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On chip random lasing performance of the acceptor dye in a specially designed linear and zig zag array of microdroplets with intrinsic disorder

We demonstrate high-quality on chip random lasing of the acceptor dye using a specially designed dynamic linear array of microdroplets with unconventional shapes that do not support the whispering gallery modes. The intrinsic disorder in the droplet array consequent to its dynamic nature is utilized...

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Autores principales: Sundaresan, Aswathy, Nuchikkat, Soniya, Alee, K. Shadak
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8913607/
https://www.ncbi.nlm.nih.gov/pubmed/35273196
http://dx.doi.org/10.1038/s41598-022-07104-8
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author Sundaresan, Aswathy
Nuchikkat, Soniya
Alee, K. Shadak
author_facet Sundaresan, Aswathy
Nuchikkat, Soniya
Alee, K. Shadak
author_sort Sundaresan, Aswathy
collection PubMed
description We demonstrate high-quality on chip random lasing of the acceptor dye using a specially designed dynamic linear array of microdroplets with unconventional shapes that do not support the whispering gallery modes. The intrinsic disorder in the droplet array consequent to its dynamic nature is utilized in achieving the randomness in the lasing emission without deliberately adding the disorder as in ordinary random laser systems. The novelty of the generated structure is illustrated by comparing its emission characteristics with two other arrays made of microspheres and microtriangular droplets arranged in a zig zag fashion. We show that only the linear array of microdroplets supports lasing in the acceptor emission. The design of the array structure allows to further reduce the lasing threshold drastically either by incorporating the radiative energy transfer or by tuning the number of acceptor dye molecules. The highly directional, well-controlled, and intense emission of weakly emitting dye generated on chip without the aid of conventional methods opens up a new scheme of random lasing generation mediated by microdroplets.
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spelling pubmed-89136072022-03-11 On chip random lasing performance of the acceptor dye in a specially designed linear and zig zag array of microdroplets with intrinsic disorder Sundaresan, Aswathy Nuchikkat, Soniya Alee, K. Shadak Sci Rep Article We demonstrate high-quality on chip random lasing of the acceptor dye using a specially designed dynamic linear array of microdroplets with unconventional shapes that do not support the whispering gallery modes. The intrinsic disorder in the droplet array consequent to its dynamic nature is utilized in achieving the randomness in the lasing emission without deliberately adding the disorder as in ordinary random laser systems. The novelty of the generated structure is illustrated by comparing its emission characteristics with two other arrays made of microspheres and microtriangular droplets arranged in a zig zag fashion. We show that only the linear array of microdroplets supports lasing in the acceptor emission. The design of the array structure allows to further reduce the lasing threshold drastically either by incorporating the radiative energy transfer or by tuning the number of acceptor dye molecules. The highly directional, well-controlled, and intense emission of weakly emitting dye generated on chip without the aid of conventional methods opens up a new scheme of random lasing generation mediated by microdroplets. Nature Publishing Group UK 2022-03-10 /pmc/articles/PMC8913607/ /pubmed/35273196 http://dx.doi.org/10.1038/s41598-022-07104-8 Text en © The Author(s) 2022 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article's Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article's Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Sundaresan, Aswathy
Nuchikkat, Soniya
Alee, K. Shadak
On chip random lasing performance of the acceptor dye in a specially designed linear and zig zag array of microdroplets with intrinsic disorder
title On chip random lasing performance of the acceptor dye in a specially designed linear and zig zag array of microdroplets with intrinsic disorder
title_full On chip random lasing performance of the acceptor dye in a specially designed linear and zig zag array of microdroplets with intrinsic disorder
title_fullStr On chip random lasing performance of the acceptor dye in a specially designed linear and zig zag array of microdroplets with intrinsic disorder
title_full_unstemmed On chip random lasing performance of the acceptor dye in a specially designed linear and zig zag array of microdroplets with intrinsic disorder
title_short On chip random lasing performance of the acceptor dye in a specially designed linear and zig zag array of microdroplets with intrinsic disorder
title_sort on chip random lasing performance of the acceptor dye in a specially designed linear and zig zag array of microdroplets with intrinsic disorder
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8913607/
https://www.ncbi.nlm.nih.gov/pubmed/35273196
http://dx.doi.org/10.1038/s41598-022-07104-8
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