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A kiloelectron-volt ultrafast electron micro-diffraction apparatus using low emittance semiconductor photocathodes

We report the design and performance of a time-resolved electron diffraction apparatus capable of producing intense bunches with simultaneously single digit micrometer probe size, long coherence length, and 200 fs rms time resolution. We measure the 5d (peak) beam brightness at the sample location i...

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Detalles Bibliográficos
Autores principales: Li, W. H., Duncan, C. J. R., Andorf, M. B., Bartnik, A. C., Bianco, E., Cultrera, L., Galdi, A., Gordon, M., Kaemingk, M., Pennington, C. A., Kourkoutis, L. F., Bazarov, I. V., Maxson, J. M.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Crystallographic Association 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8934190/
https://www.ncbi.nlm.nih.gov/pubmed/35350376
http://dx.doi.org/10.1063/4.0000138
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author Li, W. H.
Duncan, C. J. R.
Andorf, M. B.
Bartnik, A. C.
Bianco, E.
Cultrera, L.
Galdi, A.
Gordon, M.
Kaemingk, M.
Pennington, C. A.
Kourkoutis, L. F.
Bazarov, I. V.
Maxson, J. M.
author_facet Li, W. H.
Duncan, C. J. R.
Andorf, M. B.
Bartnik, A. C.
Bianco, E.
Cultrera, L.
Galdi, A.
Gordon, M.
Kaemingk, M.
Pennington, C. A.
Kourkoutis, L. F.
Bazarov, I. V.
Maxson, J. M.
author_sort Li, W. H.
collection PubMed
description We report the design and performance of a time-resolved electron diffraction apparatus capable of producing intense bunches with simultaneously single digit micrometer probe size, long coherence length, and 200 fs rms time resolution. We measure the 5d (peak) beam brightness at the sample location in micro-diffraction mode to be [Formula: see text]. To generate high brightness electron bunches, the system employs high efficiency, low emittance semiconductor photocathodes driven with a wavelength near the photoemission threshold at a repetition rate up to 250 kHz. We characterize spatial, temporal, and reciprocal space resolution of the apparatus. We perform proof-of-principle measurements of ultrafast heating in single crystal Au samples and compare experimental results with simulations that account for the effects of multiple scattering.
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spelling pubmed-89341902022-03-28 A kiloelectron-volt ultrafast electron micro-diffraction apparatus using low emittance semiconductor photocathodes Li, W. H. Duncan, C. J. R. Andorf, M. B. Bartnik, A. C. Bianco, E. Cultrera, L. Galdi, A. Gordon, M. Kaemingk, M. Pennington, C. A. Kourkoutis, L. F. Bazarov, I. V. Maxson, J. M. Struct Dyn ARTICLES We report the design and performance of a time-resolved electron diffraction apparatus capable of producing intense bunches with simultaneously single digit micrometer probe size, long coherence length, and 200 fs rms time resolution. We measure the 5d (peak) beam brightness at the sample location in micro-diffraction mode to be [Formula: see text]. To generate high brightness electron bunches, the system employs high efficiency, low emittance semiconductor photocathodes driven with a wavelength near the photoemission threshold at a repetition rate up to 250 kHz. We characterize spatial, temporal, and reciprocal space resolution of the apparatus. We perform proof-of-principle measurements of ultrafast heating in single crystal Au samples and compare experimental results with simulations that account for the effects of multiple scattering. American Crystallographic Association 2022-03-18 /pmc/articles/PMC8934190/ /pubmed/35350376 http://dx.doi.org/10.1063/4.0000138 Text en © 2022 Author(s). https://creativecommons.org/licenses/by/4.0/All article content, except where otherwise noted, is licensed under a Creative Commons Attribution (CC BY) license (http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) ).
spellingShingle ARTICLES
Li, W. H.
Duncan, C. J. R.
Andorf, M. B.
Bartnik, A. C.
Bianco, E.
Cultrera, L.
Galdi, A.
Gordon, M.
Kaemingk, M.
Pennington, C. A.
Kourkoutis, L. F.
Bazarov, I. V.
Maxson, J. M.
A kiloelectron-volt ultrafast electron micro-diffraction apparatus using low emittance semiconductor photocathodes
title A kiloelectron-volt ultrafast electron micro-diffraction apparatus using low emittance semiconductor photocathodes
title_full A kiloelectron-volt ultrafast electron micro-diffraction apparatus using low emittance semiconductor photocathodes
title_fullStr A kiloelectron-volt ultrafast electron micro-diffraction apparatus using low emittance semiconductor photocathodes
title_full_unstemmed A kiloelectron-volt ultrafast electron micro-diffraction apparatus using low emittance semiconductor photocathodes
title_short A kiloelectron-volt ultrafast electron micro-diffraction apparatus using low emittance semiconductor photocathodes
title_sort kiloelectron-volt ultrafast electron micro-diffraction apparatus using low emittance semiconductor photocathodes
topic ARTICLES
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8934190/
https://www.ncbi.nlm.nih.gov/pubmed/35350376
http://dx.doi.org/10.1063/4.0000138
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