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Exact closure and solution for spatial correlations in single-file diffusion

In single-file transport particles diffuse in narrow channels while not overtaking each other. it is a fundamental model for the tracer subdiffusion observed in confined systems, such as zeolites or carbon nanotubes. This anomalous behavior originates from strong bath-tracer correlations in one dime...

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Autores principales: Grabsch, Aurélien, Poncet, Alexis, Rizkallah, Pierre, Illien, Pierre, Bénichou, Olivier
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Association for the Advancement of Science 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8956262/
https://www.ncbi.nlm.nih.gov/pubmed/35333581
http://dx.doi.org/10.1126/sciadv.abm5043
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author Grabsch, Aurélien
Poncet, Alexis
Rizkallah, Pierre
Illien, Pierre
Bénichou, Olivier
author_facet Grabsch, Aurélien
Poncet, Alexis
Rizkallah, Pierre
Illien, Pierre
Bénichou, Olivier
author_sort Grabsch, Aurélien
collection PubMed
description In single-file transport particles diffuse in narrow channels while not overtaking each other. it is a fundamental model for the tracer subdiffusion observed in confined systems, such as zeolites or carbon nanotubes. This anomalous behavior originates from strong bath-tracer correlations in one dimension. Despite extensive effort, these remained elusive, because they involve an infinite hierarchy of equations. For the symmetric exclusion process, a paradigmatic model of single-file diffusion, we break the hierarchy to unveil and solve a closed exact equation satisfied by these correlations. Beyond quantifying the correlations, the role of this key equation as a tool for interacting particle systems is further demonstrated by its application to out-of-equilibrium situations, other observables, and other representative single-file systems.
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spelling pubmed-89562622022-04-04 Exact closure and solution for spatial correlations in single-file diffusion Grabsch, Aurélien Poncet, Alexis Rizkallah, Pierre Illien, Pierre Bénichou, Olivier Sci Adv Physical and Materials Sciences In single-file transport particles diffuse in narrow channels while not overtaking each other. it is a fundamental model for the tracer subdiffusion observed in confined systems, such as zeolites or carbon nanotubes. This anomalous behavior originates from strong bath-tracer correlations in one dimension. Despite extensive effort, these remained elusive, because they involve an infinite hierarchy of equations. For the symmetric exclusion process, a paradigmatic model of single-file diffusion, we break the hierarchy to unveil and solve a closed exact equation satisfied by these correlations. Beyond quantifying the correlations, the role of this key equation as a tool for interacting particle systems is further demonstrated by its application to out-of-equilibrium situations, other observables, and other representative single-file systems. American Association for the Advancement of Science 2022-03-25 /pmc/articles/PMC8956262/ /pubmed/35333581 http://dx.doi.org/10.1126/sciadv.abm5043 Text en Copyright © 2022 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution NonCommercial License 4.0 (CC BY-NC). https://creativecommons.org/licenses/by-nc/4.0/This is an open-access article distributed under the terms of the Creative Commons Attribution-NonCommercial license (https://creativecommons.org/licenses/by-nc/4.0/) , which permits use, distribution, and reproduction in any medium, so long as the resultant use is not for commercial advantage and provided the original work is properly cited.
spellingShingle Physical and Materials Sciences
Grabsch, Aurélien
Poncet, Alexis
Rizkallah, Pierre
Illien, Pierre
Bénichou, Olivier
Exact closure and solution for spatial correlations in single-file diffusion
title Exact closure and solution for spatial correlations in single-file diffusion
title_full Exact closure and solution for spatial correlations in single-file diffusion
title_fullStr Exact closure and solution for spatial correlations in single-file diffusion
title_full_unstemmed Exact closure and solution for spatial correlations in single-file diffusion
title_short Exact closure and solution for spatial correlations in single-file diffusion
title_sort exact closure and solution for spatial correlations in single-file diffusion
topic Physical and Materials Sciences
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8956262/
https://www.ncbi.nlm.nih.gov/pubmed/35333581
http://dx.doi.org/10.1126/sciadv.abm5043
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