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Planar Chirality and Optical Spin–Orbit Coupling for Chiral Fabry–Perot Cavities

[Image: see text] We design, in a most simple way, Fabry–Perot cavities with longitudinal chiral modes by sandwiching between two smooth metallic silver mirrors a layer of polystyrene made planar chiral by torsional shear stress. We demonstrate that the helicity-preserving features of our cavities s...

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Detalles Bibliográficos
Autores principales: Gautier, Jérôme, Li, Minghao, Ebbesen, Thomas W., Genet, Cyriaque
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2022
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8931756/
https://www.ncbi.nlm.nih.gov/pubmed/35308406
http://dx.doi.org/10.1021/acsphotonics.1c00780
Descripción
Sumario:[Image: see text] We design, in a most simple way, Fabry–Perot cavities with longitudinal chiral modes by sandwiching between two smooth metallic silver mirrors a layer of polystyrene made planar chiral by torsional shear stress. We demonstrate that the helicity-preserving features of our cavities stem from a spin–orbit coupling mechanism seeded inside the cavities by the specific chiroptical features of planar chirality. Planar chirality gives rise to an extrinsic source of three-dimensional chirality under oblique illumination that endows the cavities with enantiomorphic signatures measured experimentally and simulated with excellent agreement. The simplicity of our scheme is particularly promising in the context of chiral cavity QED and polaritonic asymmetric chemistry.