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Ultrafast plasmonic photoemission in the single-cycle and few-cycle regimes

Due to the highly increased interest in the development of state-of-the-art applications of photoemission in ultrafast electron microscopy, development of photocathodes and many more applications, a correct theoretical understanding of the underlying phenomena is needed. Within the framework of the...

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Autores principales: Kiss, G. Zs, Földi, P., Dombi, P.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8913738/
https://www.ncbi.nlm.nih.gov/pubmed/35273213
http://dx.doi.org/10.1038/s41598-022-07259-4
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author Kiss, G. Zs
Földi, P.
Dombi, P.
author_facet Kiss, G. Zs
Földi, P.
Dombi, P.
author_sort Kiss, G. Zs
collection PubMed
description Due to the highly increased interest in the development of state-of-the-art applications of photoemission in ultrafast electron microscopy, development of photocathodes and many more applications, a correct theoretical understanding of the underlying phenomena is needed. Within the framework of the single active electron approximation the most accurate results can be obtained by the direct solution of the time-dependent Schrödinger equation (TDSE). In this work, after a brief presentation of a numerically improved version of a mixed 1D-TDSE method, we investigated the characteristics of electron spectra obtained from the surface of metal nanoparticles irradiated with ultrashort laser pulses. During our investigation different decay lengths of the plasmonic-enhanced incident field in the vicinity of the metal were considered. Using the simulated spectra we managed to identify the behavior of the cutoff energy as a function of decay length in the strong-field, multiphoton and transition regimes.
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spelling pubmed-89137382022-03-14 Ultrafast plasmonic photoemission in the single-cycle and few-cycle regimes Kiss, G. Zs Földi, P. Dombi, P. Sci Rep Article Due to the highly increased interest in the development of state-of-the-art applications of photoemission in ultrafast electron microscopy, development of photocathodes and many more applications, a correct theoretical understanding of the underlying phenomena is needed. Within the framework of the single active electron approximation the most accurate results can be obtained by the direct solution of the time-dependent Schrödinger equation (TDSE). In this work, after a brief presentation of a numerically improved version of a mixed 1D-TDSE method, we investigated the characteristics of electron spectra obtained from the surface of metal nanoparticles irradiated with ultrashort laser pulses. During our investigation different decay lengths of the plasmonic-enhanced incident field in the vicinity of the metal were considered. Using the simulated spectra we managed to identify the behavior of the cutoff energy as a function of decay length in the strong-field, multiphoton and transition regimes. Nature Publishing Group UK 2022-03-10 /pmc/articles/PMC8913738/ /pubmed/35273213 http://dx.doi.org/10.1038/s41598-022-07259-4 Text en © The Author(s) 2022 https://creativecommons.org/licenses/by/4.0/Open AccessThis article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article's Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article's Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Kiss, G. Zs
Földi, P.
Dombi, P.
Ultrafast plasmonic photoemission in the single-cycle and few-cycle regimes
title Ultrafast plasmonic photoemission in the single-cycle and few-cycle regimes
title_full Ultrafast plasmonic photoemission in the single-cycle and few-cycle regimes
title_fullStr Ultrafast plasmonic photoemission in the single-cycle and few-cycle regimes
title_full_unstemmed Ultrafast plasmonic photoemission in the single-cycle and few-cycle regimes
title_short Ultrafast plasmonic photoemission in the single-cycle and few-cycle regimes
title_sort ultrafast plasmonic photoemission in the single-cycle and few-cycle regimes
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8913738/
https://www.ncbi.nlm.nih.gov/pubmed/35273213
http://dx.doi.org/10.1038/s41598-022-07259-4
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