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Real-space nanoimaging of THz polaritons in the topological insulator Bi(2)Se(3)

Plasmon polaritons in topological insulators attract attention from a fundamental perspective and for potential THz photonic applications. Although polaritons have been observed by THz far-field spectroscopy on topological insulator microstructures, real-space imaging of propagating THz polaritons h...

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Autores principales: Chen, Shu, Bylinkin, Andrei, Wang, Zhengtianye, Schnell, Martin, Chandan, Greeshma, Li, Peining, Nikitin, Alexey Y., Law, Stephanie, Hillenbrand, Rainer
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8927118/
https://www.ncbi.nlm.nih.gov/pubmed/35296642
http://dx.doi.org/10.1038/s41467-022-28791-x
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author Chen, Shu
Bylinkin, Andrei
Wang, Zhengtianye
Schnell, Martin
Chandan, Greeshma
Li, Peining
Nikitin, Alexey Y.
Law, Stephanie
Hillenbrand, Rainer
author_facet Chen, Shu
Bylinkin, Andrei
Wang, Zhengtianye
Schnell, Martin
Chandan, Greeshma
Li, Peining
Nikitin, Alexey Y.
Law, Stephanie
Hillenbrand, Rainer
author_sort Chen, Shu
collection PubMed
description Plasmon polaritons in topological insulators attract attention from a fundamental perspective and for potential THz photonic applications. Although polaritons have been observed by THz far-field spectroscopy on topological insulator microstructures, real-space imaging of propagating THz polaritons has been elusive so far. Here, we show spectroscopic THz near-field images of thin Bi(2)Se(3) layers (prototypical topological insulators) revealing polaritons with up to 12 times increased momenta as compared to photons of the same energy and decay times of about 0.48 ps, yet short propagation lengths. From the images we determine and analyze the polariton dispersion, showing that the polaritons can be explained by the coupling of THz radiation to various combinations of Dirac and massive carriers at the Bi(2)Se(3) surfaces, massive bulk carriers and optical phonons. Our work provides critical insights into the nature of THz polaritons in topological insulators and establishes instrumentation and methodology for imaging of THz polaritons.
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spelling pubmed-89271182022-04-01 Real-space nanoimaging of THz polaritons in the topological insulator Bi(2)Se(3) Chen, Shu Bylinkin, Andrei Wang, Zhengtianye Schnell, Martin Chandan, Greeshma Li, Peining Nikitin, Alexey Y. Law, Stephanie Hillenbrand, Rainer Nat Commun Article Plasmon polaritons in topological insulators attract attention from a fundamental perspective and for potential THz photonic applications. Although polaritons have been observed by THz far-field spectroscopy on topological insulator microstructures, real-space imaging of propagating THz polaritons has been elusive so far. Here, we show spectroscopic THz near-field images of thin Bi(2)Se(3) layers (prototypical topological insulators) revealing polaritons with up to 12 times increased momenta as compared to photons of the same energy and decay times of about 0.48 ps, yet short propagation lengths. From the images we determine and analyze the polariton dispersion, showing that the polaritons can be explained by the coupling of THz radiation to various combinations of Dirac and massive carriers at the Bi(2)Se(3) surfaces, massive bulk carriers and optical phonons. Our work provides critical insights into the nature of THz polaritons in topological insulators and establishes instrumentation and methodology for imaging of THz polaritons. Nature Publishing Group UK 2022-03-16 /pmc/articles/PMC8927118/ /pubmed/35296642 http://dx.doi.org/10.1038/s41467-022-28791-x Text en © The Author(s) 2022 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Chen, Shu
Bylinkin, Andrei
Wang, Zhengtianye
Schnell, Martin
Chandan, Greeshma
Li, Peining
Nikitin, Alexey Y.
Law, Stephanie
Hillenbrand, Rainer
Real-space nanoimaging of THz polaritons in the topological insulator Bi(2)Se(3)
title Real-space nanoimaging of THz polaritons in the topological insulator Bi(2)Se(3)
title_full Real-space nanoimaging of THz polaritons in the topological insulator Bi(2)Se(3)
title_fullStr Real-space nanoimaging of THz polaritons in the topological insulator Bi(2)Se(3)
title_full_unstemmed Real-space nanoimaging of THz polaritons in the topological insulator Bi(2)Se(3)
title_short Real-space nanoimaging of THz polaritons in the topological insulator Bi(2)Se(3)
title_sort real-space nanoimaging of thz polaritons in the topological insulator bi(2)se(3)
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8927118/
https://www.ncbi.nlm.nih.gov/pubmed/35296642
http://dx.doi.org/10.1038/s41467-022-28791-x
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