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Long-range transport of 2D excitons with acoustic waves

Excitons are elementary optical excitation in semiconductors. The ability to manipulate and transport these quasiparticles would enable excitonic circuits and devices for quantum photonic technologies. Recently, interlayer excitons in 2D semiconductors have emerged as a promising candidate for engin...

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Autores principales: Peng, Ruoming, Ripin, Adina, Ye, Yusen, Zhu, Jiayi, Wu, Changming, Lee, Seokhyeong, Li, Huan, Taniguchi, Takashi, Watanabe, Kenji, Cao, Ting, Xu, Xiaodong, Li, Mo
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8921513/
https://www.ncbi.nlm.nih.gov/pubmed/35289330
http://dx.doi.org/10.1038/s41467-022-29042-9
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author Peng, Ruoming
Ripin, Adina
Ye, Yusen
Zhu, Jiayi
Wu, Changming
Lee, Seokhyeong
Li, Huan
Taniguchi, Takashi
Watanabe, Kenji
Cao, Ting
Xu, Xiaodong
Li, Mo
author_facet Peng, Ruoming
Ripin, Adina
Ye, Yusen
Zhu, Jiayi
Wu, Changming
Lee, Seokhyeong
Li, Huan
Taniguchi, Takashi
Watanabe, Kenji
Cao, Ting
Xu, Xiaodong
Li, Mo
author_sort Peng, Ruoming
collection PubMed
description Excitons are elementary optical excitation in semiconductors. The ability to manipulate and transport these quasiparticles would enable excitonic circuits and devices for quantum photonic technologies. Recently, interlayer excitons in 2D semiconductors have emerged as a promising candidate for engineering excitonic devices due to their long lifetime, large exciton binding energy, and gate tunability. However, the charge-neutral nature of the excitons leads to weak response to the in-plane electric field and thus inhibits transport beyond the diffusion length. Here, we demonstrate the directional transport of interlayer excitons in bilayer WSe(2) driven by the propagating potential traps induced by surface acoustic waves (SAW). We show that at 100 K, the SAW-driven excitonic transport is activated above a threshold acoustic power and reaches 20 μm, a distance at least ten times longer than the diffusion length and only limited by the device size. Temperature-dependent measurement reveals the transition from the diffusion-limited regime at low temperature to the acoustic field-driven regime at elevated temperature. Our work shows that acoustic waves are an effective, contact-free means to control exciton dynamics and transport, promising for realizing 2D materials-based excitonic devices such as exciton transistors, switches, and transducers up to room temperature.
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spelling pubmed-89215132022-04-01 Long-range transport of 2D excitons with acoustic waves Peng, Ruoming Ripin, Adina Ye, Yusen Zhu, Jiayi Wu, Changming Lee, Seokhyeong Li, Huan Taniguchi, Takashi Watanabe, Kenji Cao, Ting Xu, Xiaodong Li, Mo Nat Commun Article Excitons are elementary optical excitation in semiconductors. The ability to manipulate and transport these quasiparticles would enable excitonic circuits and devices for quantum photonic technologies. Recently, interlayer excitons in 2D semiconductors have emerged as a promising candidate for engineering excitonic devices due to their long lifetime, large exciton binding energy, and gate tunability. However, the charge-neutral nature of the excitons leads to weak response to the in-plane electric field and thus inhibits transport beyond the diffusion length. Here, we demonstrate the directional transport of interlayer excitons in bilayer WSe(2) driven by the propagating potential traps induced by surface acoustic waves (SAW). We show that at 100 K, the SAW-driven excitonic transport is activated above a threshold acoustic power and reaches 20 μm, a distance at least ten times longer than the diffusion length and only limited by the device size. Temperature-dependent measurement reveals the transition from the diffusion-limited regime at low temperature to the acoustic field-driven regime at elevated temperature. Our work shows that acoustic waves are an effective, contact-free means to control exciton dynamics and transport, promising for realizing 2D materials-based excitonic devices such as exciton transistors, switches, and transducers up to room temperature. Nature Publishing Group UK 2022-03-14 /pmc/articles/PMC8921513/ /pubmed/35289330 http://dx.doi.org/10.1038/s41467-022-29042-9 Text en © The Author(s) 2022 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Peng, Ruoming
Ripin, Adina
Ye, Yusen
Zhu, Jiayi
Wu, Changming
Lee, Seokhyeong
Li, Huan
Taniguchi, Takashi
Watanabe, Kenji
Cao, Ting
Xu, Xiaodong
Li, Mo
Long-range transport of 2D excitons with acoustic waves
title Long-range transport of 2D excitons with acoustic waves
title_full Long-range transport of 2D excitons with acoustic waves
title_fullStr Long-range transport of 2D excitons with acoustic waves
title_full_unstemmed Long-range transport of 2D excitons with acoustic waves
title_short Long-range transport of 2D excitons with acoustic waves
title_sort long-range transport of 2d excitons with acoustic waves
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8921513/
https://www.ncbi.nlm.nih.gov/pubmed/35289330
http://dx.doi.org/10.1038/s41467-022-29042-9
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