Cargando…
Exact closure and solution for spatial correlations in single-file diffusion
In single-file transport particles diffuse in narrow channels while not overtaking each other. it is a fundamental model for the tracer subdiffusion observed in confined systems, such as zeolites or carbon nanotubes. This anomalous behavior originates from strong bath-tracer correlations in one dime...
Autores principales: | , , , , |
---|---|
Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Association for the Advancement of Science
2022
|
Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8956262/ https://www.ncbi.nlm.nih.gov/pubmed/35333581 http://dx.doi.org/10.1126/sciadv.abm5043 |
_version_ | 1784676527315615744 |
---|---|
author | Grabsch, Aurélien Poncet, Alexis Rizkallah, Pierre Illien, Pierre Bénichou, Olivier |
author_facet | Grabsch, Aurélien Poncet, Alexis Rizkallah, Pierre Illien, Pierre Bénichou, Olivier |
author_sort | Grabsch, Aurélien |
collection | PubMed |
description | In single-file transport particles diffuse in narrow channels while not overtaking each other. it is a fundamental model for the tracer subdiffusion observed in confined systems, such as zeolites or carbon nanotubes. This anomalous behavior originates from strong bath-tracer correlations in one dimension. Despite extensive effort, these remained elusive, because they involve an infinite hierarchy of equations. For the symmetric exclusion process, a paradigmatic model of single-file diffusion, we break the hierarchy to unveil and solve a closed exact equation satisfied by these correlations. Beyond quantifying the correlations, the role of this key equation as a tool for interacting particle systems is further demonstrated by its application to out-of-equilibrium situations, other observables, and other representative single-file systems. |
format | Online Article Text |
id | pubmed-8956262 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2022 |
publisher | American Association for the Advancement of Science |
record_format | MEDLINE/PubMed |
spelling | pubmed-89562622022-04-04 Exact closure and solution for spatial correlations in single-file diffusion Grabsch, Aurélien Poncet, Alexis Rizkallah, Pierre Illien, Pierre Bénichou, Olivier Sci Adv Physical and Materials Sciences In single-file transport particles diffuse in narrow channels while not overtaking each other. it is a fundamental model for the tracer subdiffusion observed in confined systems, such as zeolites or carbon nanotubes. This anomalous behavior originates from strong bath-tracer correlations in one dimension. Despite extensive effort, these remained elusive, because they involve an infinite hierarchy of equations. For the symmetric exclusion process, a paradigmatic model of single-file diffusion, we break the hierarchy to unveil and solve a closed exact equation satisfied by these correlations. Beyond quantifying the correlations, the role of this key equation as a tool for interacting particle systems is further demonstrated by its application to out-of-equilibrium situations, other observables, and other representative single-file systems. American Association for the Advancement of Science 2022-03-25 /pmc/articles/PMC8956262/ /pubmed/35333581 http://dx.doi.org/10.1126/sciadv.abm5043 Text en Copyright © 2022 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution NonCommercial License 4.0 (CC BY-NC). https://creativecommons.org/licenses/by-nc/4.0/This is an open-access article distributed under the terms of the Creative Commons Attribution-NonCommercial license (https://creativecommons.org/licenses/by-nc/4.0/) , which permits use, distribution, and reproduction in any medium, so long as the resultant use is not for commercial advantage and provided the original work is properly cited. |
spellingShingle | Physical and Materials Sciences Grabsch, Aurélien Poncet, Alexis Rizkallah, Pierre Illien, Pierre Bénichou, Olivier Exact closure and solution for spatial correlations in single-file diffusion |
title | Exact closure and solution for spatial correlations in single-file diffusion |
title_full | Exact closure and solution for spatial correlations in single-file diffusion |
title_fullStr | Exact closure and solution for spatial correlations in single-file diffusion |
title_full_unstemmed | Exact closure and solution for spatial correlations in single-file diffusion |
title_short | Exact closure and solution for spatial correlations in single-file diffusion |
title_sort | exact closure and solution for spatial correlations in single-file diffusion |
topic | Physical and Materials Sciences |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8956262/ https://www.ncbi.nlm.nih.gov/pubmed/35333581 http://dx.doi.org/10.1126/sciadv.abm5043 |
work_keys_str_mv | AT grabschaurelien exactclosureandsolutionforspatialcorrelationsinsinglefilediffusion AT poncetalexis exactclosureandsolutionforspatialcorrelationsinsinglefilediffusion AT rizkallahpierre exactclosureandsolutionforspatialcorrelationsinsinglefilediffusion AT illienpierre exactclosureandsolutionforspatialcorrelationsinsinglefilediffusion AT benichouolivier exactclosureandsolutionforspatialcorrelationsinsinglefilediffusion |