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Simulating the Feasibility of Using Liquid Micro-Jets for Determining Electron–Liquid Scattering Cross-Sections

The extraction of electron–liquid phase cross-sections (surface and bulk) is proposed through the measurement of (differential) energy loss spectra for electrons scattered from a liquid micro-jet. The signature physical elements of the scattering processes on the energy loss spectra are highlighted...

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Detalles Bibliográficos
Autores principales: Muccignat, Dale L., Stokes, Peter W., Cocks, Daniel G., Gascooke, Jason R., Jones, Darryl B., Brunger, Michael J., White, Ronald D.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8954820/
https://www.ncbi.nlm.nih.gov/pubmed/35328775
http://dx.doi.org/10.3390/ijms23063354
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author Muccignat, Dale L.
Stokes, Peter W.
Cocks, Daniel G.
Gascooke, Jason R.
Jones, Darryl B.
Brunger, Michael J.
White, Ronald D.
author_facet Muccignat, Dale L.
Stokes, Peter W.
Cocks, Daniel G.
Gascooke, Jason R.
Jones, Darryl B.
Brunger, Michael J.
White, Ronald D.
author_sort Muccignat, Dale L.
collection PubMed
description The extraction of electron–liquid phase cross-sections (surface and bulk) is proposed through the measurement of (differential) energy loss spectra for electrons scattered from a liquid micro-jet. The signature physical elements of the scattering processes on the energy loss spectra are highlighted using a Monte Carlo simulation technique, originally developed for simulating electron transport in liquids. Machine learning techniques are applied to the simulated electron energy loss spectra, to invert the data and extract the cross-sections. The extraction of the elastic cross-section for neon was determined within 9% accuracy over the energy range 1–100 eV. The extension toward the simultaneous determination of elastic and ionisation cross-sections resulted in a decrease in accuracy, now to within 18% accuracy for elastic scattering and 1% for ionisation. Additional methods are explored to enhance the accuracy of the simultaneous extraction of liquid phase cross-sections.
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spelling pubmed-89548202022-03-26 Simulating the Feasibility of Using Liquid Micro-Jets for Determining Electron–Liquid Scattering Cross-Sections Muccignat, Dale L. Stokes, Peter W. Cocks, Daniel G. Gascooke, Jason R. Jones, Darryl B. Brunger, Michael J. White, Ronald D. Int J Mol Sci Article The extraction of electron–liquid phase cross-sections (surface and bulk) is proposed through the measurement of (differential) energy loss spectra for electrons scattered from a liquid micro-jet. The signature physical elements of the scattering processes on the energy loss spectra are highlighted using a Monte Carlo simulation technique, originally developed for simulating electron transport in liquids. Machine learning techniques are applied to the simulated electron energy loss spectra, to invert the data and extract the cross-sections. The extraction of the elastic cross-section for neon was determined within 9% accuracy over the energy range 1–100 eV. The extension toward the simultaneous determination of elastic and ionisation cross-sections resulted in a decrease in accuracy, now to within 18% accuracy for elastic scattering and 1% for ionisation. Additional methods are explored to enhance the accuracy of the simultaneous extraction of liquid phase cross-sections. MDPI 2022-03-20 /pmc/articles/PMC8954820/ /pubmed/35328775 http://dx.doi.org/10.3390/ijms23063354 Text en © 2022 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Muccignat, Dale L.
Stokes, Peter W.
Cocks, Daniel G.
Gascooke, Jason R.
Jones, Darryl B.
Brunger, Michael J.
White, Ronald D.
Simulating the Feasibility of Using Liquid Micro-Jets for Determining Electron–Liquid Scattering Cross-Sections
title Simulating the Feasibility of Using Liquid Micro-Jets for Determining Electron–Liquid Scattering Cross-Sections
title_full Simulating the Feasibility of Using Liquid Micro-Jets for Determining Electron–Liquid Scattering Cross-Sections
title_fullStr Simulating the Feasibility of Using Liquid Micro-Jets for Determining Electron–Liquid Scattering Cross-Sections
title_full_unstemmed Simulating the Feasibility of Using Liquid Micro-Jets for Determining Electron–Liquid Scattering Cross-Sections
title_short Simulating the Feasibility of Using Liquid Micro-Jets for Determining Electron–Liquid Scattering Cross-Sections
title_sort simulating the feasibility of using liquid micro-jets for determining electron–liquid scattering cross-sections
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8954820/
https://www.ncbi.nlm.nih.gov/pubmed/35328775
http://dx.doi.org/10.3390/ijms23063354
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