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Application of an Event-Based Camera for Real-Time Velocity Resolved Kinetics

[Image: see text] We describe here the application of an inexpensive event-based/neuromorphic camera in an ion imaging experiment operated at 1 kHz detection rate to study real-time velocity-resolved kinetics of thermal desorption. Such measurements involve a single gas pulse to initiate a time-depe...

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Autores principales: Golibrzuch, Kai, Schwabe, Sven, Zhong, Tianli, Papendorf, Kim, Wodtke, Alec M.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2022
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8996233/
https://www.ncbi.nlm.nih.gov/pubmed/35319892
http://dx.doi.org/10.1021/acs.jpca.2c00806
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author Golibrzuch, Kai
Schwabe, Sven
Zhong, Tianli
Papendorf, Kim
Wodtke, Alec M.
author_facet Golibrzuch, Kai
Schwabe, Sven
Zhong, Tianli
Papendorf, Kim
Wodtke, Alec M.
author_sort Golibrzuch, Kai
collection PubMed
description [Image: see text] We describe here the application of an inexpensive event-based/neuromorphic camera in an ion imaging experiment operated at 1 kHz detection rate to study real-time velocity-resolved kinetics of thermal desorption. Such measurements involve a single gas pulse to initiate a time-dependent desorption process and a high repetition rate laser, where each pulse of the laser is used to produce an ion image. The sequence of ion images allows the time dependence of the desorption flux to be followed in real time. In previous work where a conventional framing camera was used, the large number of megapixel-sized images required data transfer and storage rates of up to 16 GB/s. This necessitated a large onboard memory that was quickly filled and limited continuous measurement to only a few seconds. Read-out of the memory became the bottleneck to the rate of data acquisition. We show here that since most pixels in each ion image contain no data, the data rate can be dramatically reduced by using an event-based/neuromorphic camera. The data stream is thus reduced to the intensity and location information on the pixels that are lit up by each ion event together with a time-stamp indicating the arrival time of an ion at the detector. This dramatically increases the duty cycle of the method and provides insights for the execution of other high rep-rate ion imaging experiments.
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spelling pubmed-89962332022-04-12 Application of an Event-Based Camera for Real-Time Velocity Resolved Kinetics Golibrzuch, Kai Schwabe, Sven Zhong, Tianli Papendorf, Kim Wodtke, Alec M. J Phys Chem A [Image: see text] We describe here the application of an inexpensive event-based/neuromorphic camera in an ion imaging experiment operated at 1 kHz detection rate to study real-time velocity-resolved kinetics of thermal desorption. Such measurements involve a single gas pulse to initiate a time-dependent desorption process and a high repetition rate laser, where each pulse of the laser is used to produce an ion image. The sequence of ion images allows the time dependence of the desorption flux to be followed in real time. In previous work where a conventional framing camera was used, the large number of megapixel-sized images required data transfer and storage rates of up to 16 GB/s. This necessitated a large onboard memory that was quickly filled and limited continuous measurement to only a few seconds. Read-out of the memory became the bottleneck to the rate of data acquisition. We show here that since most pixels in each ion image contain no data, the data rate can be dramatically reduced by using an event-based/neuromorphic camera. The data stream is thus reduced to the intensity and location information on the pixels that are lit up by each ion event together with a time-stamp indicating the arrival time of an ion at the detector. This dramatically increases the duty cycle of the method and provides insights for the execution of other high rep-rate ion imaging experiments. American Chemical Society 2022-03-23 2022-04-07 /pmc/articles/PMC8996233/ /pubmed/35319892 http://dx.doi.org/10.1021/acs.jpca.2c00806 Text en © 2022 The Authors. Published by American Chemical Society https://creativecommons.org/licenses/by/4.0/Permits the broadest form of re-use including for commercial purposes, provided that author attribution and integrity are maintained (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Golibrzuch, Kai
Schwabe, Sven
Zhong, Tianli
Papendorf, Kim
Wodtke, Alec M.
Application of an Event-Based Camera for Real-Time Velocity Resolved Kinetics
title Application of an Event-Based Camera for Real-Time Velocity Resolved Kinetics
title_full Application of an Event-Based Camera for Real-Time Velocity Resolved Kinetics
title_fullStr Application of an Event-Based Camera for Real-Time Velocity Resolved Kinetics
title_full_unstemmed Application of an Event-Based Camera for Real-Time Velocity Resolved Kinetics
title_short Application of an Event-Based Camera for Real-Time Velocity Resolved Kinetics
title_sort application of an event-based camera for real-time velocity resolved kinetics
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8996233/
https://www.ncbi.nlm.nih.gov/pubmed/35319892
http://dx.doi.org/10.1021/acs.jpca.2c00806
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