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Planar Chirality and Optical Spin–Orbit Coupling for Chiral Fabry–Perot Cavities

[Image: see text] We design, in a most simple way, Fabry–Perot cavities with longitudinal chiral modes by sandwiching between two smooth metallic silver mirrors a layer of polystyrene made planar chiral by torsional shear stress. We demonstrate that the helicity-preserving features of our cavities s...

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Autores principales: Gautier, Jérôme, Li, Minghao, Ebbesen, Thomas W., Genet, Cyriaque
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2022
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8931756/
https://www.ncbi.nlm.nih.gov/pubmed/35308406
http://dx.doi.org/10.1021/acsphotonics.1c00780
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author Gautier, Jérôme
Li, Minghao
Ebbesen, Thomas W.
Genet, Cyriaque
author_facet Gautier, Jérôme
Li, Minghao
Ebbesen, Thomas W.
Genet, Cyriaque
author_sort Gautier, Jérôme
collection PubMed
description [Image: see text] We design, in a most simple way, Fabry–Perot cavities with longitudinal chiral modes by sandwiching between two smooth metallic silver mirrors a layer of polystyrene made planar chiral by torsional shear stress. We demonstrate that the helicity-preserving features of our cavities stem from a spin–orbit coupling mechanism seeded inside the cavities by the specific chiroptical features of planar chirality. Planar chirality gives rise to an extrinsic source of three-dimensional chirality under oblique illumination that endows the cavities with enantiomorphic signatures measured experimentally and simulated with excellent agreement. The simplicity of our scheme is particularly promising in the context of chiral cavity QED and polaritonic asymmetric chemistry.
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spelling pubmed-89317562022-03-18 Planar Chirality and Optical Spin–Orbit Coupling for Chiral Fabry–Perot Cavities Gautier, Jérôme Li, Minghao Ebbesen, Thomas W. Genet, Cyriaque ACS Photonics [Image: see text] We design, in a most simple way, Fabry–Perot cavities with longitudinal chiral modes by sandwiching between two smooth metallic silver mirrors a layer of polystyrene made planar chiral by torsional shear stress. We demonstrate that the helicity-preserving features of our cavities stem from a spin–orbit coupling mechanism seeded inside the cavities by the specific chiroptical features of planar chirality. Planar chirality gives rise to an extrinsic source of three-dimensional chirality under oblique illumination that endows the cavities with enantiomorphic signatures measured experimentally and simulated with excellent agreement. The simplicity of our scheme is particularly promising in the context of chiral cavity QED and polaritonic asymmetric chemistry. American Chemical Society 2022-02-14 2022-03-16 /pmc/articles/PMC8931756/ /pubmed/35308406 http://dx.doi.org/10.1021/acsphotonics.1c00780 Text en © 2022 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by-nc-nd/4.0/Permits non-commercial access and re-use, provided that author attribution and integrity are maintained; but does not permit creation of adaptations or other derivative works (https://creativecommons.org/licenses/by-nc-nd/4.0/).
spellingShingle Gautier, Jérôme
Li, Minghao
Ebbesen, Thomas W.
Genet, Cyriaque
Planar Chirality and Optical Spin–Orbit Coupling for Chiral Fabry–Perot Cavities
title Planar Chirality and Optical Spin–Orbit Coupling for Chiral Fabry–Perot Cavities
title_full Planar Chirality and Optical Spin–Orbit Coupling for Chiral Fabry–Perot Cavities
title_fullStr Planar Chirality and Optical Spin–Orbit Coupling for Chiral Fabry–Perot Cavities
title_full_unstemmed Planar Chirality and Optical Spin–Orbit Coupling for Chiral Fabry–Perot Cavities
title_short Planar Chirality and Optical Spin–Orbit Coupling for Chiral Fabry–Perot Cavities
title_sort planar chirality and optical spin–orbit coupling for chiral fabry–perot cavities
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8931756/
https://www.ncbi.nlm.nih.gov/pubmed/35308406
http://dx.doi.org/10.1021/acsphotonics.1c00780
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