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Wafer-scale epitaxial modulation of quantum dot density

Precise control of the properties of semiconductor quantum dots (QDs) is vital for creating novel devices for quantum photonics and advanced opto-electronics. Suitable low QD-densities for single QD devices and experiments are challenging to control during epitaxy and are typically found only in lim...

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Autores principales: Bart, N., Dangel, C., Zajac, P., Spitzer, N., Ritzmann, J., Schmidt, M., Babin, H. G., Schott, R., Valentin, S. R., Scholz, S., Wang, Y., Uppu, R., Najer, D., Löbl, M. C., Tomm, N., Javadi, A., Antoniadis, N. O., Midolo, L., Müller, K., Warburton, R. J., Lodahl, P., Wieck, A. D., Finley, J. J., Ludwig, A.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8960873/
https://www.ncbi.nlm.nih.gov/pubmed/35347120
http://dx.doi.org/10.1038/s41467-022-29116-8
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author Bart, N.
Dangel, C.
Zajac, P.
Spitzer, N.
Ritzmann, J.
Schmidt, M.
Babin, H. G.
Schott, R.
Valentin, S. R.
Scholz, S.
Wang, Y.
Uppu, R.
Najer, D.
Löbl, M. C.
Tomm, N.
Javadi, A.
Antoniadis, N. O.
Midolo, L.
Müller, K.
Warburton, R. J.
Lodahl, P.
Wieck, A. D.
Finley, J. J.
Ludwig, A.
author_facet Bart, N.
Dangel, C.
Zajac, P.
Spitzer, N.
Ritzmann, J.
Schmidt, M.
Babin, H. G.
Schott, R.
Valentin, S. R.
Scholz, S.
Wang, Y.
Uppu, R.
Najer, D.
Löbl, M. C.
Tomm, N.
Javadi, A.
Antoniadis, N. O.
Midolo, L.
Müller, K.
Warburton, R. J.
Lodahl, P.
Wieck, A. D.
Finley, J. J.
Ludwig, A.
author_sort Bart, N.
collection PubMed
description Precise control of the properties of semiconductor quantum dots (QDs) is vital for creating novel devices for quantum photonics and advanced opto-electronics. Suitable low QD-densities for single QD devices and experiments are challenging to control during epitaxy and are typically found only in limited regions of the wafer. Here, we demonstrate how conventional molecular beam epitaxy (MBE) can be used to modulate the density of optically active QDs in one- and two- dimensional patterns, while still retaining excellent quality. We find that material thickness gradients during layer-by-layer growth result in surface roughness modulations across the whole wafer. Growth on such templates strongly influences the QD nucleation probability. We obtain density modulations between 1 and 10 QDs/µm(2) and periods ranging from several millimeters down to at least a few hundred microns. This method is universal and expected to be applicable to a wide variety of different semiconductor material systems. We apply the method to enable growth of ultra-low noise QDs across an entire 3-inch semiconductor wafer.
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spelling pubmed-89608732022-04-20 Wafer-scale epitaxial modulation of quantum dot density Bart, N. Dangel, C. Zajac, P. Spitzer, N. Ritzmann, J. Schmidt, M. Babin, H. G. Schott, R. Valentin, S. R. Scholz, S. Wang, Y. Uppu, R. Najer, D. Löbl, M. C. Tomm, N. Javadi, A. Antoniadis, N. O. Midolo, L. Müller, K. Warburton, R. J. Lodahl, P. Wieck, A. D. Finley, J. J. Ludwig, A. Nat Commun Article Precise control of the properties of semiconductor quantum dots (QDs) is vital for creating novel devices for quantum photonics and advanced opto-electronics. Suitable low QD-densities for single QD devices and experiments are challenging to control during epitaxy and are typically found only in limited regions of the wafer. Here, we demonstrate how conventional molecular beam epitaxy (MBE) can be used to modulate the density of optically active QDs in one- and two- dimensional patterns, while still retaining excellent quality. We find that material thickness gradients during layer-by-layer growth result in surface roughness modulations across the whole wafer. Growth on such templates strongly influences the QD nucleation probability. We obtain density modulations between 1 and 10 QDs/µm(2) and periods ranging from several millimeters down to at least a few hundred microns. This method is universal and expected to be applicable to a wide variety of different semiconductor material systems. We apply the method to enable growth of ultra-low noise QDs across an entire 3-inch semiconductor wafer. Nature Publishing Group UK 2022-03-28 /pmc/articles/PMC8960873/ /pubmed/35347120 http://dx.doi.org/10.1038/s41467-022-29116-8 Text en © The Author(s) 2022 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Bart, N.
Dangel, C.
Zajac, P.
Spitzer, N.
Ritzmann, J.
Schmidt, M.
Babin, H. G.
Schott, R.
Valentin, S. R.
Scholz, S.
Wang, Y.
Uppu, R.
Najer, D.
Löbl, M. C.
Tomm, N.
Javadi, A.
Antoniadis, N. O.
Midolo, L.
Müller, K.
Warburton, R. J.
Lodahl, P.
Wieck, A. D.
Finley, J. J.
Ludwig, A.
Wafer-scale epitaxial modulation of quantum dot density
title Wafer-scale epitaxial modulation of quantum dot density
title_full Wafer-scale epitaxial modulation of quantum dot density
title_fullStr Wafer-scale epitaxial modulation of quantum dot density
title_full_unstemmed Wafer-scale epitaxial modulation of quantum dot density
title_short Wafer-scale epitaxial modulation of quantum dot density
title_sort wafer-scale epitaxial modulation of quantum dot density
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8960873/
https://www.ncbi.nlm.nih.gov/pubmed/35347120
http://dx.doi.org/10.1038/s41467-022-29116-8
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