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Enhanced critical current density in K-doped Ba122 polycrystalline bulk superconductors via fast densification

Iron-based superconductors are expected to be used in strong magnet applications owing to their excellent superconducting properties. The process of sintering a mechanically alloyed precursor powder is effective in achieving a high upper critical field and critical current density in BaFe(2)As(2) (B...

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Autores principales: Tokuta, Shinnosuke, Hasegawa, Yuta, Shimada, Yusuke, Yamamoto, Akiyasu
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Elsevier 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8927914/
https://www.ncbi.nlm.nih.gov/pubmed/35310943
http://dx.doi.org/10.1016/j.isci.2022.103992
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author Tokuta, Shinnosuke
Hasegawa, Yuta
Shimada, Yusuke
Yamamoto, Akiyasu
author_facet Tokuta, Shinnosuke
Hasegawa, Yuta
Shimada, Yusuke
Yamamoto, Akiyasu
author_sort Tokuta, Shinnosuke
collection PubMed
description Iron-based superconductors are expected to be used in strong magnet applications owing to their excellent superconducting properties. The process of sintering a mechanically alloyed precursor powder is effective in achieving a high upper critical field and critical current density in BaFe(2)As(2) (Ba122) polycrystalline bulk materials. However, when this process is applied to K-doped Ba122, which shows the highest critical temperature in the Ba122 family, suppressing the vaporization of potassium is challenging. In this study, spark plasma sintering (SPS) method was applied to K-doped Ba122 to achieve fast densification. In contrast to the conventional synthesis method, which requires several tens of hours, optimally K-doped bulks with near theoretical density were obtained after only 5 min of SPS, and the magnetic critical current density reached 10(5) A/cm(2) at 5 K. The demonstrated superconducting properties suggest that this fast densification technique is a useful tool for applying K-doped Ba122 to bulk trapped field magnets.
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spelling pubmed-89279142022-03-18 Enhanced critical current density in K-doped Ba122 polycrystalline bulk superconductors via fast densification Tokuta, Shinnosuke Hasegawa, Yuta Shimada, Yusuke Yamamoto, Akiyasu iScience Article Iron-based superconductors are expected to be used in strong magnet applications owing to their excellent superconducting properties. The process of sintering a mechanically alloyed precursor powder is effective in achieving a high upper critical field and critical current density in BaFe(2)As(2) (Ba122) polycrystalline bulk materials. However, when this process is applied to K-doped Ba122, which shows the highest critical temperature in the Ba122 family, suppressing the vaporization of potassium is challenging. In this study, spark plasma sintering (SPS) method was applied to K-doped Ba122 to achieve fast densification. In contrast to the conventional synthesis method, which requires several tens of hours, optimally K-doped bulks with near theoretical density were obtained after only 5 min of SPS, and the magnetic critical current density reached 10(5) A/cm(2) at 5 K. The demonstrated superconducting properties suggest that this fast densification technique is a useful tool for applying K-doped Ba122 to bulk trapped field magnets. Elsevier 2022-02-26 /pmc/articles/PMC8927914/ /pubmed/35310943 http://dx.doi.org/10.1016/j.isci.2022.103992 Text en © 2022 The Authors https://creativecommons.org/licenses/by-nc-nd/4.0/This is an open access article under the CC BY-NC-ND license (http://creativecommons.org/licenses/by-nc-nd/4.0/).
spellingShingle Article
Tokuta, Shinnosuke
Hasegawa, Yuta
Shimada, Yusuke
Yamamoto, Akiyasu
Enhanced critical current density in K-doped Ba122 polycrystalline bulk superconductors via fast densification
title Enhanced critical current density in K-doped Ba122 polycrystalline bulk superconductors via fast densification
title_full Enhanced critical current density in K-doped Ba122 polycrystalline bulk superconductors via fast densification
title_fullStr Enhanced critical current density in K-doped Ba122 polycrystalline bulk superconductors via fast densification
title_full_unstemmed Enhanced critical current density in K-doped Ba122 polycrystalline bulk superconductors via fast densification
title_short Enhanced critical current density in K-doped Ba122 polycrystalline bulk superconductors via fast densification
title_sort enhanced critical current density in k-doped ba122 polycrystalline bulk superconductors via fast densification
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8927914/
https://www.ncbi.nlm.nih.gov/pubmed/35310943
http://dx.doi.org/10.1016/j.isci.2022.103992
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