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Frustration Dynamics and Electron-Transfer Reorganization Energies in Wild-Type and Mutant Azurins

[Image: see text] Long-range electron tunneling through metalloproteins is facilitated by evolutionary tuning of donor–acceptor electronic couplings, formal electrochemical potentials, and active-site reorganization energies. Although the minimal frustration of the folding landscape enables this tun...

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Detalles Bibliográficos
Autores principales: Chen, Xun, Chen, Mingchen, Wolynes, Peter G., Wittung-Stafshede, Pernilla, Gray, Harry B.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2022
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8915257/
https://www.ncbi.nlm.nih.gov/pubmed/35171591
http://dx.doi.org/10.1021/jacs.1c13454