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Quantum–classical simulations of rhodopsin reveal excited-state-population splitting and its effects on quantum efficiency
The activation of rhodopsin, the light-sensitive G-protein coupled receptor responsible for dim-light vision in vertebrates, is driven by an ultrafast excited-state double-bond isomerization with a quantum efficiency of almost 70%. The origin of such light sensitivity is not understood and a key que...
Autores principales: | Yang, Xuchun, Manathunga, Madushanka, Gozem, Samer, Léonard, Jérémie, Andruniów, Tadeusz, Olivucci, Massimo |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
2022
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8983576/ https://www.ncbi.nlm.nih.gov/pubmed/35241801 http://dx.doi.org/10.1038/s41557-022-00892-6 |
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