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Planar Chirality and Optical Spin–Orbit Coupling for Chiral Fabry–Perot Cavities
[Image: see text] We design, in a most simple way, Fabry–Perot cavities with longitudinal chiral modes by sandwiching between two smooth metallic silver mirrors a layer of polystyrene made planar chiral by torsional shear stress. We demonstrate that the helicity-preserving features of our cavities s...
Autores principales: | , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Chemical Society
2022
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Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8931756/ https://www.ncbi.nlm.nih.gov/pubmed/35308406 http://dx.doi.org/10.1021/acsphotonics.1c00780 |
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author | Gautier, Jérôme Li, Minghao Ebbesen, Thomas W. Genet, Cyriaque |
author_facet | Gautier, Jérôme Li, Minghao Ebbesen, Thomas W. Genet, Cyriaque |
author_sort | Gautier, Jérôme |
collection | PubMed |
description | [Image: see text] We design, in a most simple way, Fabry–Perot cavities with longitudinal chiral modes by sandwiching between two smooth metallic silver mirrors a layer of polystyrene made planar chiral by torsional shear stress. We demonstrate that the helicity-preserving features of our cavities stem from a spin–orbit coupling mechanism seeded inside the cavities by the specific chiroptical features of planar chirality. Planar chirality gives rise to an extrinsic source of three-dimensional chirality under oblique illumination that endows the cavities with enantiomorphic signatures measured experimentally and simulated with excellent agreement. The simplicity of our scheme is particularly promising in the context of chiral cavity QED and polaritonic asymmetric chemistry. |
format | Online Article Text |
id | pubmed-8931756 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2022 |
publisher | American Chemical Society |
record_format | MEDLINE/PubMed |
spelling | pubmed-89317562022-03-18 Planar Chirality and Optical Spin–Orbit Coupling for Chiral Fabry–Perot Cavities Gautier, Jérôme Li, Minghao Ebbesen, Thomas W. Genet, Cyriaque ACS Photonics [Image: see text] We design, in a most simple way, Fabry–Perot cavities with longitudinal chiral modes by sandwiching between two smooth metallic silver mirrors a layer of polystyrene made planar chiral by torsional shear stress. We demonstrate that the helicity-preserving features of our cavities stem from a spin–orbit coupling mechanism seeded inside the cavities by the specific chiroptical features of planar chirality. Planar chirality gives rise to an extrinsic source of three-dimensional chirality under oblique illumination that endows the cavities with enantiomorphic signatures measured experimentally and simulated with excellent agreement. The simplicity of our scheme is particularly promising in the context of chiral cavity QED and polaritonic asymmetric chemistry. American Chemical Society 2022-02-14 2022-03-16 /pmc/articles/PMC8931756/ /pubmed/35308406 http://dx.doi.org/10.1021/acsphotonics.1c00780 Text en © 2022 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by-nc-nd/4.0/Permits non-commercial access and re-use, provided that author attribution and integrity are maintained; but does not permit creation of adaptations or other derivative works (https://creativecommons.org/licenses/by-nc-nd/4.0/). |
spellingShingle | Gautier, Jérôme Li, Minghao Ebbesen, Thomas W. Genet, Cyriaque Planar Chirality and Optical Spin–Orbit Coupling for Chiral Fabry–Perot Cavities |
title | Planar Chirality and Optical Spin–Orbit
Coupling for Chiral Fabry–Perot Cavities |
title_full | Planar Chirality and Optical Spin–Orbit
Coupling for Chiral Fabry–Perot Cavities |
title_fullStr | Planar Chirality and Optical Spin–Orbit
Coupling for Chiral Fabry–Perot Cavities |
title_full_unstemmed | Planar Chirality and Optical Spin–Orbit
Coupling for Chiral Fabry–Perot Cavities |
title_short | Planar Chirality and Optical Spin–Orbit
Coupling for Chiral Fabry–Perot Cavities |
title_sort | planar chirality and optical spin–orbit
coupling for chiral fabry–perot cavities |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8931756/ https://www.ncbi.nlm.nih.gov/pubmed/35308406 http://dx.doi.org/10.1021/acsphotonics.1c00780 |
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