Cargando…

A mechanism for the strange metal phase in rare-earth intermetallic compounds

A major mystery in strongly interacting quantum systems is the microscopic origin of the “strange metal” phenomenology, with unconventional metallic behavior that defies Landau’s Fermi liquid framework for ordinary metals. This state is found across a wide range of quantum materials, notably in rare...

Descripción completa

Detalles Bibliográficos
Autores principales: Wang, Jiangfan, Chang, Yung-Yeh, Chung, Chung-Hou
Formato: Online Artículo Texto
Lenguaje:English
Publicado: National Academy of Sciences 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8915960/
https://www.ncbi.nlm.nih.gov/pubmed/35238676
http://dx.doi.org/10.1073/pnas.2116980119
_version_ 1784668175939403776
author Wang, Jiangfan
Chang, Yung-Yeh
Chung, Chung-Hou
author_facet Wang, Jiangfan
Chang, Yung-Yeh
Chung, Chung-Hou
author_sort Wang, Jiangfan
collection PubMed
description A major mystery in strongly interacting quantum systems is the microscopic origin of the “strange metal” phenomenology, with unconventional metallic behavior that defies Landau’s Fermi liquid framework for ordinary metals. This state is found across a wide range of quantum materials, notably in rare-earth intermetallic compounds at finite temperatures (T) near a magnetic quantum phase transition, and shows a quasilinear-in-temperature resistivity and a logarithmic-in-temperature specific heat coefficient. Recently, an even more enigmatic behavior pointing toward a stable strange metal ground state was observed in CePd [Formula: see text] Ni(x)Al, a geometrically frustrated Kondo lattice compound. Here, we propose a mechanism for such phenomena driven by the interplay of the gapless fermionic short-ranged antiferromagnetic spin correlations (spinons) and critical bosonic charge (holons) fluctuations near a Kondo breakdown quantum phase transition. Within a dynamical large-N approach to the Kondo–Heisenberg lattice model, the strange metal phase is realized in transport and thermodynamical quantities. It is manifested as a fluctuating Kondo-scattering–stabilized critical (gapless) fermionic spin-liquid metal. It shows [Formula: see text] scaling in dynamical electron scattering rate, a signature of quantum criticality. Our results offer a qualitative understanding of the CePd [Formula: see text] Ni(x)Al compound and suggest a possibility of realizing the quantum critical strange metal phase in correlated electron systems in general.
format Online
Article
Text
id pubmed-8915960
institution National Center for Biotechnology Information
language English
publishDate 2022
publisher National Academy of Sciences
record_format MEDLINE/PubMed
spelling pubmed-89159602022-03-12 A mechanism for the strange metal phase in rare-earth intermetallic compounds Wang, Jiangfan Chang, Yung-Yeh Chung, Chung-Hou Proc Natl Acad Sci U S A Physical Sciences A major mystery in strongly interacting quantum systems is the microscopic origin of the “strange metal” phenomenology, with unconventional metallic behavior that defies Landau’s Fermi liquid framework for ordinary metals. This state is found across a wide range of quantum materials, notably in rare-earth intermetallic compounds at finite temperatures (T) near a magnetic quantum phase transition, and shows a quasilinear-in-temperature resistivity and a logarithmic-in-temperature specific heat coefficient. Recently, an even more enigmatic behavior pointing toward a stable strange metal ground state was observed in CePd [Formula: see text] Ni(x)Al, a geometrically frustrated Kondo lattice compound. Here, we propose a mechanism for such phenomena driven by the interplay of the gapless fermionic short-ranged antiferromagnetic spin correlations (spinons) and critical bosonic charge (holons) fluctuations near a Kondo breakdown quantum phase transition. Within a dynamical large-N approach to the Kondo–Heisenberg lattice model, the strange metal phase is realized in transport and thermodynamical quantities. It is manifested as a fluctuating Kondo-scattering–stabilized critical (gapless) fermionic spin-liquid metal. It shows [Formula: see text] scaling in dynamical electron scattering rate, a signature of quantum criticality. Our results offer a qualitative understanding of the CePd [Formula: see text] Ni(x)Al compound and suggest a possibility of realizing the quantum critical strange metal phase in correlated electron systems in general. National Academy of Sciences 2022-03-01 2022-03-08 /pmc/articles/PMC8915960/ /pubmed/35238676 http://dx.doi.org/10.1073/pnas.2116980119 Text en Copyright © 2022 the Author(s). Published by PNAS. https://creativecommons.org/licenses/by/4.0/This open access article is distributed under Creative Commons Attribution License 4.0 (CC BY) (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Physical Sciences
Wang, Jiangfan
Chang, Yung-Yeh
Chung, Chung-Hou
A mechanism for the strange metal phase in rare-earth intermetallic compounds
title A mechanism for the strange metal phase in rare-earth intermetallic compounds
title_full A mechanism for the strange metal phase in rare-earth intermetallic compounds
title_fullStr A mechanism for the strange metal phase in rare-earth intermetallic compounds
title_full_unstemmed A mechanism for the strange metal phase in rare-earth intermetallic compounds
title_short A mechanism for the strange metal phase in rare-earth intermetallic compounds
title_sort mechanism for the strange metal phase in rare-earth intermetallic compounds
topic Physical Sciences
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8915960/
https://www.ncbi.nlm.nih.gov/pubmed/35238676
http://dx.doi.org/10.1073/pnas.2116980119
work_keys_str_mv AT wangjiangfan amechanismforthestrangemetalphaseinrareearthintermetalliccompounds
AT changyungyeh amechanismforthestrangemetalphaseinrareearthintermetalliccompounds
AT chungchunghou amechanismforthestrangemetalphaseinrareearthintermetalliccompounds
AT wangjiangfan mechanismforthestrangemetalphaseinrareearthintermetalliccompounds
AT changyungyeh mechanismforthestrangemetalphaseinrareearthintermetalliccompounds
AT chungchunghou mechanismforthestrangemetalphaseinrareearthintermetalliccompounds