtained, indicating that chemical absorption occurred between the carbonyl of formaldehyde and the hydroxyl of BCA. Therefore, silver nanoparticle-modified bamboo-based carbon aerogels play a positive role in the selective removal of formaldehyde. Silver nanoparticles promoted the activation of oxygen and strengthened the effect of BCA on HCHO adsorption.
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spelling pubmed-89125112022-03-11 One-Pot Method to Synthesize Silver Nanoparticle-Modified Bamboo-Based Carbon Aerogels for Formaldehyde Removal Jing, Wenxiang Yang, Chai Luo, Shuang Lin, Xiaoyan Tang, Min Zheng, Renhong Lian, Dongming Luo, Xuegang Polymers (Basel) Article The present study demonstrated a freeze-drying-carbonization method to synthesize silver nanoparticle-modified bamboo-based carbon aerogels to remove formaldehyde. The bamboo-based carbon aerogel (BCA) has the advantages of controllable pore size and rich oxygen-containing groups, which can provide a good foundation for surface modification. BCA can greatly enhance the purification of formaldehyde by loading silver nanoparticles. The maximum adsorption capacity of 5% Ag/BCA for formaldehyde reached 42 mg/g under 25 ppm formaldehyde concentration, which is 5.25 times more than that of BCA. The relevant data were fitted by the Langmuir model and the pseudo 2nd-order model and good results were obtained, indicating that chemical absorption occurred between the carbonyl of formaldehyde and the hydroxyl of BCA. Therefore, silver nanoparticle-modified bamboo-based carbon aerogels play a positive role in the selective removal of formaldehyde. Silver nanoparticles promoted the activation of oxygen and strengthened the effect of BCA on HCHO adsorption. MDPI 2022-02-22 /pmc/articles/PMC8912511/ /pubmed/35267682 http://dx.doi.org/10.3390/polym14050860 Text en © 2022 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Jing, Wenxiang
Yang, Chai
Luo, Shuang
Lin, Xiaoyan
Tang, Min
Zheng, Renhong
Lian, Dongming
Luo, Xuegang
One-Pot Method to Synthesize Silver Nanoparticle-Modified Bamboo-Based Carbon Aerogels for Formaldehyde Removal
title One-Pot Method to Synthesize Silver Nanoparticle-Modified Bamboo-Based Carbon Aerogels for Formaldehyde Removal
title_full One-Pot Method to Synthesize Silver Nanoparticle-Modified Bamboo-Based Carbon Aerogels for Formaldehyde Removal
title_fullStr One-Pot Method to Synthesize Silver Nanoparticle-Modified Bamboo-Based Carbon Aerogels for Formaldehyde Removal
title_full_unstemmed One-Pot Method to Synthesize Silver Nanoparticle-Modified Bamboo-Based Carbon Aerogels for Formaldehyde Removal
title_short One-Pot Method to Synthesize Silver Nanoparticle-Modified Bamboo-Based Carbon Aerogels for Formaldehyde Removal
title_sort one-pot method to synthesize silver nanoparticle-modified bamboo-based carbon aerogels for formaldehyde removal
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8912511/
https://www.ncbi.nlm.nih.gov/pubmed/35267682
http://dx.doi.org/10.3390/polym14050860
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